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相关论文: Fluorescence intermittency in blinking quantum dot…

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Analysis of stochastic processes can be used to engender critical thinking. Quantum dots have a reversible, stochastic transition between luminescent and non-luminescent states. The luminescence intermittency is known as blinking, and is…

物理教育 · 物理学 2020-01-16 Laszlo Frazer , Heather F. Higginbotham , Toby D. M. Bell , Alison M. Funston

In this letter we examine a model recently proposed to produce phase synchronization [K. Wood et al, Phys. Rev. Lett. 96, 145701 (2006)] and we show that the onset to synchronization corresponds to the emergence of an intermittent process…

统计力学 · 物理学 2007-05-23 Simone Bianco , Elvis Geneston , Paolo Grigolini , Massimiliano Ignaccolo

The photoluminescence intermittency (blinking) of quantum dots is interesting because it is an easily-measured quantum process whose transition statistics cannot be explained by Fermi's Golden Rule. Commonly, the transition statistics are…

介观与纳米尺度物理 · 物理学 2023-01-23 Roberto N. Munoz , Laszlo Frazer , Gangcheng Yuan , Paul Mulvaney , Felix A. Pollock , Kavan Modi

We study the intermittent fluorescence of a single molecule, jumping from the "light on" to the "light off" state, as a Poisson process modulated by a fluctuating environment. We show that the quasi-periodic and quasi-deterministic…

软凝聚态物质 · 物理学 2009-11-11 Simone Bianco , Paolo Grigolini , Paolo Paradisi

We present a new physical model resolving a long-standing mystery of the power-law distributions of the blinking times in single colloidal quantum dot fluorescence. The model considers the non-radiative relaxation of the exciton through…

统计力学 · 物理学 2009-11-16 Pavel A. Frantsuzov , Sandor Volkan-Kacso , Bolizsar Janko

Single photon emitters are core building blocks of quantum technologies, with established and emerging applications ranging from quantum computing and communication to metrology and sensing. Regardless of their nature, quantum emitters…

量子物理 · 物理学 2023-08-28 G. Landry , C. Bradac

Fluctuations in the fluorescence from macroscopic ensembles of colloidal semiconductor quantum dots have the spectral form of 1/f noise. The measured power spectral density reflects the fluorescence intermittency of individual dots with…

材料科学 · 物理学 2009-11-10 Matthew Pelton , David Grier , Philippe Guyot-Sionnest

We consider two different proposals to generate a time series with the same non-Poisson distribution of waiting times, to which we refer to as renewal and modulation. We show that, in spite of the apparent statistical equivalence, the two…

统计力学 · 物理学 2009-11-11 Paolo Allegrini , Francesco Barbi , Paolo Grigolini , Paolo Paradisi

We present a study of residence time statistics for $N$ blinking quantum dots. With numerical simulations and exact calculations we show sharp transitions for a critical number of dots. In contrast to expectation the fluctuations in the…

统计力学 · 物理学 2013-05-29 S. Burov , E. Barkai

A simple model explaining the experimental data on QDs luminescence blinking is suggested. The model does not assume the presence of the long-lived electron traps. The bleaching of the QD luminescence is a result of the Auger assisted…

介观与纳米尺度物理 · 物理学 2009-11-11 Pavel A. Frantsuzov , R. A. Marcus

We study the processes in a quantum dot and its surrounds under resonant excitation with the addition of weak non-resonant light. We observe a decrease in inhomogeneous emission linewidth, as well as previously observed enhancement of…

量子物理 · 物理学 2017-02-15 O. Gazzano , T. Huber , V. Loo , S. Polyakov , E. B. Flagg , G. S. Solomon

Single quantum light-emitters are valuable resources for engineered quantum systems. They can function as robust single-photon generators, allow optical control of single spins, provide readout capabilities for atomic-scale sensors, and…

量子物理 · 物理学 2019-09-04 Jemy Geordy , Lachlan J. Rogers , Cameron M Rogers , Thomas Volz , Alexei Gilchrist

The observed intermittent light emission from colloidal semiconductor nanocrystals has long been associated with Auger recombination assisted quenching. We test this view by observing transient emission dynamics of CdSe/CdS/ZnS…

介观与纳米尺度物理 · 物理学 2010-02-23 Shamir Rosen , Osip Schwartz , Dan Oron

We analyze intermittency in intensity and fluorescence lifetime of CsPbBr$_3$ perovskite quantum dots by applying unbiased Bayesian inference analysis methods. We apply changepoint analysis (CPA) and a Bayesian state clustering algorithm to…

介观与纳米尺度物理 · 物理学 2021-05-06 Isabelle M. Palstra , Ilse Maillette de Buy Wenniger , Biplab K. Patra , Erik C. Garnett , A. Femius Koenderink

We study theoretically the time-resolved four-wave mixing (FWM) response of an ensemble of pairs of quantum dots undergoing radiative recombination. At short (picosecond) delay times, the response signal shows beats that may be dominated by…

介观与纳米尺度物理 · 物理学 2009-10-04 Anna Sitek , Pawel Machnikowski

The paper describes the means to reveal and characterize slow periodic modulation of qubit frequency. Such modulation can come from different sources and can impact qubit stability. We show that the modulation leads to very sharp peaks in…

量子物理 · 物理学 2024-08-16 Filip Wudarski , Yaxing Zhang , Juan Atalaya , M. I. Dykman

We studied time-dependent features of high-frequency fluorescent radiation from a two-level quantum system with broken inversion spatial symmetry. The system in question was modelled after a one-electron two-level asymmetric polar…

量子物理 · 物理学 2024-12-17 Andrey V. Soldatov

It has been observed experimentally [H.R. Xia, C.Y. Ye, and S.Y. Zhu, Phys. Rev. Lett. {\bf 77}, 1032 (1996)] that quantum interference between two molecular transitions can lead to a suppression or enhancement of spontaneous emission. This…

量子物理 · 物理学 2009-10-31 Jin Wang , H. M. Wiseman , Z. Ficek

Three models of single colloidal quantum dot emission fluctuations (blinking) based on spectral diffusion were considered analytically and numerically. It was shown that the only one of them, namely the Frantsuzov and Marcus model…

统计力学 · 物理学 2019-07-24 Vladislav K. Busov , Pavel A. Frantsuzov

We use photon correlation measurements to study blinking in single, epitaxially-grown self-assembled InAs quantum dots situated in circular Bragg grating and microdisk cavities. The normalized second-order correlation function g(2)(\tau) is…

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