相关论文: Basic characterization of highly enriched uranium …
The 232U content of various uranium-bearing items was measured using low-background gamma spectrometry. The method is independent of the measurement geometry, sample form and chemical composition. Since 232U is an artificially produced…
A non-destructive, gamma-spectrometric method for uranium age-dating is presented which is applicable to material of any physical form and geometrical shape. It relies on measuring the daughter/parent activity ratio 214Bi/234U by…
A non-destructive, gamma-spectrometric method for verifying the plutonium content of Pu-Be neutron sources has been developed. It is also shown that the isotopic composition and the age of plutonium (Pu) can be determined in the intensive…
Every country that has made nuclear weapons has used uranium enrichment. Despite the centrality of this technology to international security, there is still no reliable physical marker of past enrichment that can be used to perform forensic…
Spatially resolved analysis of uranium isotopes in small volumes of actinide-bearing materials is critical for a variety of technical disciplines, including earth and planetary sciences, environmental monitoring, bioremediation, and the…
Four methods for determining the composition of low-level uranium- and thorium-chain surface contamination are presented. One method is the observation of Cherenkov light production in water. In two additional methods a position-sensitive…
Antineutrino spectra of fissile isotopes calculated using summation method being used to fit experimental spectra got in several experiments. Summation method was used with the possibility of changing individual spectrum shape of unknown…
The alpha-radiometric determination of uranium after its pre-concentration from natural water samples using the cation-exchange resin Chelex-100, its selective extraction by tributylphosphate and electrodeposition on stainless steel discs…
We study Uranium isotopes and surrounding elements at very large neutron number excess. Relativistic mean field and Skyrme-type approaches with different parametrizations are used in the study. Most models show clear indications for…
The atomic mass of uranium-238 has been determined to be $238.050\,787\,618(15)\,\text{u}$, improving the literature uncertainty by two orders of magnitude. It is obtained from a measurement of the mass ratio of $^{238}$U$^{47+}$ and…
In recent work [Vavrek et al. (2025)], we developed the performance optimization framework spectre-ml for gamma spectrometers with variable performance across many readout channels. The framework uses non-negative matrix factorization (NMF)…
The smuggling of special nuclear materials (SNMs) across national borders is becoming a serious threat to nuclear nonproliferation. This paper presents a feasibility study on the rapid interrogation of concealed SNMs by combining scattering…
Neutron Resonance Transmission Analysis (NRTA) was explored as an arms control verification approach to support potential future nuclear weapon limiting treaties. A compact and portable neutron Time of Flight (ToF) system was developed to…
A distributed uranium source with the accurately certified activity of 238U has been used to verify the effective mass of the HPGe detector intended for the {\nu}GeN neutrino experiment. The source, dissolved in nitric acid, provides…
The ages of the oldest stars shed light on the birth, chemical enrichment, and chemical evolution of the Universe. Nucleocosmochronometry provides an avenue to determining the ages of these stars independent from stellar evolution models.…
We carried out calculations of the energies and magnetic dipole hyperfine structure constants of the low-lying states of 233U^+ and 233U using two different approaches. With six valence electrons and a very heavy core, uranium represents a…
We test common fluence diagnostics in the regime of very low burnup natural uranium reactor samples. The fluence diagnostics considered are the uranium isotopics ratios $^{235}$U/$^{238}$U and $^{236}$U/$^{235}$U, for which we find simple…
In nuclear fuel cycles, an enrichment facility typically provides low enriched uranium (LEU) to a number of customers. We consider monitoring an enrichment facility to timely detect a possible diversion of highly enriched uranium (HEU). To…
A method is presented for the identification of high-energy neutrinos from gamma ray bursts by means of a large-scale neutrino telescope. The procedure makes use of a time profile stacking technique of observed neutrino induced signals in…
Nuclear security operations and forensic investigations require the utilization of a suite of instruments ranging from passive gamma spectrometers to high-precision laboratory sample analyzers. Gamma spectroscopy survey is further broken…