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By combining neutron four-circle diffraction and polarized neutron diffraction techniques we have determined the complex spin structures of a multiferroic, YMn2O5, that exhibits two ferroelectric phases at low temperatures. The obtained…

We have determined the magnetic structure of the low-temperature incommensurate phase of multiferroic YMn2O5 using single-crystal neutron diffraction. By employing corepresentation analysis, we have ensured full compliance with both…

材料科学 · 物理学 2009-11-13 P. G. Radaelli , C. Vecchini , L. C. Chapon , P. J. Brown , S. Park , S-W. Cheong

The structural, electronic and lattice dielectric properties of multiferroic TbMn$_2$O$_5$ are investigated using density functional theory within the generalized gradient approximation (GGA). We use collinear spin approximations and ignore…

材料科学 · 物理学 2009-11-13 Chenjie Wang , Guang-Can Guo , Lixin He

We uncover a new pathway towards multiferroicity, showing how magnetism can drive ferroelectricity without relying on inversion symmetry breaking of the magnetic ordering. Our free-energy analysis demonstrates that any commensurate…

材料科学 · 物理学 2009-11-11 Joseph J. Betouras , Gianluca Giovannetti , Jeroen van den Brink

We report the observation of a magnetic polarization of the O\,$2p$-states in YMn$_2$O$_5$ through the use of soft X-ray resonant scattering at the oxygen $K$-edge. Remarkably, we find that the temperature dependence of the integrated…

强关联电子 · 物理学 2015-03-19 S. Partzsch , S. B. Wilkins , J. P. Hill , E. Schierle , E. Weschke , D. Souptel , B. Büchner , J. Geck

The low-temperature ferroelectric polarization of multiferroic $YMn_2O_5$ is completely reversed at a critical pressure of 10 kbar and the phase transition from the incommensurate to the commensurate magnetic phase is induced by pressures…

It was recently observed that materials showing most striking multiferroic phenomena are frustrated spin-density-wave magnets. We present a simple phenomenological theory, which describes the orientation of the induced electric polarization…

强关联电子 · 物理学 2009-11-11 Maxim Mostovoy

Ferroelectricity has been found to occur in several insulating systems, such as TbMnO$_3$ (TMO) and Ni$_3$V$_2$O$_8$ (NVO) which have more than one phase with incommensurately modulated long-range magnetic order. Here we give a…

材料科学 · 物理学 2009-11-11 A. Brooks Harris

We review the phenomenology of coupled magnetic and electric order parameters for systems in which ferroelectric and incommensurate magnetic order occur simultaneously. We discuss the role that such materials might play in fabricating novel…

材料科学 · 物理学 2007-05-23 A. B. Harris , G. Lawes

We have carried out a first-principles theoretical study of the magnetically induced polarization in orthorhombic TbMnO3, a prototypical material in which a cycloidal spin structure generates an electric polarization via the spin-orbit…

材料科学 · 物理学 2009-12-16 Andrei Malashevich , David Vanderbilt

Magnetic and ferroelectric properties of layered geometrically frustrated cluster compound FeTe$_2$O$_5$Br were investigated with single-crystal neutron diffraction and dielectric measurements. Incommensurate amplitude modulated magnetic…

材料科学 · 物理学 2009-10-01 M. Pregelj , O. Zaharko , A. Zorko , Z. Kutnjak , P. Jeglic , P. J. Brown , M. Jagodic , Z. Jaglicic , H. Berger , D. Arcon

The ground state structural, electronic and magnetic properties of multiferroic TbMn$_2$O$_5$ are investigated via first-principles calculations. We show that the ferroelectricity in TbMn$_2$O$_5$ is driven by the non-centrosymmetric…

材料科学 · 物理学 2009-11-13 Chenjie Wang , Guang-Can Guo , Lixin He

The phenomenological theory of ferroelectricity in spiral magnets presented in [M. Mostovoy, Phys. Rev. Lett. 96, 067601 (2006)] is generalized to describe consistently states with both uniform and modulated-in-space ferroelectric…

材料科学 · 物理学 2009-11-13 A. Cano , E. I. Kats

In multiferroic TbMn$_2$O$_5$, the behavior of the terbium ions forms a crucial part of the magneto-electric coupling. The result is a magnetically induced reversal of the electric polarization at 2 T. In this article we present the first…

强关联电子 · 物理学 2011-06-27 R. D. Johnson , C. Mazzoli , S. R. Bland , C-H. Du , P. D. Hatton

We report a systematic study of the structure, electric and magnetic properties of Ca$_3$Co$_{2-x}$Mn$_x$O$_6$ single crystals with $x =$ 0.72 and 0.26. The DC and AC magnetic susceptibilities display anomalies with characteristic of the…

材料科学 · 物理学 2017-09-08 J. Shi , J. D. Song , J. C. Wu , X. Rao , H. L. Che , Z. Y. Zhao , H. D. Zhou , J. Ma , R. R. Zhang , L. Zhang , X. G. Liu , X. Zhao , X. F. Sun

Density-functional calculations are carried out to investigate incommensurate magnetic structures and ferroelectric polarization in newly discovered multiferroic material MnI$_2$. The exchange interactions among local moments on Mn are…

强关联电子 · 物理学 2013-05-30 Xianxin Wu , Yingxiang Cai , Qing Xie , Hongming Weng , Heng Fan , Jiangping Hu

Observation of ferroelectricity among non-d0 systems, which was believed for a long time an unrealistic concept, led to various proposals for the mechanisms to explain the same (i.e. magnetically induced ferroelectricity) during last…

We report the direct measurement of antiferromagnetic spin polarization at the oxygen sites in the multiferroic TbMn2O5, through resonant soft x-ray magnetic scattering. This supports recent theoretical models suggesting that the oxygen…

Using first principle calculations under the framework of density functional theory we have investigated the electronic structure, magnetism and ferroelectric polarization in the triangular lattice antiferromagnet AgFeO2, and its comparison…

材料科学 · 物理学 2018-01-03 Jayita Chakraborty , Indra Dasgupta

Neutron diffraction measurements under high magnetic fields have been performed for the multiferroic compound HoMn$_{2}$O$_{5}$. At zero field, high-temperature incommensurate magnetic (HT-ICM) -- commensurate magnetic (CM) --…

强关联电子 · 物理学 2007-05-23 H. Kimura , Y. Kamada , Y. Noda , K. Kaneko , N. Metoki , K. Kohn
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