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The pyrochlore oxides Dy$_{2}$Ti$_{2}$O$_{7}$ and Ho$_{2}$Ti$_{2}$O$_{7}$ are well studied spin ice systems and have shown the evidences of magnetic monopole excitations. Unlike these, Dy$_{2}$Zr$_{2}$O$_{7}$ is reported to crystallize in a…

强关联电子 · 物理学 2020-08-26 Sheetal , Anzar Ali , Sarita Rajput , Yogesh Singh , Tulika Maitra , C. S. Yadav

A spin-ice compound dysprosium titanate, Dy2Ti2O7, is studied by specific heat measurements in magnetic fields applied along the [110] direction of the cubic unit cell. Above a magnetic field of 0.4 T a relatively sharp peak at T = 1.1 K in…

材料科学 · 物理学 2009-11-10 Zenji Hiroi , Kazuyuki Matsuhira , Masao Ogata

The pyrochlore spin ice compounds Dy2Ti2O7 and Ho2Ti2O7 are well described by classical Ising models down to very low temperatures. Given the empirical success of this description, the question of the importance of quantum effects in these…

强关联电子 · 物理学 2015-10-28 Jeffrey G. Rau , Michel J. P. Gingras

We studied the field-induced magnetic structures of the Tb2Ti2O7 pyrochlore by single-crystal neutron diffraction with a magnetic field applied along a [110] axis, focusing on the influence of a small misalignment. Both induced magnetic…

强关联电子 · 物理学 2010-11-10 A. P. Sazonov , A. Gukasov , I. Mirebeau , H. Cao , P. Bonville , B. Grenier , G. Dhalenne

The recent identification of the dysprosium titanate compound $Dy_2 Ti_2 O_7$ as a ``Spin-Ice'', i.e. the spin analog of regular entropic ice of Pauling, has created considerable excitement. The ability to manipulate spins using magnetic…

统计力学 · 物理学 2009-11-07 B. Sriram Shastry

We study the three-dimensional Kasteleyn transition in both nearest neighbours and dipolar spin ice models using an algorithm that conserves the number of excitations. We first limit the interactions range to nearest neighbours to test the…

强关联电子 · 物理学 2017-01-04 M. L. Baez , R. A. Borzi

We have studied the field induced magnetic structures in the spin liquid Tb$_2$Ti$_2$O$_7$, in a wide temperature (0.3$<$$T$$<$270 K) and field (0$<$$H$$<$7 T) range, by single crystal neutron diffraction with $\bf{H}$ // [110] axis. We…

强关联电子 · 物理学 2009-11-13 H. Cao , A. Gukasov , I. Mirebeau , P. Bonville , G. Dhalenne

Magnetization and susceptibility studies on single crystals of the pyrochlore Ho$_{2}$Ti$_{2}$O$_{7}$ are reported for the first time. Magnetization isotherms are shown to be qualitatively similar to that predicted by the nearest neighbor…

无序系统与神经网络 · 物理学 2009-11-07 A. L. Cornelius , J. S. Gardner

Nonequilibrium processes are probed by ultrasound waves in the spin-ice material Dy2Ti2O7 at low temperatures. The sound velocity and the sound attenuation exhibit a number of anomalies versus applied magnetic field for temperatures below…

强关联电子 · 物理学 2011-12-07 S. Erfanifam , S. Zherlitsyn , J. Wosnitza , R. Moessner , O. A. Petrenko , G. Balakrishnan , A. A. Zvyagin

The magnetization (both dc and ac) of pyrochlore Eu2Ti2O7 have been investigated. Ac susceptibility measurements reveal a new unusual spin freezing below 35K for pure Eu2Ti2O7. Frequency dependence of these ac peak positions indicate slow…

材料科学 · 物理学 2018-05-23 Arkadeb Pal , Abhishek Singh , Prajyoti Singh , A. K. Ghosh , Sandip Chatterjee

Recent experiments on the spin-ice material Dy2Ti2O7 suggest that the Pauling "ice entropy", characteristic of its classical Coulombic spin-liquid state, may be lost at low temperatures [D. Pomaranski et al., Nature Phys. 9, 353 (2013)].…

强关联电子 · 物理学 2015-09-16 Paul McClarty , Olga Sikora , Roderich Moessner , Karlo Penc , Frank Pollmann , Nic Shannon

We present numerical studies of dipolar spin ice in the presence of a magnetic field slightly tilted away from the [111] axis. We find a first-order transition from a kagome ice to a $\mathbf{q}=$X state when the external field is tilted…

统计力学 · 物理学 2016-06-08 Wen-Han Kao , Peter Holdsworth , Ying-Jer Kao

We herein present the spin freezing dynamics of stuffed polycrystalline compound Dy$_2$Ti$_{1.8}$Mn$_{0.2}$O$_7$. In Dy$_2$Ti$_2$O$_7$, spin freezes with ice-like spin relaxations at a temperature around 3 K (T$_i$) along with another spin…

材料科学 · 物理学 2022-05-10 Rajnikant Upadhyay , Manjari Shukla , Rachana Sain , Martin Tolkiehn , Chandan Upadhyay

We have studied spin relaxation in the spin ice compound Dy2Ti2O7 through measurements of the a.c. magnetic susceptibility. While the characteristic spin relaxation time is thermally activated at high temperatures, it becomes almost…

材料科学 · 物理学 2009-11-10 J. Snyder , B. G. Ueland , J. S. Slusky , H. Karunadasa , R. J. Cava , Ari Mizel , P. Schiffer

We report measurements performed on a polycrystalline sample of the pyrochlore compound Nd2Sn2O7. It undergoes a second order magnetic phase transition at Tc ~ 0.91 K to a noncoplanar all-in-all-out magnetic structure of the Nd3+ magnetic…

The spin ice system Dy$_{2}$Ti$_{2}$O$_{7}$ exhibits strong frequency-dependent spin-freezing at $\sim$ 16 K temperature. Although it has been a matter of discussion for years, the origin of this unusual spin freezing is still unknown. The…

强关联电子 · 物理学 2022-04-06 Sheetal , C. S. Yadav

In the ground state of Ho2Ti2O7 spin ice, the disorder of the magnetic moments follows the same rules as the proton disorder in water ice. Excitations take the form of magnetic monopoles that interact via a magnetic Coulomb interaction.…

强关联电子 · 物理学 2013-05-24 L. J. Chang , M. R. Lees , G. Balakrishnan , Y. -J. Kao , A. D. Hillier

Dy$_{2}$Zr$_{2}$O$_{7}$ a disordered pyrochlore system, exhibits the spin ice freezing under the application of magnetic field. Our studies suggest the stabilization of pyrochlore phase in Dy$_{2-x}$La$_{x}$Zr$_{2}$O$_{7}$ with the…

强关联电子 · 物理学 2021-10-12 Sheetal , C. S. Yadav

We have studied the field-induced magnetic structures of Tb2Ti2O7 pyrochlore by single-crystal neutron diffraction under a field applied along the [111] local anisotropy axis, up to H=12T and down to T=40mK. We collected a hundred magnetic…

强关联电子 · 物理学 2013-07-03 A. P. Sazonov , A. Gukasov , H. B. Cao , P. Bonville , E. Ressouche , C. Decorse , I. Mirebeau

Iron (II) complexes with substituted tris(pyrazolyl) ligands, which exhibit a thermally driven transition from a low-spin state at low temperatures to a high-spin state at elevated temperatures, have been studied by M\"ossbauer spectroscopy…