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Inelastic neutron scattering experiments combining time-of-flight and polarized techniques yield a comprehensive picture of the magnon dispersion in multiferroic TbMnO3 including the dynamic chirality. Taking into account only Mn3+ moments,…

强关联电子 · 物理学 2024-02-27 S. Holbein , P. Steffens , S. Biesenkamp , J. Ollivier , A. C. Komarek , M. Baum , M. Braden

The ferroelectric phase of the multiferroic hexagonal manganites (h-ReMnO3) has been reported to undergo a series of magnetic transitions involving long-range ordering/reorientation of 4fRe3+ and/or 3dMn3+ spins below room temperature.…

We fabricated epitaxial thin films of hexagonal DyMnO3, which otherwise form in a bulk perovskite structure, via deposition on Pt(111)//Al2O3 (0001) and YSZ(111) substrates: each of which has in-plane hexagonal symmetry. The polarization…

材料科学 · 物理学 2015-06-25 J. -H. Lee , P. Murugavel , D. Lee , T. W. Noh , Y. Jo , M. -H. Jung , K. H. Jang , J. -G. Park

DyFeO3 exhibits a weak ferromagnetism (TNFe ~ 645 K) that disappears below a spin-reorientation (Morin) transition at TSRFe ~ 50 K. It is also known that applied magnetic field induces ferroelectricity at the magnetic ordering temperature…

材料科学 · 物理学 2013-01-16 B. Rajeswaran , D. Sanyal , Mahuya Chakrabarti , Y. Sundarayya , A. Sundaresan , C. N. R. Rao

The floating-zone method with different growth ambiances has been used to selectively obtain hexagonal or orthorhombic DyMnO$_{3}$ single crystals. The crystals were characterized by X-ray powder diffraction of ground specimen and a…

强关联电子 · 物理学 2009-11-13 S Harikrishnan , S Roessler , C M Naveen Kumar , H L Bhat , U K Roessler , S Wirth , F Steglich , Suja Elizabeth

Magnetoelectric multiferroics are highly sought after for applications in low-power electronics and for advancing fundamental research, including axion insulators and dark matter detection. However, achieving a combination of ferroic spin…

材料科学 · 物理学 2024-12-02 Libor Šmejkal

We have found a remarkable increase (up to 60 %) of the dielectric constant with the onset of magnetic order at 42 K in the metastable orthorhombic structures of YMnO3 and HoMnO3 that proves the existence of a strong magneto-dielectric…

强关联电子 · 物理学 2009-11-10 B. Lorenz , Y. Q. Wang , Y. Y. Sun , C. W. Chu

Neutron diffraction, magnetic susceptibility, specific heat, and dielectric constant measurements of single crystal Co3TeO6 have been measured to study the interplay between the ferroelectricity and magnetic order. Long range incommensurate…

Eu1-xYxMnO3 exhibits, unlike other magnetoelectric systems, very distinctive features. Its magnetoelectric properties is driven by the magnetic spin of the Mn3+ ion, but they can be drastically changed by varying the content of Y3+, which…

We report Electron Paramagnetic Resonance measurements on single crystalline and powder samples of Nd_0.5Ca_0.5MnO_3 across the charge-ordering transition at T_co=240 K down to the antiferromagnetic ordering transition at T_N = 140 K. The…

强关联电子 · 物理学 2021-05-26 Janhavi P. Joshi , Rajeev Gupta , A. K. Sood , S. V. Bhat , A. R. Raju , C. N. R. Rao

Improper ferroelectrics are described by two order parameters: a primary one, driving a transition to long-range distortive, magnetic or otherwise non-electric order, and the electric polarization, which is induced by the primary order…

We propose a microscopic theory for magnetic switching of electric polarization (P) in the spin-spiral multiferroics by taking TbMnO3 and DyMnO3 as examples. We reproduce their phase diagrams under a magnetic field H_ex by Monte-Carlo…

强关联电子 · 物理学 2010-10-29 Masahito Mochizuki , Nobuo Furukawa

The present study reports on the structural and magnetic phase transitions in Pr-doped polycrystalline Tb0.6Pr0.4MnO3, using high-resolution neutron powder diffraction (NPD) collected at SINQ spallation source (PSI), to emphasize the…

材料科学 · 物理学 2021-07-07 Harshit Agarwal , Jose A Alonso , Ángel Muñoz , R J Choudhary , O N Srivastava , M A Shaz

Hexagonal HoMnO$_{3}$ is a frustrated antiferromagnet (T$_{N}$=72 K) ferroelectric (T$_{C}$=875 K) in which these two order parameters are coupled. Our neutron measurements of the spin wave dispersion for the S=2 Mn$^{3+}$ on the layered…

强关联电子 · 物理学 2009-11-11 O. P. Vajk , M. Kenzelmann , J. W. Lynn , S. B. Kim , S. -W. Cheong

The precise crystal symmetry and hence the emergence of the electric polarization still remains an open question in the multiferroic materials $R$Mn$_2$O$_5$ ($R$ = rare-earth, Bi, Y). While previous diffraction studies have indicated that…

We investigate the crystal structure in multiferroic tetragonal perovskite Sr$_{1/2}$Ba$_{1/2}$MnO$_3$ with high accuracy of the order of 10$^{-3}$ Angstrom for an atomic displacement. The large atomic displacement for Mn ion from the…

材料科学 · 物理学 2020-07-15 D. Okuyama , K. Yamauchi , H. Sakai , Y. Taguchi , Y. Tokura , K. Sugimoto , T. J. Sato , T. Oguchi

The coupling between localized spins and phonons can lead to shifts in the dielectric constant of insulating materials at magnetic ordering transitions. Studies on isostructural SeCuO3 (ferromagnetic) and TeCuO3 (antiferromagnetic)…

材料科学 · 物理学 2009-04-14 G. Lawes , T. Kimura , C. M. Varma , M. A. Subramanian , R. J. Cava , A. P. Ramirez

Structural, magnetic and multiferroic properties of single crystals of Dy$_{1-x}$Ho$_x$MnO$_3$ ($x = 0, 0.2$) were investigated by the different methods of polarized and classical neutron diffraction and macroscopic methods in order to…

Magnetic and dielectric properties of the hexagonal triangular lattice antiferromagnet 2H-AgFeO2 have been studied by neutron diffraction, magnetic susceptibility, specific heat, pyroelectric current, and dielectric constant measurements.…

强关联电子 · 物理学 2019-03-05 Noriki Terada , Dmitry D. Khalyavin , Pascal Manuel , Yoshihiro Tsujimoto , Alexei A. Belik

The ferroelectric order and magnetic field induced effects observed in the spiral phase of MnWO4 are described theoretically. It is demonstrated explicitly that the Dzyaloshinskii-Moriya antisymmetric interactions contribute to the…

强关联电子 · 物理学 2010-01-25 P. Toledano , B. Mettout , W. Schranz , G. Krexner