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A quantum optical model for the high-order harmonic generation is presented, in which both the exciting field and the high harmonic modes are quantized, while the target material appears via parameters only. As a consequence, the model is…

High-order harmonic generation (HHG) by hydrogenlike atoms/ions in the uniform periodic electric field, formed by the two linearly polarized counterpropagating laser beams of relativistic intensities, is studied. The relativistic quantum…

原子物理 · 物理学 2011-06-14 H. K. Avetissian , A. G. Markossian , G. F. Mkrtchian

Generation of high-order harmonics in gases enabled to probe the attosecond electron dynamics in atoms and molecules with unprecedented resolution. Extending the techniques developed originally for atomic and molecular gases to solid state…

光学 · 物理学 2020-02-04 Mrudul M. S. , Nicolas Tancogne-Dejean , Angel Rubio , Gopal Dixit

High-harmonic generation is one of the most extreme nonlinear-optical processes observed to date. By focusing an intense laser pulse into a gas, the light-atom interaction that occurs during the process of ionising the atoms results in the…

Based upon our previous works (Eur.Phys.J.D 6, 319(1999); Chin.Phys.Lett. 18, 236(2001)), we develop a classical approach to calculate the high-order harmonic generation of the laser driven atoms and molecules. The Coulomb singularities in…

原子物理 · 物理学 2007-05-23 Chaohong Lee , Yiwu Duan , Wing-Ki Liu , Jian-Min Yuan , Lei Shi , Xiwen Zhu , Kelin Gao

High-order harmonic generation in polyatomic molecules generally involves multiple channels, each associated with a different orbital. Their unambiguous assignment remains a major challenge for high-harmonic spectroscopy. Here we present a…

High-harmonic generation in solids allows probing and controlling electron dynamics in crystals on few femtosecond timescales, paving the way to lightwave electronics. In the spatial domain, recent advances in the real-space interpretation…

We present a new theory that the molecular high order harmonic generation in an intense laser field is determined by molecular internal symmetry and momentum distribution of the tunneling-ionized electron. The molecular internal symmetry…

原子物理 · 物理学 2008-01-30 J. Chen , Y. J. Chen , J. Fan , J. Liu , S. G. Chen , X. T. He

The mechanism of harmonic generation in both O and X-mode configurations for a magnetized plasma has been explored here in detail with the help of Particle-In-Cell (PIC) simulations. A detailed characterization of both the reflected and…

等离子体物理 · 物理学 2021-10-27 Srimanta Maity , Devshree Mandal , Ayushi Vashistha , Laxman Prasad Goswami , Amita Das

We investigate the process of circularly polarized high harmonic generation in molecules using a bicircular laser field. In this context, we show that molecules offer a very robust framework for the production of circularly polarized…

原子物理 · 物理学 2016-06-22 F Mauger , A. D. Bandrauk , T Uzer

The generation of high-order harmonics in bulk solids subjected to intense ultrashort laser pulses has opened up new avenues for research in extreme nonlinear optics and light-matter interaction on sub-cycle timescales. Despite significant…

We consider optical high harmonic generation in a hydrogen atom confined in a breathing spherical box by considering atomic nucleus as fixed at the center of sphere. In such spherically symmetric, dynamical trap, the high harmonic…

量子物理 · 物理学 2019-02-19 S. Rakhmanov , D. Matrasulov , B. Eshchanov , V. I. Matveev

We present theoretical calculations for polarization and ellipticity of high-order harmonics from aligned N$_2$, CO$_2$, and O$_2$ molecules generated by linearly polarized lasers. Within the rescattering model, the two polarization…

原子物理 · 物理学 2010-12-13 Anh-Thu Le , R. R. Lucchese , C. D. Lin

We develop the strong-field approximation for high-order harmonic generation in hydrogen molecules, including the vibrational motion and the laser-induced coupling of the lowest two Born-Oppenheimer states in the molecular ion that is…

原子物理 · 物理学 2009-11-13 C. C. Chirila , M. Lein

A theory of ultra-fast pump-probe experiments proposed by us earlier [F.H.M. Faisal et al., Phys. Rev. Lett. 98, 143001 (2007) and F.H.M. Faisal and A. Abdurrouf, Phys. Rev. Lett. 100, 123005 (2008)] is developed here fully and applied to…

原子与分子团簇 · 物理学 2009-11-13 A. Abdurrouf , F. H. M. Faisal

The order of high harmonics emitted by an atom in an intense laser field is limited by the so-called cutoff frequency. Solving the time-dependent Schr\"odinger equation, we show that this frequency can be increased considerably by a…

原子物理 · 物理学 2016-09-08 Carla Figueira de Morisson Faria , Jan-Michael Rost

High-order harmonic generation (HHG) is combined with resonant x-ray excitation of a core electron into the transient valence vacancy that is created in the course of the HHG process. To describe this setting, I develop a…

原子物理 · 物理学 2015-10-15 Christian Buth

We investigate the orientation dependence of molecular high-order harmonic generation (HHG) both numerically and analytically. We show that the molecular recollision electronic wave packets (REWPs) in the HHG are closely related to the…

原子物理 · 物理学 2009-11-13 Yanjun. Chen , Yan. Li , Shiping. Yang , Jie. Liu

We use extreme-ultraviolet interferometry to measure the phase of high-order harmonic generation from transiently aligned CO2 molecules. We unambiguously observe a reversal in phase of the high order harmonic emission for higher harmonic…

原子物理 · 物理学 2009-11-13 Xibin Zhou , Robynne Lock , Wen Li , Nick Wagner , Margaret. M. Murnane , Henry C. Kapteyn

We investigate the polarization properties of high harmonic generation from polar molecules with a linearly polarized field. It is found that elliptically polarized harmonics are observed in a wide spectral range from the plateau to the…

光学 · 物理学 2011-12-06 Meiyan Qin , Xiaosong Zhu , Qingbin Zhang , Weiyi Hong , Peixiang Lu