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Relaxor ferroelectrics are difficult to study and understand. The experiment shows that at low energy scattering there is an acoustic mode, an optic mode, dynamic quasi-elastic scattering and strictly elastic scattering as well as Bragg…

材料科学 · 物理学 2008-08-29 R. A. Cowley , S. N. Gvasaliya , B. Roessli

Single crystals of a ternary relaxor ferroelectric system, 0.29Pb(In1/2Nb1/2)O3-0.45Pb(Mg1/3Nb2/3)O3-0.26PbTiO3, have been studied using triple-axis based elastic and inelastic neutron scattering. Elastic diffuse scattering confirms the…

材料科学 · 物理学 2022-08-10 Qian Li , Sergey Danilkin , Guochu Deng , Jian Wang , Zhengrong Li. Ray L. Withers , Zhuo Xu , Yun Liu

We report neutron inelastic scattering measurements of the lowest-energy transverse optic (TO) phonon branch in the relaxor Pb(Mg_1/3Nb_2/3)O_3 from 400 to 1100 K. Far above the Burns temperature T_d ~ 620 K we observe well-defined…

材料科学 · 物理学 2009-11-07 P. M. Gehring , S. Wakimoto , Z. -G. Ye , G. Shirane

Cold neutron scattering experiments have been performed to explore the energy, temperature, and wave-vector dependence of the diffuse scattering and the transverse acoustic (TA) phonons in the relaxor PbMg(1/3)Nb(2/3)O3. We have observed a…

材料科学 · 物理学 2009-11-10 H. Hiraka , S. -H. Lee , P. M. Gehring , Guangyong Xu , G. Shirane

Neutron scattering techniques have been used to study the relaxor ferroelectric 0.68PbMg1/3Nb2/3O3-0.32PbTiO3 denoted in this paper as 0.68PMN-0.32PT. On cooling, these relaxor ferroelectrics have a long-range ordered ferroelectric phase…

材料科学 · 物理学 2007-05-23 S. N. Gvasaliya , B. Roessli , R. A. Cowley , S. Kojima , S. G. Lushnikov

The low-energy part of vibration spectrum in PbMg$_{1/3}$Nb$_{2/3}$O$_3$ relaxor ferroelectric was studied by inelastic neutron scattering. We observed the coexistence of a resolution-limited central peak with strong quasielastic…

材料科学 · 物理学 2007-05-23 S. N. Gvasaliya , S. G. Lushnikov , B. Roessli

We show that the neutron diffuse scattering in relaxor ferroelectric (1-x)PbZn$_{1/3}$Nb$_{2/3}$O$_{3}$ - x PbTiO$_{3}$ (x=0.07) consists of two components. The first component is strictly elastic but extended in q-space and grows below 600…

材料科学 · 物理学 2019-08-12 G. -M. Rotaru , S. N. Gvasaliya , B. Roessli , S. Kojima , S. G. Lushnikov , P. Günter

We report neutron inelastic scattering experiments on single crystal PbMg$_{1/3}$Nb$_{2/3}$O$_{3}$ doped with 32\% PbTiO$_{3}$, a relaxor ferroelectric that lies close to the morphotropic phase boundary. When cooled under an electric field…

材料科学 · 物理学 2016-01-06 John A. Schneeloch , Zhijun Xu , B. Winn , C. Stock , P. M. Gehring , R. J. Birgeneau , Guangyong Xu

Neutron scattering measurements of the lowest-energy TO phonons in the relaxor Pb(Mg1/3Nb2/3)O3 (PMN) are reported for 10<=T<=750 K. The soft mode, which is overdamped by the polar nanoregions below the Burns temperature T_d = 620 K,…

材料科学 · 物理学 2009-11-07 S. Wakimoto , C. Stock , R. J. Birgeneau , Z. -G. Ye , W. Chen , W. J. L. Buyers , P. M. Gehring , G. Shirane

Inelastic neutron scattering measurements of the relaxor ferroelectric PbMg$_{1 / 3}$Nb$_{2 / 3}$O$_{3}$ (PMN) in the temperature range 490~K$<$T$<$880~K directly observe the soft mode (SM) associated with the Curie-Weiss behavior of the…

材料科学 · 物理学 2009-11-07 S. Vakhrushev , S. Shapiro

The low-energy part of the vibration spectrum in KNbO$_3$ was studied by cold neutron inelastic scattering in the cubic phase. In addition to acoustic phonons, we observe strong diffuse scattering, which consists of two components. The…

材料科学 · 物理学 2007-05-23 S. N. Gvasaliya , B. Roessli , R. A. Cowley , S. G. Lushnikov , A. Choubey , P. Gunter

We report lattice dynamical measurements, made using neutron inelastic scattering methods, of the relaxor perovskite PbMg1/3Nb2/3O3 (PMN) at momentum transfers near the edge of the Brillouin zone. Unusual"columns" of phonon scattering that…

材料科学 · 物理学 2015-05-13 I. P. Swainson , C. Stock , P. M. Gehring , Guangyong Xu , K. Hirota , Y. Qiu , H. Luo , X. Zhao , J. -F. Li , D. Viehland

Resonance Raman scattering, a very effective and sensitive technique for atomically thin semiconducting transition metal dichalcogenide, can be used to observe the phonons from the entire Brillouin zone. In addition to the significance of…

材料科学 · 物理学 2023-02-06 Deepu Kumar , Nasaru Khan , Rahul Kumar , Mahesh Kumar , Pradeep Kumar

We have used neutron scattering techniques to characterize the diffuse scattering and lattice dynamics in single crystals of the relaxor PMN from 10K to 900K. We observed two distinct types of diffuse scattering. The first is weak,…

材料科学 · 物理学 2009-06-11 P. M. Gehring , H. Hiraka , C. Stock , S. -H. Lee , W. Chen , Z. -G. Ye , S. B. Vakhrushev , Z. Chowdhuri

Spin correlations and fluctuations in the 3d-transition-metal-based icosahedral quasicrystal Zn-Fe-Sc have been investigated by neutron scattering using polycrystalline samples. Magnetic diffuse scattering has been observed in the elastic…

We have studied the neutron diffuse scattering in the relaxor PMN. The diffuse scattering appears around the Burns temperature (~620K), indicating its origin from the polar nanoregions (PNR). While the relative diffuse intensities are…

材料科学 · 物理学 2009-11-07 K. Hirota , Z. -G. Ye , S. Wakimoto , P. M. Gehring , G. Shirane

Neutron inelastic scattering measurements of the polar TO phonon mode in the cubic relaxor Pb(Mg1/3Nb2/3)O3, at room temperature, reveal anomalous behavior similar to that recently observed in the Pb(Zn1/3Nb2/3)_{0.92}Ti_{0.08}O3 system in…

材料科学 · 物理学 2009-10-31 P. M. Gehring , S. B. Vakhrushev , G. Shirane

Raman scattering in the three-dimensional Dirac semimetal Cd3As2 shows an intricate interplay of electronic and phonon degrees of freedom. We observe resonant phonon scattering due to interband transitions, an anomalous anharmonicity of…

材料科学 · 物理学 2017-07-05 A. Sharafeev , V. Gnezdilov , R. Sankar , F. C. Chou , P. Lemmens

The relaxor ferroelectric PbMg1/Nb2/3O3 was investigated by means of broad-band dielectric and Fourier Transform Infrared (FTIR) transmission spectroscopy in the frequency range from 1 MHz to 15 THz at temperatures between 20 and 900 K…

材料科学 · 物理学 2009-11-10 S. Kamba , M. Kempa , V. Bovtun , J. Petzelt , K. Brinkman , N. Setter

We present a neutron scattering study of phonons in single crystals of (Pb$_{0.5}$Sn$_{0.5}$)$_{1-x}$In$_x$Te with $x=0$ (metallic, but nonsuperconducting) and $x=0.2$ (nonmetallic normal state, but superconducting). We map the phonon…

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