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We have performed detailed magnetic susceptibility measurements as well as synchrotron x-ray diffraction studies to determine the temperature vs concentration ($T$ - $x$) phase diagram of Cu${}_{1-x}$Mg${}_x$GeO${}_3$. We observe clear…

强关联电子 · 物理学 2009-10-31 T. Masuda , I. Tsukada , K. Uchinokura , Y. J. Wang , V. Kiryukhin , R. J. Birgeneau

We have measured the magnetic susceptibility of single-crystal Cu_{1-x}Ni_xGeO_3 to study doping effects of the magnetic impurity (Ni^{2+} has S=1 spin) on the inorganic spin-Peierls (SP) material CuGeO_3. We observed the disappearance of…

强关联电子 · 物理学 2007-05-23 N. Koide , Y. Uchiyama , T. Hayashi , T. Masuda , Y. Sasago , K. Uchinokura , K. Manabe , H. Ishimoto

A series of high-quality single crystals of Cu$_{1-x}$Zn$_x$GeO$_3$ have been examined by neutron scattering techniques. An antiferromagnetic (AF) ordering is confirmed for samples with $x\geq 0.02$, in complete agreement with previous…

凝聚态物理 · 物理学 2009-10-28 Y. Sasago , N. Koide , K. Uchinokura , Michael C. Martin , M. Hase , K. Hirota , G. Shirane

The impurity induced antiferromagnetic ordering of the doped spin-Peierls magnet Cu(1-x)Mg(x)GeO(3) was studied by ESR technique. Crystals with the Mg concentration x<4% demonstrate a coexistence of paramagnetic and antiferromagnetic ESR…

强关联电子 · 物理学 2009-11-07 V. N. Glazkov , A. I. Smirnov , K. Uchinokura , T. Masuda

We report a synchrotron x-ray scattering study of the diluted spin-Peierls (SP) material Cu_{1-x}Mg_xGeO_3. In a recent paper we have shown that the SP dimerization attains long-range order only for x < x_c = 0.022(0.001). Here we report…

强关联电子 · 物理学 2009-10-31 V. Kiryukhin , Y. J. Wang , S. C. LaMarra , R. J. Birgeneau , T. Masuda , I. Tsukada , K. Uchinokura

In doped CuGeO3 systems, such as (Cu1-xZnx)GeO3 and Cu(Ge1-xSix)O3, the spin-Peierls (SP) ordering (T<Tsp) coexists with the antiferromagnetic (AF) phase (T<TN<Tsp). Tsp decreases while TN increases with increasing x in low doping region.…

材料科学 · 物理学 2009-10-31 H. Nakao , M. Nishi , Y. Fujii , T. Masuda , I. Tsukada , K. Uchinokura , K. Hirota , G. Shirane

We have measured the magnetic susceptibilities of single crystals of Cu_{1-x}Zn_xGeO_3 with extremely low Zn concentration (x) lower than x=5x10^{-3} at very low temperatures to investigate the spin-Peierls and antiferromagnetic…

强关联电子 · 物理学 2009-10-31 K. Manabe , H. Ishimoto , N. Koide , Y. Sasago , K. Uchinokura

The fraction of the paramagnetic phase surviving at the impurity-induced antiferromagnetic order transition of the doped spin-Peierls magnet Cu(1-x)Mg(x)GeO3 (x < 5%) is found to increase with an external magnetic field. This effect is…

强关联电子 · 物理学 2009-11-10 V. N. Glazkov , A. I. Smirnov , H. -A. Krug von Nidda , A. Loidl , K. Uchinokura , T. Masuda

We report comprehensive synchrotron x-ray scattering and magnetic susceptibility studies of the doped spin-Peierls materials Cu_{1-x}Zn_xGeO_3 and CuGe_{1-y}Si_yO_3. Temperature versus dopant concentration phase diagrams are mapped out for…

Comprehensive neutron scattering studies were carried out on a series of high-quality single crystals of Cu_{1-x}Zn_xGeO_3. The Zn concentration, x, was determined for each sample using Electron Probe Micro-Analysis. The measured Zn…

强关联电子 · 物理学 2009-10-30 Michael C. Martin , M. Hase , K. Hirota , G. Shirane , Y. Sasago , N. Koide , K. Uchinokura

Magnetic phase transition under hydrostatic pressure in TlCu$_{0.988}$Mg$_{0.012}$Cl$_3$ was investigated by magnetization measurements. The parent compound TlCuCl$_3$ is a coupled spin dimer system, which undergoes a pressure-induced…

强关联电子 · 物理学 2009-11-11 H. Imamura , T. Ono , K. Goto , H. Tanaka

We report on a zero-field 63Cu nuclear quadrupole resonance (NQR) study of nonmagnetic Mg impurity substituted Cu1-xMgxGeO3 (single crystals; the spin-Peierls transition temperature Tsp~14, 13.5, and 11 K for x=0, 0.0043, and 0.020) in a…

强关联电子 · 物理学 2009-11-07 Y. Itoh , T. Machi , N. Koshizuka , T. Masuda , K. Uchinokura

We study the S=1/2 Heisenberg antiferromagnet on a square lattice with nearest-neighbor and plaquette four-spin exchanges (introduced by A.W. Sandvik, Phys. Rev. Lett. {\bf 98}, 227202 (2007).) This model undergoes a quantum phase…

强关联电子 · 物理学 2009-11-14 Valeri N. Kotov , Dao-Xin Yao , A. H. Castro Neto , D. K. Campbell

The interest in the study of spin-Peierls phenomenon has increased with the discovery of copper germanium oxide (CuGeO_3) as an example of spin-Peierls systems. The availability of this inorganic compound as large, high quality single…

强关联电子 · 物理学 2007-05-23 J. Srivatsava

The phase transition in the compound LiVGe2O6 has been proposed as a unique example of a spin-Peierls transition in an S=1 antiferromagnetic chain. We report neutron and x-ray diffraction measurements of LiVGe2O6 above and below the phase…

强关联电子 · 物理学 2009-10-31 M. D. Lumsden , G. E. Granroth , D. Mandrus , S. E. Nagler , J. R. Thompson , J. P. Castellan , B. D. Gaulin

We study the competition between the spin-Peierls and the antiferromagnetic ordering in disordered quasi-one-dimensional spin systems. We obtain the temperature vs disorder-strength phase diagram, which qualitatively agrees with recent…

凝聚态物理 · 物理学 2009-10-30 Maxim Mostovoy , Daniel Khomskii , Jasper Knoester

This study rigorously investigates the phenomenon of a pseudo-transition in a minimal spinpseudospin model, serving as a simplified model of one-dimensional cuprate chains [CuO]n, by making use of the transfer-matrix method. The studied…

统计力学 · 物理学 2024-09-10 Jozef Strecka , Katarina Karlova

We report a synchrotron x-ray scattering study of the diluted spin-Peierls (SP) material Cu_(1-x)Mg_xGeO_3. We find that for x>0 the temperature T_m at which the spin gap is established is significantly higher than the temperature T_s at…

强关联电子 · 物理学 2009-10-31 Y. J. Wang , V. Kiryukhin , R. J. Birgeneau , T. Masuda , I. Tsukada , K. Uchinokura

The spin-Peierls transition is modeled in the dimer phase of the spin-$1/2$ chain with exchanges $J_1$, $J_2 = \alpha J_1$ between first and second neighbors. The degenerate ground state generates an energy cusp that qualitatively changes…

强关联电子 · 物理学 2019-07-09 Sudip Kumar Saha , Manoranjan Kumar , Zoltán G. Soos

Measurements of magnetic susceptibility, heat capacity and thermal expansion are reported for single crystalline CuSb$_{2}$O$_{6}$ in the temperature range $5<T<350$ K. The magnetic susceptibility exhibits a broad peak centered near 60 K…

强关联电子 · 物理学 2015-06-16 A. Rebello , M. G. Smith , J. J. Neumeier , B. D. White , Yi-Kuo Yu
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