相关论文: Laser controlled molecular switches and transistor…
Optically trapped laser-cooled polar molecules hold promise for new science and technology in quantum information and quantum simulation. Large numerical aperture optical access and long trap lifetimes are needed for many studies, but these…
We propose a new approach to coherent control of transport via molecular junctions, which bypasses several of the hurdles to experimental realization of optically manipulated nanoelectronics noted in the previous literature. The method is…
We review recent progresses in the theoretical description of correlation and quantum fluctuation phenomena in charge transport through single molecules, quantum dots, and quantum wires. A variety of physical phenomena is addressed,…
For the successful implementation of organic electrochemical transistors in neuromorphic computing, bioelectronics, and real-time sensing applications it is essential to understand the factors that influence device switching times. Here we…
We apply a time-dependent perturbation theory based on unitary transformations combined with averaging techniques, on molecular orientation dynamics by ultrashort pulses. We test the validity and the accuracy of this approach on LiCl…
Polar molecules confined in an optical lattice are a versatile platform to explore spin-motion dynamics based on strong, long-range dipolar interactions. The precise tunability of Ising and spin-exchange interactions with both microwave and…
The electronic conduction of a novel, three-terminal molecular architecture, analogous to a heterojunction bipolar transistor is studied. In this architecture, two diode arms consisting of donor-acceptor molecular wires fuse through a ring,…
We demonstrate that directed transport of particles in a two dimensional driven lattice can be dynamically reversed multiple times by superimposing additional spatially localized lattices on top of a background lattice. The timescales of…
We propose and analyze a nanomechanical architecture where light is used to perform linear quantum operations on a set of many vibrational modes. Suitable amplitude modulation of a single laser beam is shown to generate squeezing,…
We propose a light emitting device with voltage controlled degree of linear polarization of emission. The device combines the ability of metasurfaces to control light with an energy-tunable light source based on indirect excitons in coupled…
The time-dependent optical properties of molecular systems are investigated by step-scan Fourier-transform spectroscopy in order to explore the dynamics at phase transitions and molecular orientation in the milli- and microsecond range. The…
We study the dynamics of two capacitively coupled quantum dots, each coupled to a lead. A Floquet Green's function approach described the system's dynamics, with the electron-electron interactions handled with the fluctuation-exchange…
We present some approaches to the computation of ultra-fast laser pulses capable of selectively breaking molecular bonds. The calculations are based on a mixed quantum-classical description: The electrons are treated quantum mechanically…
The control of ultrafast molecular rotational motion has benefited from the development of innovative techniques in strong-field laser physics. Here, we theoretically demonstrate a novel type of coherent control by inducing rotation of an…
We investigate a phase-controllable mechanism for generating optical torque in a five-level double-tripod (DT) atom-light coupling scheme interacting with four strong coherent control fields as well as two weak optical vortex probe beams…
We provide a generic scheme offering real time control of directed particle transport in superimposed driven lattices. This scheme allows to accelerate, slow and freeze the transport on demand, by switching one of the lattices subsequently…
This thesis investigates the mechanically controlled break junctions, with a particular emphasis on elucidating the behaviour of molecular currents at room temperature. The core of this experimental investigation involves a detailed…
We demonstrate a novel all-optical switch consisting of two molecules: a primary fluorophore that can be switched between a fluorescent and a dark state by light of different wavelengths, and a secondary chromophore that facilitates…
Time periodic forcing in the form of coherent radiation is a standard tool for the coherent manipulation of small quantum systems like single atoms. In the last years, periodic driving has more and more also been considered as a means for…
We introduce an all-optical approach to producing high-flux synthetic magnetic fields for neutral atoms or molecules by designing intrinsically time-periodic optical superlattices. A single laser source, modulated to generate two…