相关论文: Strong-field approximation for harmonic generation…
We present a detailed comparison of theoretical approaches for modeling strong-field ionization by few-cycle laser pulses. The dipole approximation is shown to accurately capture interference structures in photoelectron spectra, while…
We investigate high-harmonic generation in closed systems, using the two-level atom as a simplified model. By means of a windowed Fourier transform of the time-dependent dipole acceleration, we extract the main contributions to this process…
In recent articles [Mishima et al., Phys. Rev. A, 66, 033401(2002); Chao, Phys. Rev. A, 72, 053414 (2005)] it was proposed to use the residue theorem for the exact calculation of the transition amplitude describing strong-field ionization…
We investigate the generation of even and odd harmonics using an intense laser and a weak second harmonic field. Our theoretical approach is based on solving the saddle-point equations within the Strong Field Approximation. The phase of the…
The generation of high harmonics is a strongly nonlinear effect that allows to probe properties of the target and to study electron dynamics in matter. It has been investigated in many different kinds of targets, including molecular gases,…
The strong-field approximation can be and has been applied in both length gauge and velocity gauge with quantitatively conflicting answers. For ionization of negative ions with a ground state of odd parity, the predictions of the two gauges…
We study theoretically the two-center interferences occurring in high harmonic generation from diatomic molecules. By solving the time-dependent Schroedinger equation, either numerically or with the molecular strong-field approximation, we…
We investigated the high-order harmonic generation (HHG) process of diatomic molecular ion $\mathrm{H}_2^+$ in non-Born-Oppenheimer approximations. The corresponding three-dimensional time-dependent Schr\"odinger equation is solved with…
This paper theoretically analyzes the behavior of an atom driven by a strong electro-magnetic field. Moreover, besides traditional quantum mechanics method, we also investigate semiclassical approaches to this problem. We first performed…
Signatures of the Coulomb corrections in the photoelectron momentum distribution during laser-induced ionization of atoms or ions in tunneling and multiphoton regimes are investigated analytically in the case of an one-dimensional problem.…
High-order harmonic generation is a powerful and sensitive tool for probing atomic and molecular structures, combining in the same measurement an unprecedented attosecond temporal resolution with a high spatial resolution, of the order of…
Accurate molecular imaging via high-order harmonic generation relies on comparing the harmonic emission from a molecule and an adequate reference system. However, an ideal reference atom with the same ionization properties as the molecule…
Long-time-integrated quantities in stochastic processes, in or out of equilibrium, usually exhibit rare but huge fluctuations. Work or heat production is such a quantity, of which the probability distribution function displays an…
The high harmonic generation from atoms in the combination of chirped laser pulse and static field is theoretically investigated. For the first time, we explore a further physical mechanism of the significant extension of high harmonic…
A theory describing above-threshold ionization of atoms and ions in a strong electromagnetic field is presented. It is based on the widely known strong field approximation and incorporates the Coulomb interaction between the photoelectron…
In present paper we develop an analytic theory for the harmonic generation of symmetric diatomic molecular ions beyond two-level model, emphasizing the influence of charge-resonance (CR) states those are strongly coupled to electromagnetic…
We present the construction of molecular force fields for small molecules (less than 25 atoms) using the recently developed symmetrized gradient-domain machine learning (sGDML) approach [Chmiela et al., Nat. Commun. 9, 3887 (2018); Sci.…
The generation of harmonics by atoms interacting with two circularly polarized and frequency related laser fields is addressed through ab initio numerical simulations. A detailed charaterization of a few specific harmonics is given. In…
We extend our recently developed semiclassical strong-field Herman-Kluk propagator (SFHK) method to calculate high-order harmonic generation (HHG) for atoms in intense lasers. We show that our method, based on a combination of the…
Molecular conformation generation aims to generate three-dimensional coordinates of all the atoms in a molecule and is an important task in bioinformatics and pharmacology. Previous methods usually first predict the interatomic distances,…