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The distribution of monomers along a linear polymer grafted on a hard wall is modelled by determining the probability distribution of occupied vertices of Dyck and ballot path models of adsorbing linear polymers. For example, the…

软凝聚态物质 · 物理学 2023-03-08 EJ Janse van Rensburg

In view of recent intense experimental and theoretical interests in the biophysics of liquid-liquid phase separation (LLPS) of intrinsically disordered proteins (IDPs), heteropolymer models with chain molecules configured as self-avoiding…

生物大分子 · 定量生物学 2018-08-30 Suman Das , Adam Eisen , Yi-Hsuan Lin , Hue Sun Chan

We study the elastic properties of a single A/B copolymer chain with a specific sequence. We predict a rich structure in the force extension relations which can be addressed to the sequence. The variational method is introduced to probe…

软凝聚态物质 · 物理学 2009-11-07 Namkyung Lee , Thomas A. Vilgis

We have studied both experimentally and theoretically the surface pressure isotherms of copolymers of polystyrene-polyethyleneoxide (PS-PEO) at the air-water interface. The SCMF (single chain mean-field) theory provides a very good…

软凝聚态物质 · 物理学 2009-10-30 M. C. Fauré , P. Bassereau , M. A. Carignano , I. Szleifer , Y. Gallot , D. Andelman

The effect of ambient disorders and sequence heterogeneities on the reptation of a long polymer is studied with the aid of a disordered tube model. The dynamics of a random heteropolymer is found to be much slower than that of a homopolymer…

软凝聚态物质 · 物理学 2009-10-30 D. Cule , T. Hwa

Adsorption of polymers to surfaces is crucial for understanding many fundamental processes in nature. Recent experimental studies indicate that the adsorption dynamics is dominated by non-equilibrium effects. We investigate the adsorption…

软凝聚态物质 · 物理学 2009-05-12 Debabrata Panja , Gerard T. Barkema , Anatoly B. Kolomeisky

We study the depinning phase transition of a directed polymer in a $d$-dimensional space by a periodic potential localized on a straight line. We give exact formulas in all dimensions for the critical pinning we need to localize the…

凝聚态物理 · 物理学 2009-10-28 S. Galluccio , R. Graber

An infinite hierarchy of layering transitions exists for model polymers in solution under poor solvent or low temperatures and near an attractive surface. A flat histogram stochastic growth algorithm known as FlatPERM has been used on a…

统计力学 · 物理学 2009-11-10 J. Krawczyk , A. L. Owczarek , T. Prellberg , A. Rechnitzer

Molecules at the air-water interface often form inhomogeneous layers in which domains of different densities are separated by sharp interfaces. Complex interfacial pattern formation may occur through the competition of short- and long-range…

patt-sol · 物理学 2009-10-30 David K. Lubensky , Raymond E. Goldstein

A binary mixture of oppositely charged components confined to a plane such as cationic and anionic lipid bilayers may exhibit local segregation. The relative strength of the net short range interactions, which favors macroscopic…

软凝聚态物质 · 物理学 2009-11-11 Sharon M. Loverde , Yury S. Velichko , Monica Olvera de la Cruz

We develop a general analysis of the diffusive dynamics of polydisperse polymers in the presence of chemical potential gradients, within the context of the tube model (with all species entangled). We obtain a set of coupled dynamical…

软凝聚态物质 · 物理学 2009-11-07 I. Pagonabarraga , M. E. Cates

We consider forces acting on objects immersed in, or attached to, long fluctuating polymers. The confinement of the polymer by the obstacles results in polymer-mediated forces that can be repulsive (due to loss of entropy) or attractive (if…

统计力学 · 物理学 2017-08-28 Yacov Kantor , Mehran Kardar

We discuss various aspects of the randomly interacting directed polymers with emphasis on the phases and phase transition. We also discuss the behaviour of overlaps of directed paths in a random medium.

凝聚态物理 · 物理学 2015-06-25 Somendra M. Bhattacharjee , Sutapa Mukherji

The phase behavior of a cross-linked polymer blend made of two incompatible species, $A$ and $B$, of different chemical nature is analyzed. Besides a homogeneous phase, this system also exhibits two microphases and a phase of total…

凝聚态物理 · 物理学 2007-05-23 Edilson Vargas , Marcia C. Barbosa

We study the phase transitions of a random copolymer chain with quenched disorder. We apply a replica variational approach based on a Gaussian trial Hamiltonian in terms of the correlation functions of monomer Fourier coordinates. This…

无序系统与神经网络 · 物理学 2009-10-30 A. Moskalenko , Yu. A. Kuznetsov , K. A. Dawson

The coupled dynamics of entangled polymers which span a broad time and length scales govern the unique viscoelastic properties of polymers. To follow chain mobility by numerical simulations from the intermediate Rouse and reptation regimes…

软凝聚态物质 · 物理学 2016-11-03 Gary S. Grest

These lecture notes are a guided tour through the fascinating world of polymer chains interacting with themselves and/or with their environment. The focus is on the mathematical description of a number of physical and chemical phenomena,…

概率论 · 数学 2012-05-16 Francesco Caravenna , Frank den Hollander , Nicolas Pétrélis

We study the translocation of a semiflexible polymer through extended pores with patterned stickiness, using Langevin dynamics simulations. We find that the consequence of pore patterning on the translocation time dynamics is dramatic and…

软凝聚态物质 · 物理学 2018-05-02 Rajneesh Kumar , Abhishek Chaudhuri , Rajeev Kapri

Dynamics of a discrete polymer in time-dependent external potentials is studied with the master equation approach. We consider both stochastic and deterministic switching mechanisms for the potential states and give the essential equations…

统计力学 · 物理学 2008-06-25 Janne Kauttonen , Juha Merikoski , Otto Pulkkinen

We make use of the previously developed formalism for a monomer ensemble and include angular dependence of the segments of the polymer chains thus described. In particular we show how to deal with stiffness when the polymer chain is…

软凝聚态物质 · 物理学 2015-06-24 K. K. Muller-Nedebock , H. L. Frisch , J. K. Percus