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相关论文: Chemically Induced Dynamic Nuclear Polarization of…

200 篇论文

We investigate dynamic nuclear polarization in quantum point contacts (QPCs) in the integer and fractional quantum Hall regimes. Following the application of a dc bias, fractional plateaus in the QPC shift symmetrically about half filling…

介观与纳米尺度物理 · 物理学 2014-11-20 A. Kou , D. T. McClure , C. M. Marcus , L. N. Pfeiffer , K. W. West

Chemically induced dynamic nuclear polarization is a ubiquitous phenomenon in photosynthetic reaction centers. The relevant nuclear spin observables are a direct manifestation of the radical-pair mechanism. We here use quantum trajectories…

化学物理 · 物理学 2015-10-28 K. Tsampourakis , I. K. Kominis

We propose a new, more efficient, and potentially cost effective, solid-state nuclear spin hyperpolarization method combining the Cross Effect mechanism and electron spin optical hyperpolarization in rotating solids. We first demonstrate…

量子物理 · 物理学 2022-01-25 Frederic Mentink-Vigier , Vinayak Rane , Thierry Dubroca , Krishnendu Kundu

Rapid injection of spin polarization into an ensemble of nuclear spins is a problem of broad interest, spanning dynamic nuclear polarization (DNP) to quantum information science. We report on a strategy to boost the spin injection rate by…

We present dynamic nuclear polarization (DNP) in the simplest pseudospin quantum Hall ferromagnet (QHF) of an InSb two-dimensional electron gas with a large g factor using tilted magnetic fields. The DNP-induced amplitude change of a…

介观与纳米尺度物理 · 物理学 2015-05-18 H. W. Liu , K. F. Yang , T. D. Mishima , M. B. Santos , Y. Hirayama

Dynamic nuclear spin polarization (DNP) mediated by paramagnetic point defects in semiconductors is a key resource for both initializing nuclear quantum memories and producing nuclear hyperpolarization. DNP is therefore an important process…

Dynamic nuclear polarization (DNP) is an attractive method for initializing nuclear spins that are strongly coupled to optically active electron spins because it functions at room temperature and does not require strong magnetic fields. In…

Enhancing the polarization of nuclear spins surrounding the nitrogen-vacancy (NV) center in diamond has attracted widespread attention recently due to its various applications. Here we present an analytical theory and comprehensive…

量子物理 · 物理学 2016-07-15 Ping Wang , Bao Liu , Wen Yang

Effects of both the dynamic nuclear polarization (DNP) created by circularly polarized light and the fluctuations of average nuclear spin in a quantum dot (QD) on the electron spin orientation are studied for singly negatively charged InP…

介观与纳米尺度物理 · 物理学 2009-11-11 S. Yu. Verbin , B. Pal , M. Ikezawa , I. V. Ignatiev , Y. Masumoto

Nuclear spin hyperpolarization techniques, such as dynamic nuclear polarization (DNP) and parahydrogen-induced polarization (PHIP), have revolutionized nuclear magnetic resonance and magnetic resonance imaging. In these methods, a readily…

Dissolution Dynamic Nuclear Polarisation (dDNP) increases the sensitivity of magnetic resonance experiments by $>10^4$-fold, permitting isotopically-labelled molecules to be transiently visible in MRI scans. dDNP requires a source of…

The available theoretical approaches aiming at describing Dynamic Nuclear spin Polarization (DNP) in solutions containing molecules of biomedical interest and paramagnetic centers are not able to model the behaviour observed upon varying…

统计力学 · 物理学 2014-06-06 Sonia Colombo Serra , Marta Filibian , Pietro Carretta , Alberto Rosso , Fabio Tedoldi

Dynamical nuclear polarisation (DNP) is an important technique that uses polarisation transfer from electron to nuclear spins to achieve nuclear hyperpolarisation. As the electron spin of the nitrogen vacancy (NV) centres in diamond can be…

We investigated optical spin orientation and dynamic nuclear polarization (DNP) in individual self-assembled InGaAs/GaAs quantum dots (QDs) doped by a single Mn atom, a magnetic impurity providing a neutral acceptor A$^0$ with an effective…

介观与纳米尺度物理 · 物理学 2016-11-15 O. Krebs , E. Baudin , A. Lemaître

We present a quantum mechanical theory of optically induced dynamic nuclear polarization applicable to quantum dots and other interacting spin systems. The exact steady state of the optically driven coupled electron-nuclear system is…

介观与纳米尺度物理 · 物理学 2019-02-04 Thomas Nutz , Edwin Barnes , Sophia E. Economou

Polarization transfers are crucial building blocks in magnetic resonance experiments, i.e., they can be used to polarize insensitive nuclei and correlate nuclear spins in multidimensional NMR spectroscopy. The polarization can be…

化学物理 · 物理学 2022-08-24 Zhenfeng Pang , Sheetal Jain , Chen Yang , Xueqian Kong , Kong Ooi Tan

We analyze electron spin relaxation in electronic transport through coherently coupled double quantum dots in the spin blockade regime. In particular, we focus on hyperfine interaction as the spin relaxation mechanism. We pay special…

介观与纳米尺度物理 · 物理学 2015-03-13 Carlos López-Monís , Jesús Iñarrea , Gloria Platero

A sensitivity increase of two orders of magnitude in proton (1H) and carbon (13C) spins via dynamic nuclear polarization (DNP) has been accomplished recently using a compact benchtop DNP polarizer operating at 1 T and 77 K. However the DNP…

We consider the dynamic nuclear spin polarization (DNP) using two electrons in a double quantum dot in presence of external magnetic field and spin-orbit interaction, in various schemes of periodically repeated sweeps through the S-T+…

介观与纳米尺度物理 · 物理学 2015-06-17 Izhar Neder , Mark S. Rudner , Bertrand I. Halperin

Dynamic nuclear polarization (DNP) involves a polarization transfer from unpaired electrons to hyperfine coupled nuclei and can increase the sensitivity of nuclear magnetic resonance (NMR) signals by several orders of magnitude. The…

化学物理 · 物理学 2024-07-16 Gevin von Witte , Sebastian Kozerke , Matthias Ernst