相关论文: Vibrational Study of 13C-enriched C60 Crystals
The infrared bar-spectrum of a single ammonia molecule encapsulated in nano-cage C$_{60}$ fullerene molecule is modelled using the site inclusion model successfully applied to analyze spectra of CO$_2$ isotopologues isolated in rare gas…
The bremsstrahlung cross section for relativistic electrons in a crystal is split into the sum of coherent and incoherent parts (the last is due to a thermal motion of atoms in the crystal). Although the spectrum of incoherent radiation in…
We present polarization resolved Raman scattering study of surface vibration modes in the topological insulator Bi$_2$Se$_3$ single crystal and thick films. Besides the four Raman active bulk phonons, we observed four additional modes with…
Diamond is studied by path integral molecular dynamics simulations of the atomic nuclei in combination with a tight-binding Hamiltonian to describe its electronic structure and total energy. This approach allows us to quantify the influence…
The vibronic coupling effect in nitrogen 1s X-ray photoelectron spectra (XPS) was systematically studied for a family of 17 bicyclic indole molecules by combining Franck-Condon simulations (including the Duschinsky rotation effect) and…
We introduce new symmetry-based methods to test for isotropy in cosmic microwave background radiation. Each angular multipole is factored into unique products of power eigenvectors, related multipoles and singular values that provide 2 new…
The control of non-equilibrium phenomena in complex solids is an important research frontier, encompassing new effects like light induced superconductivity. Here, we show that coherent optical excitation of molecular vibrations in the…
The halide double perovskite Cs$_2$AgBiBr$_6$ has been proposed as a potential replacement for organic halide perovskites for photovoltaic applications. Further investigation of its dielectric response, optical properties and structural…
Despite decades of intensive experimental and theoretical efforts, the physics of cuprate high-temperature superconductors in general, and, in particular, their normal state, is still under debate. Here, we report our investigation of…
We present a new analysis of the pairing vibrations around 56Ni, with emphasis on odd-odd nuclei. This analysis of the experimental excitation energies is based on the subtraction of average properties that include the full symmetry energy…
Modelling ultra-low-noise far-infrared grating spectrometers has become crucial for the next generation of far-infrared space observatories. Conventional techniques are awkward to apply because of the partially coherent form of the incident…
We study the spectrum of vibrational modes in metal nanoparticles with a dielectric core. Vibrational modes are excited by the rapid heating of the particle lattice that takes place after laser excitation, and can be monitored by means of…
Our understanding of vibrations in solids currently rests on concepts and techniques designed for crystals and explicitly relying on periodicity, hence inapplicable to amorphous materials. As a consequence, no established framework enables…
We examined the Fourier power spectrum characteristics of cirrus structures in 13 sky fields with faint to bright cirrus emission observed with ISOPHOT in the 90--200µm wavelength range in order to study variations of the spectral…
In the present work the authors report results of broadband dielectric spectroscopy on various samples of CaCu3Ti4O12, including so far only rarely investigated single crystalline material. The measurements extend up to 1.3 GHz, covering…
Detonation of a three-dimensional reactive non-isotropic molecular crystal is modeled using molecular dynamics simulations. The detonation process is initiated by an impulse, followed by the creation of a stable fast reactive shock wave.…
The observed anisotropies of surface vibrations for unreconstructed FCC metal (110) surfaces are often reversed from the "common sense" expectation. The source of these reversals is investigated by performing ab initio density functional…
Dynamical decoupling multipulse sequences can be applied to solid state spins for sensing weak oscillating fields from nearby single nuclear spins. By periodically reversing the probing system's evolution, other noises are counteracted and…
We have taken K-band spectroscopy of a sample of 13 pre-CVs in order to examine them for anomalous chemical abundances. In particular, we study the strength of the 12CO and 13CO absorption bands that have been found diminished and enhanced,…
The GRIFFIN spectrometer at TRIUMF-ISAC has been used to study excited states and transitions in $^{50}$Sc following the $\beta$-decay of $^{50}$Ca. Branching ratios were determined from the measured $\gamma$-ray intensities, and angular…