相关论文: Coherent Control of Multiphoton Transitions with F…
By applying phase modulation across different frequencies, metasurfaces possess the ability to manipulate the temporal dimension of photons at the femtosecond scale. However, there remains a fundamental challenge to shape the single…
We present an experiment demonstrating high-resolution coherent control of a four-level atomic system in a closed (diamond) type configuration. A femtosecond frequency comb is used to establish phase coherence between a pair of two-photon…
We report on the demonstration of a femtosecond all-optical modulator providing, without nonlinearity and therefore at arbitrarily low intensity, ultrafast light-by-light control. The device engages the coherent interaction of optical waves…
An outstanding goal in quantum optics is the realization of fast optical non-linearities at the single-photon level. Such non-linearities would allow for the realization of optical devices with new functionalities such as a single-photon…
We demonstrate for the first time coherent control of bond making, a milestone on the way to coherent control of photo-induced bimolecular chemical reactions. In strong-field multiphoton femtosecond photoassociation experiments, we find the…
The induction of dc electronic transport in rigid and flexible trans-polyacetylene oligomers according to the $\omega$ vs. $2\omega$ coherent control scenario is investigated using a quantum-classical mean field approximation. The approach…
Selective control of decoherence is demonstrated for a multilevel system by generalizing the instantaneous phase of any chirped pulse as individual terms of a Taylor series expansion. In the case of a simple two-level system, all odd terms…
The underlying mechanisms for one photon phase control are revealed through a master equation approach. Specifically, two mechanisms are identified, one operating on the laser time scale and the other on the time scale of the system-bath…
In this survey, we first introduce quantum fields and open quantum systems, then we present continuous-mode single-photon states and discuss discrete measurements of a single-photon field. After that, we introduce linear quantum systems and…
We report the experimental demonstration of coherent control with high power, broadband squeezed vacuum. Although incoherent and exhibiting the statistics of a thermal noise, broadband squeezed vacuum is shown to induce certain two-photon…
We propose an efficient all-optical phase modulation based on a double-{\Lambda} system and demonstrate a {\pi} phase shift of a few-photon pulse induced by another few-photon pulse in cold rubidium atoms with this scheme. By changing the…
Recent experimental techniques in multicolor waveform synthesis allow the temporal shaping of strong femtosecond laser pulses with applications in the control of quantum mechanical processes in atoms, molecules, and nanostructures.…
Coherent generation of indistinguishable single photons is crucial for many quantum communication and processing protocols. Solid-state realizations of two-level atomic transitions or three-level spin-$\Lambda$ systems offer significant…
The recent development of ultrafast extreme ultraviolet (XUV) coherent light sources bears great potential for a better understanding of the structure and dynamics of matter. Promising routes are advanced coherent control and nonlinear…
Control over the joint spectral amplitude of a photon pair has proved highly desirable for many quantum applications, since it contains the spectral quantum correlations, and has crucial effects on the indistinguishability of photons, as…
Attosecond science promises to reveal the most fundamental electronic dynamics occurring in matter and it can develop further by meeting two linked technological goals related to high-order harmonic sources: higher photon flux (permitting…
Femtosecond time-resolved x-ray diffraction is employed to study the dynamics of the periodic lattice distortion (PLD) associated with the charge-density-wave (CDW) in K0.3MoO3. Using a multi-pulse scheme we show the ability to extend the…
Intensive light pulse interaction with a dense resonant medium is considered. The possibilities of optical switching and pulse compression at realistic parameters of the medium are analyzed. Pulse shape transformation in different photonic…
Semiconductor quantum dots are excellent candidates for ultrafast coherent manipulation of qubits by laser pulses on picosecond timescales or even faster. In inhomogeneous ensembles a macroscopic optical polarization decays rapidly due to…
We have studied the effects of chirped femtosecond laser pulses on the formation of ultracold molecules in a Rb magneto-optical trap. We have found that application of chirped femtosecond pulses suppressed the formation of 85Rb-2 and 87Rb-2…