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The adsorption of flexible and highly charged polyelectrolytes onto oppositely charged planar surfaces is investigated by means of Monte Carlo simulations. The effect of image forces stemming from the dielectric discontinuity at the…

软凝聚态物质 · 物理学 2016-08-31 Rene Messina

The adsorption of highly \textit{oppositely} charged flexible polyelectrolytes (PEs) on a charged planar substrate is investigated by means of Monte Carlo (MC) simulations. We study in detail the equilibrium structure of the first few PE…

软凝聚态物质 · 物理学 2007-05-23 Rene Messina

The adsorption of highly charged flexible polycations and polyanions on a charged cylindrical substrate is investigated by means of Monte Carlo (MC) simulations. A detailed structural study, including monomer and fluid charge distributions,…

软凝聚态物质 · 物理学 2007-05-23 Rene Messina

The behavior of polyampholytes near a charged planar surface is studied by means of Monte Carlo simulations. The investigated polyampholytes are overall electrically neutral and made up of oppositely charged units (called blocks) that are…

软凝聚态物质 · 物理学 2009-11-11 Rene Messina

The behavior of a polyelectrolyte adsorbed on a charged substrate of high-dielectric constant is studied by both Monte-Carlo simulation and analytical methods. It is found that in a low enough ionic strength medium, the adsorption…

软凝聚态物质 · 物理学 2007-05-23 Chi-Ho Cheng , Pik-Yin Lai

The problem of charged polymer chains (polyelectrolytes) as they adsorb on a planar surface is addressed theoretically. We review the basic mechanisms and theory underlying polyelectrolyte adsorption on a single surface in two situations:…

软凝聚态物质 · 物理学 2012-01-31 David Andelman , Jean-Francois Joanny

The behavior of polyelectrolytes between charged surfaces immersed in semi-dilute solutions is investigated theoretically. A continuum mean field approach is used for calculating numerically concentration profiles between two electrodes…

软凝聚态物质 · 物理学 2007-05-23 I. Borukhov , D. Andelman , H. Orland

The behavior of a polyelectrolyte adsorbed on a charged surface of high-dielectric constant is studied by both Monte-Carlo simulation and analytical methods. It is found that in a low ionic strength medium, the transition is first-order…

软凝聚态物质 · 物理学 2007-05-23 Chi-Ho Cheng , Pik-Yin Lai

We study the effective interaction between differently charged polyelectrolyte-colloid complexes in electrolyte solutions via Monte Carlo simulations. These complexes are formed when short and flexible polyelectrolyte chains adsorb onto…

软凝聚态物质 · 物理学 2010-05-05 D. Truzzolillo , F. Bordi , F. Sciortino , S. Sennato

Using self-assembly techniques, x-ray reflectivity measurements, and computer simulations, we study the effective interaction between charged polymer rods and surfaces. Long-time Brownian dynamics simulations are used to measure the…

软凝聚态物质 · 物理学 2009-10-31 R. Jay Mashl , Niels Grønbech-Jensen , M. R. Fitzsimmons , M. Lütt , DeQuan Li

In the present study, we have investigated, using Monte Carlo simulations (MC), the adsorption of polyelectrolytes on the charged nanopatterned surfaces. Different surface patterns were considered and we noticed that the amount of…

软凝聚态物质 · 物理学 2020-02-04 Amin Bakhshandeh , Maximiliano Segala

This chapter deals with charged polymers (polyelectrolytes) in solution and at surfaces. The behavior of polyelectrolytes is markedly different from that of neutral polymers. In bulk solutions, i.e. disregarding the surface effect, there…

软凝聚态物质 · 物理学 2009-09-25 Roland R. Netz , David Andelman

We propose a detailed description of the structure of the layer formed by polyelectrolyte chains adsorbed onto an oppositely charged surface in the semi-dilute regime. We combine the mean-field Poisson-Boltzmann-Edwards theory and the…

软凝聚态物质 · 物理学 2019-02-20 Manoel Manghi , Miguel Aubouy

We study the effective interaction between a planar array of uniformly negatively charged, stiff rods parallel to a negatively charged planar substrate in the absence of salt in a continuous, isotropic dielectric medium. Using Brownian…

软凝聚态物质 · 物理学 2009-10-31 R. Jay Mashl , Niels Grønbech-Jensen

We studied polyelectrolyte adsorption on a repulsive charged surface by scaling analysis. At low ionic strength and low surface charge density in which a single polyelectrolyte is able to be adsorbed onto the surface, different regimes in…

软凝聚态物质 · 物理学 2016-08-31 Chi-Ho Cheng , Pik-Yin Lai

Monte Carlo simulations were employed to study two negative rods confined between two parallel plates. The system is immersed in a 1-1 restricted primitive model electrolyte. Ion distributions and forces per unit of area (pressures) on rods…

介观与纳米尺度物理 · 物理学 2015-05-20 G. Odriozola , F. Jiménez-Ángeles , M. Lozada-Cassou

We study the attractive interactions between rod-like charged polymers in solution that appear in the presence of multi-valence counterions. The counterions condensed to the rods exhibit both a strong transversal polarization and a…

软凝聚态物质 · 物理学 2009-10-31 Francisco J. Solis , Monica Olvera de la Cruz

The influence of the chain degree of ionization on the adsorption of weak polyelectrolytes on neutral and on oppositely and likely charged surfaces is investigated for the first time, by means of Monte Carlo simulations with the mesoscopic…

生物物理 · 物理学 2012-10-02 F. Alarcón , E. Pérez , A. Gama Goicochea

Structural and thermodynamic properties of the model solution containing charged oligomers and the equivalent number of counterions were studied by means of the canonical Monte Carlo simulation technique. The oligomers are represented as…

软凝聚态物质 · 物理学 2012-02-21 T. Sajevic , J. Rescic , V. Vlachy

The adsorption of highly \textit{oppositely} charged flexible polyelectrolytes onto a charged spherical surface is investigated by means of Monte Carlo simulations in a fashion which resembles the layer-by-layer deposition technique…

软凝聚态物质 · 物理学 2007-05-23 Rene Messina , Christian Holm , Kurt Kremer
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