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Comprehensive inelastic neutron-scattering measurements were performed to study the soft optical phonons in La2-xSrxCuO4 at x=0.10, 0.12 and 0.18. We found at x=0.18 that the softening of Z-point phonon, suggesting incipient structural…

超导电性 · 物理学 2009-10-31 H. Kimura , K. Hirota , C. H. Lee , K. Yamada , G. Shirane

We have carried out temperature and pressure-dependent Raman and x-ray measurements on single crystals of Tb$_2$Ti$_2$O$_7$. We attribute the observed anomalous temperature dependence of phonons to phonon-phonon anharmonic interactions. The…

Materials which possess coupling between different degrees of freedom such as charge, spin, orbital and lattice are of tremendous interest due to their potential for device applications. It has been recently realized that some of manganite…

材料科学 · 物理学 2021-10-27 Bommareddy Poojitha , Surajit Saha

Magnetic spinels (with chemical formula $AX_{2}$O$_{4}$, with $X$ a 3$d$ transition metal ion) that also have an orbital degeneracy are Jahn-Teller active and hence possess a coupling between spin and lattice degrees of freedom. At high…

强关联电子 · 物理学 2017-11-13 T. Weber , B. Roessli , C. Stock , T. Keller , K. Schmalzl , F. Bourdarot , R. Georgii , R. A. Ewings , R. S. Perry , P. Böni

A new effect originating from the crystal-field-excitation - phonon coupling was observed (in the far infrared spectra of a multiferroic PrFe3(BO3)4). The reststrahlen band corresponding to the A2 symmetry nondegenerate phonon mode near 50…

材料科学 · 物理学 2014-11-05 K. N. Boldyrev , T. N. Stanislavchuk , A. A. Sirenko , L. N. Bezmaternykh , M. N. Popova

We performed a finite-temperature quantum Monte Carlo simulation of the one-dimensional spin-1/2 Heisenberg model with nearest-neighbor interaction coupled to Einstein phonons. Our method allows to treat easily up to 100 phonons per site…

凝聚态物理 · 物理学 2007-05-23 Rainer W. Kühne , Ute Löw

Layered antiferromagnetic materials have emerged as a novel subset of the two-dimensional family providing a highly accessible regime with prospects for layer-number-dependent magnetism. Furthermore, transition metal phosphorous…

We report inelastic neutron scattering studies of magnetic excitations in antiferromagnetically ordered SrFe$_{2}$As$_{2}$ ($T_{N}=220$ K), the parent compound of the FeAs-based superconductors. At low temperatures (T=7 K), the spectrum of…

The perovskite TbFe$_{0.5}$Cr$_{0.5}$O$_3$ shows two anomalies in the magnetic susceptibility at $T_N$ = 257K and $T_{SR}$ = 190K which are respectively, the antiferromagnetic and spin reorientation transition that occur in the Fe/Cr…

The canting angles and fluctuation of the magnetic ion spins of spinel oxide MnCr${}_2$O${}_4$ were studied by nuclear magnetic resonance (NMR) at low temperatures, which has a collinear ferrimagnetic order below $T_C$ and a ferrimagnetic…

强关联电子 · 物理学 2015-05-19 Dong Young Yoon , Soonchil Lee , Yoon Seok Oh , Kee Hoon Kim

The enhancement of spin-phonon coupling in gadolinium filled double walled carbon nanotubes (GdCl3@DWNTs) is demonstrated through temperature dependent magnetrometry and polarized Raman Spectroscopy (PRS). Temperature dependent…

介观与纳米尺度物理 · 物理学 2019-06-05 S. Ncube , R. Erasmus , S. Bhattacharyya

In this paper, we present the spin-phonon coupling and dielectric response of nano-crystalline Pr$_2$CoMnO$_6$ employing Raman and dielectric spectroscopic study. Pr$_2$CoMnO$_6$ is a manganite compound , it undergoes a paramagnetic to…

强关联电子 · 物理学 2021-04-13 Ilyas Noor Bhatti , Imtiaz Noor Bhatti

We investigated the magnetic and magnetoelastic properties of MnSc$_2$Se$_4$ single crystals at low temperature under a magnetic field directed along the crystallographic [111] axis. The magnetization data at low temperature show a linear…

强关联电子 · 物理学 2024-10-29 J. Sourd , Y. Skourski , L. Prodan , V. Tsurkan , A. Miyata , J. Wosnitza , S. Zherlitsyn

Although the rutile structure of TiO$_2$ is stable at high temperatures, the conventional quasiharmonic approximation predicts that several acoustic phonons decrease anomalously to zero frequency with thermal expansion, incorrectly…

材料科学 · 物理学 2015-08-19 Tian Lan , C. W. Li , O. Hellman , D. Kim , J. A. Muñoz , H. Smith , D. L. Abernathy , B. Fultz

The symmetric splitting of two spin-wave branches in an antiferromagnetic resonance (AFR) experiment has been an essential measurement of antiferromagnets for over half a century. In this work, circularly polarized time-domain THz…

强关联电子 · 物理学 2017-12-05 N. J. Laurita , Yi Luo , Rongwei Hu , Meixia Wu , S. W. Cheong , O. Tchernyshyov , N. P. Armitage

The ternary iron arsenide BaFe2As2 with the tetragonal ThCr2Si2-type structure exhibits a spin density wave (SDW) anomaly at 140 K, very similar to LaFeAsO, the parent compound of the iron arsenide superconductors. BaFe2As2 is a poor…

Raman study on a select few orthochromites, RCrO$_3$ (R = Y, Lu, Gd, Eu and Sm) shows that the phonon behavior at TN in compounds with magnetic R-ion (Gd and Sm) is remarkably different from that of non-magnetic R-ion (Y, Lu and Eu). While…

材料科学 · 物理学 2013-06-11 Venkata Srinu Bhadram , B. Rajeswaran , A. Sundaresan , Chandrabhas Narayana

The spin dynamics in the geometrically frustrated pyrochlore antiferromagnet $\rm Gd_2Sn_2O_7$ is studied by means of the electron spin resonance. In the ordered phase ($T_N = 1$ K), we have detected three gapped resonance modes. Their…

强关联电子 · 物理学 2013-05-29 S. S. Sosin , L. A. Prozorova , P. Bonville , M. E. Zhitomirsky

Single crystals of quasi-2D chromium telluride system represented by Cr1+xTe2 (x = 0.22), which crystallizes in the trigonal structure with the c-axis as the growth direction, are synthesized by the flux method. The magnetization…

We report inelastic light scattering experiments on CaFe_2As_2 in the temperature range of 4 to 290 K. In in-plane polarizations two Raman-active phonon modes are observed at 189 and 211 cm-1, displaying A_1g and B_1g symmetries,…

超导电性 · 物理学 2009-11-13 K. -Y. Choi , D. Wulferding , P. Lemmens , N. Ni , S. L. Bud'ko , P. C. Canfield