相关论文: Macrodimers: ultralong range Rydberg molecules
Vibrational properties of ultralong Rydberg Cs$_2$ molecules are investigated on corresponding potential curves obtained by perturbation theory. The Rydberg Cs$_2$ molecules are associated by a Rydberg Cs($nS/nP$) atom $(n=30-70)$ and a…
Atom-atom interactions within a small volume were investigated through the excitation of ultracold Rb atoms. The application of microwaves enhances these interactions, causing the suppression of Rydberg state excitation. The suppression of…
Recent studies of strong interaction effects in kaonic atoms suggest that analysing so-called `lower' and `upper' levels in the same atom could separate one-nucleon absorption from multinucleon processes. The present work examines the…
Obtaining full control over the internal and external quantum states of molecules is the central goal of ultracold chemistry and allows for the study of coherent molecular dynamics, collisions and tests of fundamental laws of physics. When…
We present methods for accurate evaluation of van der Waals coefficients of dimers with excited atoms that have a strong decay channel. We calculate C_6 coefficients for the Yb-Yb 1S_0+ 3P_{0,1}, 3P_0+3P_0 and Yb-Rb 3P_1+5s, 1S_0+ 5p_{1/2}…
Ultralong-range Rydberg molecules provide an exciting testbed for molecular physics at exaggerated scales. In the so-called trilobite and butterfly Rydberg molecules, the Born-Oppenheimer approximation can fail due to strong non-adiabatic…
Long-range $(n+2)D_{5/2} \, nF_J$ Rydberg macro-dimers are observed in an ultracold cesium Rydberg gas for $39\leq n\leq48$. Strong dipolar "flip" ($\langle D_{5/2} F_{5/2} \vert \hat{V}_{dd} \vert F_{5/2} D_{5/2} \rangle$, $\langle D_{5/2}…
Rydberg atoms, with their giant electronic orbitals, exhibit dipole-dipole interaction reaching the GHz range at a distance of a micron, making them a prominent contender for realizing quantum operations well within their coherence time.…
Combining the measured binding energies of four of the most weakly bound rovibrational levels of the $^{87}$Rb$_2$ molecule with the results of two other recent high-precision rubidium experiments, we obtain exceptionally strong constraints…
Rydberg atoms, with one highly-excited, nearly-ionized electron, have extreme sensitivity to electric fields, including microwave fields ranging from 100 MHz to over 1 THz. Here we show that room-temperature Rydberg atoms can be used as…
Ultralong-range Rydberg molecules (ULRM) are highly imbalanced bound systems formed via the low-energy scattering of a Rydberg electron with a ground-state atom. We investigate for $^{23}$Na the $d$-state and the energetically close-by…
Rydberg atoms excited by cold blackbody radiation are shown to display long-lived quantum coherences on timescales of tens of picoseconds. By solving non-Markovian equations of motion with no free parameters we obtain the time evolution of…
The coupling of an isolated quantum state to a continuum is typically associated with decoherence and decreased lifetime. Here, we demonstrate that Rydberg macrodimers, weakly bound pairs of Rydberg atoms, can overcome this dissipative…
The exceptionally large polarisability of highly excited Rydberg atoms (six orders of magnitude higher than ground-state atoms) makes them of great interest in fields such as quantum optics, quantum computing, quantum simulation and…
We investigate the impact of an electric field on the structure of ultralong-range polar diatomic Rydberg molecules. Both the s-wave and p-wave interactions of the Rydberg electron and the neutral ground state atom are taken into account.…
A non-resonant microwave dressing field at 38.465 GHz was used to eliminate the static electric dipole moment difference between the $49s_{1/2}$ and $48s_{1/2}$ Rydberg states of $^{87}$Rb in dc fields of approximately 1 V/cm. The reduced…
Quantum sensing has attracted significant attention due to its ability to measure physical quantities with extremely high accuracy. Rydberg atoms - typically alkali atoms with a highly excited valence electron that is far from the nucleus -…
We introduce a novel method to engineer sharply peaked, distance-selective interactions between neutral atoms by exploiting interaction-induced resonances within a resonantly driven Rydberg ladder system. By tuning laser parameters, a…
We propose a novel experimental method to extend the investigation of ion-atom collisions from the so far studied cold, essentially classical regime to the ultracold, quantum regime. Key aspect of this method is the use of Rydberg molecules…
Rydberg molecules, often exemplified by long-range "trilobite" molecules, are a subject of much recent interest at high principal quantum number $n$. States that use the same bonding mechanism can exist at much lower $n$ and less-extreme…