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We report a synchrotron x-ray scattering study of the diluted spin-Peierls (SP) material Cu_{1-x}Mg_xGeO_3. In a recent paper we have shown that the SP dimerization attains long-range order only for x < x_c = 0.022(0.001). Here we report…

强关联电子 · 物理学 2009-10-31 V. Kiryukhin , Y. J. Wang , S. C. LaMarra , R. J. Birgeneau , T. Masuda , I. Tsukada , K. Uchinokura

We report comprehensive synchrotron x-ray scattering and magnetic susceptibility studies of the doped spin-Peierls materials Cu_{1-x}Zn_xGeO_3 and CuGe_{1-y}Si_yO_3. Temperature versus dopant concentration phase diagrams are mapped out for…

In doped CuGeO3 systems, such as (Cu1-xZnx)GeO3 and Cu(Ge1-xSix)O3, the spin-Peierls (SP) ordering (T<Tsp) coexists with the antiferromagnetic (AF) phase (T<TN<Tsp). Tsp decreases while TN increases with increasing x in low doping region.…

材料科学 · 物理学 2009-10-31 H. Nakao , M. Nishi , Y. Fujii , T. Masuda , I. Tsukada , K. Uchinokura , K. Hirota , G. Shirane

Neutron scattering measurements on a large single crystal of CuGeO$_3$ have been used to determine the temperature-dependence of the spin-Peierls energy gap. While the power law behavior of the intensity of structural superlattice peaks is…

凝聚态物理 · 物理学 2009-10-28 Michael C. Martin , G. Shirane , Y. Fujii , M. Nishi , O. Fujita , J. Akimitsu , M. Hase , K. Uchinokura

Using Raman scattering we studied the effect of substitutions on 1D spin fluctuations in CuGeO_3 observed as a spinon continuum in frustration induced exchange scattering. For temperatures below the spin-Peierls transition (T_{SP}=14K) the…

强关联电子 · 物理学 2016-08-31 M. Fischer , P. Lemmens , G. Güntherodt , M. Weiden , W. Richter , C. Geibel , F. Steglich

Raman experiments on the spin-Peierls compound CuGeO$_3$ and the substituted (Cu$_{1- x}$,Zn$_x$)GeO$_3$ and Cu(Ge$_{1-x}$,Ga$_x$)O$_3$ compounds were performed in order to investigate the response of specific magnetic excitations of the…

A series of high-quality single crystals of Cu$_{1-x}$Zn$_x$GeO$_3$ have been examined by neutron scattering techniques. An antiferromagnetic (AF) ordering is confirmed for samples with $x\geq 0.02$, in complete agreement with previous…

凝聚态物理 · 物理学 2009-10-28 Y. Sasago , N. Koide , K. Uchinokura , Michael C. Martin , M. Hase , K. Hirota , G. Shirane

We have measured the magnetic susceptibility of single-crystal Cu_{1-x}Ni_xGeO_3 to study doping effects of the magnetic impurity (Ni^{2+} has S=1 spin) on the inorganic spin-Peierls (SP) material CuGeO_3. We observed the disappearance of…

强关联电子 · 物理学 2007-05-23 N. Koide , Y. Uchiyama , T. Hayashi , T. Masuda , Y. Sasago , K. Uchinokura , K. Manabe , H. Ishimoto

Comprehensive neutron scattering studies were carried out on a series of high-quality single crystals of Cu_{1-x}Zn_xGeO_3. The Zn concentration, x, was determined for each sample using Electron Probe Micro-Analysis. The measured Zn…

强关联电子 · 物理学 2009-10-30 Michael C. Martin , M. Hase , K. Hirota , G. Shirane , Y. Sasago , N. Koide , K. Uchinokura

Single crystals of the lightly-doped spin-Peierls system Cu(1-x)Cd(x)GeO3 have been studied using bulk susceptibility, x-ray diffraction, and inelastic neutron scattering techniques. We investigate the triplet gap in the magnetic excitation…

强关联电子 · 物理学 2009-11-13 S. Haravifard , K. C. Rule , H. A. Dabkowska , B. D. Gaulin , Z. Yamani , W. J. L. Buyers

We have measured temperature dependence of low-frequency Raman spectra in CuGeO$_3$, and have observed the quasi-elastic scattering in the $(c,c)$ polarization above the spin-Peierls transition temperature. We attribute it to the…

We discovered a first-order phase transition between dimerized-antiferromagnetic and uniform-antiferromagnetic phases in impurity-doped spin-Peierls (SP) cuprate Cu{1-x}MgxGeO3. As impurity concentration increases, linear reduction of SP…

强关联电子 · 物理学 2009-09-25 T. Masuda , A. Fujioka , Y. Uchiyama , I. Tsukada , K. Uchinokura

The influence of non-magnetic impurities on the spectrum and dynamical spin structure factor of a model for CuGeO$_3$ is studied. A simple extension to Zn-doped ${\rm Sr Cu_2 O_3}$ is also discussed. Using Exact Diagonalization techniques…

凝聚态物理 · 物理学 2016-08-15 George Martins , Elbio Dagotto , José Riera

The thermal conductivity $\kappa$ is measured in a series of Cu_1-xMg_xGeO_3 single crystals in magnetic fields up to 16 T. It has turned out that heat transport by spin excitations is coherent for lightly doped samples, in which the…

强关联电子 · 物理学 2009-10-31 J. Takeya , I. Tsukada , Yoichi Ando , T. Masuda , K. Uchinokura

X-ray scattering measurements on single crystals of TiOCl reveal the presence of commensurate dimerization peaks within both the incommensurate spin-Peierls phase and the so-called pseudogap phase above T_c2. This scattering is relatively…

强关联电子 · 物理学 2016-08-05 J. P. Clancy , B. D. Gaulin , K. C. Rule , J. P. Castellan , F. C. Chou

Temperature ($2.3<T<40$\ K) and magnetic field ($0<B<17$\ T) dependent far infrared absorption spectroscopy on the spin-Peierls coumpound CuGeO$_3$\ has revealed several new absorption processes in both the dimerised and high field phase of…

凝聚态物理 · 物理学 2009-10-28 P. H. M. van Loosdrecht , S. Huant , G. Martinez , G. Dhalenne , A. Revcolevschi

Pressure and temperature dependent susceptibility and Raman scattering experiments on single crystalline Cu_xZn_(1-x)GeO_3 have shown an unusually strong increase of the spin-Peierls phase transition temperature upon applying hydrostatic…

We report on a zero-field 63Cu nuclear quadrupole resonance (NQR) study of nonmagnetic Mg impurity substituted Cu1-xMgxGeO3 (single crystals; the spin-Peierls transition temperature Tsp~14, 13.5, and 11 K for x=0, 0.0043, and 0.020) in a…

强关联电子 · 物理学 2009-11-07 Y. Itoh , T. Machi , N. Koshizuka , T. Masuda , K. Uchinokura

The uniaxial pressure dependences of the exchange coupling and the structural distortion in the dimerized phase of CuGeO$_3$ are analyzed. A minimum magnetic dimerization of 3 % is obtained, incompatible with an adiabatic approach to the…

凝聚态物理 · 物理学 2009-10-31 B. Büchner , H. Fehske , A. P. Kampf , G. Wellein

We report a high-resolution resonant inelastic soft x-ray scattering study of the quantum magnetic spin-chain materials Li2CuO2 and CuGeO3. By tuning the incoming photon energy to the oxygen K-edge, a strong excitation around 3.5 eV energy…

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