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We report photoassociative spectroscopy of $^{88}$Sr$_2$ in a magneto-optical trap operating on the ${^1S_0}\to{^3P_1}$ intercombination line at 689 nm. Photoassociative transitions are driven with a laser red-detuned by 600-2400 MHz from…

With ultracold $^{88}$Sr in a 1D magic wavelength optical lattice, we performed narrow line photoassociation spectroscopy near the $^1$S$_0 - ^3$P$_1$ intercombination transition. Nine least-bound vibrational molecular levels associated…

原子物理 · 物理学 2009-11-11 T. Zelevinsky , M. M. Boyd , A. D. Ludlow , T. Ido , J. Ye , R. Ciurylo , P. Naidon , P. S. Julienne

We present spectroscopic measurements of seven vibrational levels $v=29-35$ of the $A(1^1\Sigma_u^+)$ excited state of Li$_2$ molecules by the photoassociation of a degenerate Fermi gas of $^6$Li atoms. The absolute uncertainty of our…

原子物理 · 物理学 2013-12-17 Will Gunton , Mariusz Semczuk , Nikesh S. Dattani , Kirk W. Madison

The properties of photoassociation (PA) spectra near the intercombination line (the weak transition between $^{1}S_{0}$ and $^{3}P_{1}$ states) of group II atoms are theoretically investigated. As an example we have carried out a…

原子物理 · 物理学 2009-11-10 R. Ciurylo , E. Tiesinga , S. Kotochigova , P. S. Julienne

Photoassociation of ultracold atoms induced by chirped picosecond pulses is analyzed in a non-perturbative treatment by following the wavepackets dynamics on the ground and excited surfaces. The initial state is described by a Boltzmann…

原子与分子团簇 · 物理学 2009-06-10 Eliane Luc-Koenig , Mihaela Vatasescu , Francoise Masnou-Seeuws

We demonstrate that a near-dissociation photoassociation resonance can be used to create a deeply bound molecular sample of ultracold NaCs. To probe the resulting vibrational distribution of the sample, we use a new technique that can be…

A numerical investigation of two-laser photoassociation (PA) spectroscopy on spin-polarized metastable helium (He*) atoms is presented within the context of experimental observation of the least-bound energy level in the scattering…

其他凝聚态物理 · 物理学 2009-11-10 J. C. J. Koelemeij , M. Leduc

We observe light-induced frequency shifts in one-color photoassociative spectra of magnetically trapped $^4$He$^*$ atoms in the metastable $2^3S_1$ state. A pair of ultracold spin-polarized $2^3S_1$ helium atoms is excited into a molecular…

原子物理 · 物理学 2009-11-11 J. Kim , S. Moal , M. Portier , J. Dugué , M. Leduc , C. Cohen-Tannoudji

We investigate the formation of weakly bound, electronically excited, heteronuclear 6Li40K* molecules by single-photon photoassociation in a magneto-optical trap. We performed trap loss spectroscopy within a range of 325 GHz below the…

In this paper we introduce an electron ptychography reconstruction framework, CAVIAR -- Correlated Atomic Vibration Imaging with sub-Angstrom Resolution -- that reveals an entirely new channel of information: spatial correlations in atomic…

When the atoms of a dimer remain most of the time very far apart, in so-called long-range molecular states, their mutual interaction is ruled by plain atomic properties. The high-resolution spectroscopic study of some molecular excited…

原子物理 · 物理学 2015-05-13 Nadia Bouloufa , Anne Crubellier , Olivier Dulieu

We report the use of photoassociative spectroscopy to determine the ground state s-wave scattering lengths for the main bosonic isotopes of strontium, 86Sr and 88Sr. Photoassociative transitions are driven with a laser red-detuned by up to…

Narrow s-wave features with subthermal widths are predicted for the ^1Pi_g photoassociation spectra of cold alkaline earth atoms. The phenomenon is explained by numerical and analytical calculations. These show that only a small subthermal…

原子物理 · 物理学 2009-11-07 M. Machholm , Paul S. Julienne , K. -A. Suominen

Photoassociation, assembling molecules from atoms using laser light, is limited by the low density of atom pairs at sufficiently short interatomic separations. Here, we show that non-resonant light with intensities of the order of 10^10…

原子物理 · 物理学 2013-01-08 Rosario González-Férez , Christiane P. Koch

We report on photoassociation (PA) spectroscopy of a degenerate Fermi gas of $^{173}$Yb atoms near the dissociation limit of the spin-forbidden ${^1}S_0-{^3}P_1$ intercombination transition. An atom-loss spectrum is measured from a trapped…

原子物理 · 物理学 2018-01-10 Jeong Ho Han , Jin Hyoun Kang , Moosong Lee , Yong-il Shin

We perform a theoretical analysis to interpret the spectra of purely long-range helium dimers produced by photoassociation (PA) in an ultra-cold gas of metastable helium atoms. The experimental spectrum obtained with the PA laser tuned…

量子物理 · 物理学 2009-11-10 J. Leonard , A. P. Mosk , M. Walhout , P. Van Der Straten , M. Leduc , C. Cohen-Tannoudji

We perform photoassociation spectroscopy in an ultracold $^{23}$Na-$^6$Li mixture to study the $c^3\Sigma^+$ excited triplet molecular potential. We observe 50 vibrational states and their substructure to an accuracy of 20 MHz, and provide…

We present experimental observations of seven vibrational levels $v'=20-26$ of the $1^{3}\Sigma_{g}^{+}$ excited state of Li$_2$ molecules by the photoassociation (PA) of a degenerate Fermi gas of $^6$Li atoms. For each vibrational level,…

Photoassociation (PA) of ultracold metastable helium to the 2s2p manifold is theoretically investigated using a non-perturbative close-coupled treatment in which the laser coupling is evaluated without assuming the dipole approximation. The…

原子物理 · 物理学 2015-05-14 Daniel G. Cocks , Ian B. Whittingham

We study optical cycling in the polar free radical calcium monohydroxide (CaOH) and establish an experimental path towards scattering $\sim$$10^4$ photons. We report rovibronic branching ratio measurements with precision at the…

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