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We report on the observation of Kondo and split Kondo peaks in single-molecule transistors containing a single spin transition molecule with a Fe2+ ion. Coulomb blockade characteristics reveal a double quantum dot behavior in a parallel…

介观与纳米尺度物理 · 物理学 2010-04-27 A. Bernand-Mantel , J. S. Seldenthuis , A. Beukman , H. S. J. van der Zant , V. Meded , R. Chandrasekhar , K. Fink , M. Ruben , F. Evers

Quantum engineering requires controllable artificial systems with quantum coherence exceeding the device size and operation time. This can be achieved with geometrically confined low-dimensional electronic structures embedded within…

Coherent interactions between spins in quantum dots are a key requirement for quantum gates. We have performed pump-probe experiments in which pulsed lasers emitting at different photon energies manipulate two distinct subsets of electron…

介观与纳米尺度物理 · 物理学 2011-10-03 S. Spatzek , A. Greilich , Sophia E. Economou , A. Schwan , S. Varwig , D. R. Yakovlev , D. Reuter , A. D. Wieck , T. L. Reinecke , M. Bayer

Spin qubits defined in carbon nanotube quantum dots are of considerable interest for encoding and manipulating quantum information because of the long electron spin coherence times expected. However, before carbon nanotubes can find…

介观与纳米尺度物理 · 物理学 2010-04-27 S. J. Chorley , G. Giavaras , J. Wabnig , G. A. C. Jones , C. G. Smith , G. A. D. Briggs , M. R. Buitelaar

We discuss advantages and limitations of the spin noise spectroscopy for characterization of interacting quantum dot systems on specific examples of individual singly and doubly charged quantum dot molecules (QDMs). It is shown that all the…

介观与纳米尺度物理 · 物理学 2013-07-29 Dibyendu Roy , Yan Li , Alex Greilich , Yuriy V. Pershin , Avadh Saxena , Nikolai A. Sinitsyn

Among the possible types of magnetic dipole interactions in molecular systems, couplings between nuclear motion and the nuclear spin have probably received the least attention in molecular spectroscopy. Although very small in comparison to…

化学物理 · 物理学 2026-04-22 Matthias Diez , Johannes K. Krondorfer , Albert Hirtenfelder , Andreas W. Hauser

We observe the low-lying excitations of a molecular dimer formed by two electrons in a GaAs semiconductor quantum dot in which the number of confined electrons is tuned by optical illumination. By employing inelastic light scattering we…

介观与纳米尺度物理 · 物理学 2010-06-16 Achintya Singha , Vittorio Pellegrini , Aron Pinczuk , Loren N. Pfeiffer , Ken W. West , Massimo Rontani

Molecular systems can exhibit a complex, chemically tailorable inner structure which allows for targeting of specific mechanical, electronic and optical properties. At the single-molecule level, two major complementary ways to explore these…

介观与纳米尺度物理 · 物理学 2017-04-05 Rocco Gaudenzi , Maciej Misiorny , Enrique Burzurí , Maarten R. Wegewijs , Herre S. J. van der Zant

We have investigated the dynamics of the electron-nuclei coupled system in quantum dots. The bunching of results of the electron spin measurements and the revival in the conditional probabilities are salient features of the nuclear spin…

介观与纳米尺度物理 · 物理学 2009-11-11 Ozgur Cakir , Toshihide Takagahara

Solid-state spins are promising as interfaces from stationary qubits to single photons for quantum communication technologies. Semiconductor quantum dots have excellent optical coherence, exhibit near unity collection efficiencies when…

We have investigated few-body states in vertically stacked quantum dots. Due to small inter-dot tunneling rate, the coupling in our system is in a previously unexplored regime where electron-hole exchange is the dominant spin interaction.…

介观与纳米尺度物理 · 物理学 2009-11-13 Stefan Falt , Mete Atature , Hakan E. Tureci , Yong Zhao , Antonio Badolato , Atac Imamoglu

A double-quantum-dot coupled to electrodes with spin-dependent splitting of chemical potentials (spin bias) is investigated theoretically by means of the Green's functions formalism. By applying a large spin bias, the quantum spin in a…

介观与纳米尺度物理 · 物理学 2008-06-16 Hai-Zhou Lu , Shun-Qing Shen

Tunnel-coupled pairs of optically active quantum dots - quantum dot molecules (QDMs) - offer the possibility to combine excellent optical properties such as strong light-matter coupling with two-spin singlet-triplet ($S-T_0$) qubits having…

Spins in semiconductor quantum dots constitute a promising platform for scalable quantum information processing. Coupling them strongly to the photonic modes of superconducting microwave resonators would enable fast non-demolition readout…

The electron spin is a natural two level system that allows a qubit to be encoded. When localized in a gate defined quantum dot, the electron spin provides a promising platform for a future functional quantum computer. The essential…

介观与纳米尺度物理 · 物理学 2013-02-04 Luka Trifunovic , Oliver Dial , Mircea Trif , James R. Wootton , Rediet Abebe , Amir Yacoby , Daniel Loss

The ground states of artificial molecules made of two vertically coupled quantum rings are studied within the spin density functional theory for systems containing up to 13 electrons. Quantum tunneling effects on the electronic structure of…

其他凝聚态物理 · 物理学 2007-05-23 L. K. Castelano , G. -Q. Hai , B. Partoens , F. M. Peeters

Spin-orbit coupling in solids describes an interaction between an electron's spin, an internal quantum-mechanical degree of freedom, with its linear momentum, an external property. Spin-orbit interaction, due to its relativistic nature, is…

介观与纳米尺度物理 · 物理学 2014-08-07 J. Shabani , Younghyun Kim , A. P. McFadden , R. M. Lutchyn , C. Nayak , C. J. palmstrøm

We measure transport at finite bias through a double quantum dot formed by top-gates in an InAs nanowire. Pauli spin-bockade is confirmed with several electrons in the dot. This is expected due to the small exchange interactions in InAs and…

介观与纳米尺度物理 · 物理学 2009-11-13 A. Pfund , I. Shorubalko , R. Leturcq , K. Ensslin

In mesoscopic systems with spin-orbit coupling, spin-injection into quantum dots at zero magnetic field is expected under a wide range of conditions. However, up to now, a viable approach for experimentally identifying such injection has…

介观与纳米尺度物理 · 物理学 2013-05-29 Mark S. Rudner , Emmanuel I. Rashba

The creation, coherent manipulation, and measurement of spins in nanostructures open up completely new possibilities for electronics and information processing, among them quantum computing and quantum communication. We review our…

介观与纳米尺度物理 · 物理学 2007-05-23 P. Recher , D. Loss , J. Levy