相关论文: Zero Point Entropy in Stuffed Spin Ice
Spin ice materials are the model systems that have a zero-point entropy as \textit{T} $\rightarrow$ 0 K, owing to the frozen disordered states. Here, we chemically alter the well-known spin ice Ho$_{2}$Ti$_{2}$O$_{7}$ by replacing Ti sites…
Water ice and spin ice are important model systems in which theory can directly account for zero point entropy associated with quenched configurational disorder. Spin ice differs from water ice in the important respect that its fundamental…
Geometric frustration usually arises in systems that comprise magnetic moments (spins) which reside on the sites of a lattice made up of elementary triangular or tetrahedral units and which interact via antiferromagnetic nearest-neighbor…
We report the specific heat and entropy of single crystals of the spin ice compound Dy2Ti2O7 at temperatures down to 0.35 K. We apply magnetic fields along the four characteristic directions: [100], [110], [111] and [112]. Because of Ising…
Thermodynamics studies of a prototypical quasi-two-dimensional frustrated magnet Ba$_2$Sn$_2$ZnCr$_{7p}$Ga$_{10-7p}$O$_{22}$ where the magnetic Cr$^{3+}$ ions are arranged in a triangular network of bipyramids show that the magnetic…
We have studied the thermodynamics of the stuffed spin ice material, Dy2(DyxTi2-x)O7-x/2, in which additional Dy3+ replace Ti4+ in the pyrochlore Dy2Ti2O7. Heat capacity measurements indicate that these materials lose the spin ice zero…
We report the low-temperature magnetothermal properties and spin dynamics of a mixed pyrochlore, Dy2GaSbO7 through the coordination of measurements of dc magnetization, ac susceptibility, and heat capacity, and CF computation. In Dy2GaSbO7,…
Complex disordered states - from liquids and glasses to exotic quantum matter - are ubiquitous in nature. Their key properties include finite entropy, power-law correlations and emergent organising principles. In spin ice, spin correlations…
The low temperature entropy of the the spin ice compounds, such as Ho$_2$Ti$_2$O$_7$ and Dy$_2$Ti$_2$O$_7$, is well described by the nearest-neighbor antiferromagnetic Ising model on the pyrochlore lattice, i.e.\ by the ``ice rules''. This…
The residual entropy of spin ice and other frustrated magnets is a property of considerable interest, yet the usual way of determining it, by integrating the heat capacity, is generally ambiguous. Here we note that a straightforward…
Identifying extensively degenerate zero-temperature states is key in characterizing spin-liquid-candidate materials and spin ices. In experiments, finding zero-point entropy (ZPE) is often attempted by measuring the entropy released by a…
The recent discovery of Spin-ice is a spectacular example of non-coplanar spin arrangements that can arise in the pyrochlore A2B2O7 structure. We present magnetic and thermodynamic studies on the metallic-ferromagnet pyrochlore Sm2Mo2O7.…
"Spin Ice" is an exotic type of frustrated magnet realized in "pyrochlore" materials Ho_{2}Ti_{2}O_{7}, Dy_{2}Ti_{2}O_{7}, Ho_{2}Sn_{2}O_{7}, etc., in which magnetic atoms (spins) reside on a sublattice made of the vertices of…
A novel macroscopically degenerate state called kagome ice, which was recently found in a spin ice compound Dy2Ti2O7 in a magnetic field applied along the [111] direction of the cubic unit cell, is studied by specific heat measurements. The…
Artificial spin ices have transcended their origins in frustrated rare-earth pyrochlores to become a versatile platform for engineering exotic states of matter. Across diverse implementations, from nanomagnets and superconducting vortices…
Neutron scattering, a.c. magnetic susceptibility and specific heat studies have been carried out on polycrystalline Dy2Zr2O7. Unlike the pyrochlore spin ice Dy2Ti2O7, Dy2Zr2O7 crystallizes into the fluorite structure and the magnetic Dy3+…
Geometrical frustration is a central challenge in contemporary condensed matter physics, a crucible favourable to the emergence of novel physics. The pyrochlore magnets, with rare earth magnetic moments localized at the vertices of…
Spin ice systems represent a prime example of constrained spin systems and exhibit rich low-energy physics. In this study, we explore how introducing a tunable anisotropic spin coupling to the conventional Ising spin ice Hamiltonian on the…
Competitive effects of so-called three-site four-spin interactions, single ion anisotropy and bilinear interactions is studied in the mixed spin-1/2 and spin-1 Ising model on a decorated square lattice. Exploring the decoration-iteration…
Geometrically frustrated clusters of Ising spins of different shapes on a triangular lattice are studied by exact enumeration and Monte Carlo simulation. The focus is laid on the ground-state energy and residual entropy behaviors as…