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相关论文: New low-temperature phases in NaxCoO2 linked to qu…

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We report the divergence of the nonlinear component of the bulk susceptibility in NaxCoO2 (0.3<x<0.62) as T goes to 0 K. These experiments provide an striking evidence of the existence of a ferromagnetic phase transition at zero Kelvin…

强关联电子 · 物理学 2007-05-23 F. Rivadulla , M. Banobre-Lopez , M. A. Lopez-Quintela , J. Rivas

Thermodynamic and transport measurements on NaxCoO2 (x ~ 0.7-0.75) over a wide temperature range reveal a strongly enhanced low energy excitation spectrum. The zero-field specific heat and resistance at low temperature are proportional to…

强关联电子 · 物理学 2007-05-23 M. Brühwiler , B. Batlogg , S. M. Kazakov , J. Karpinski

We synthesized Nax(H3O)zCoO2yH2O samples with various Na/H3O ratios but with the constant Co valence of s = +3.40, and measured their magnetic properties to draw phase diagrams of the system. The superconductivity is very sensitive to the…

超导电性 · 物理学 2009-11-11 H. Sakurai , K. Takada , T. Sasaki , E. Takayama-Muromachi

Data taken by various kinds of methods including NMR/NQR and neutron scattering are presented for NaxCoO2, in particular, for Na0.5CoO2. Attentions have also been paid to the x dependence of the electronic nature. The pseudo-gap-like…

Powder Na$_{x}$CoO$_{2}$ ($0.70\leq x\leq 0.84$) samples were synthesized and characterized carefully by X-ray diffraction analysis, inductive-coupled plasma atomic emission spectroscopy, and redox titration. It was proved that…

材料科学 · 物理学 2009-11-10 H. Sakurai , S. Takenouchi , N. Tsujii , E. Takayama-Muromachi

Here we report the magnetic properties of the layered cobalt oxide system, LixCoO2, in the whole range of Li composition, 0 <= x <= 1. Based on dc-magnetic susceptibility data, combined with results of 59Co-NMR/NQR observations, the…

强关联电子 · 物理学 2009-10-17 T. Motohashi , T. Ono , Y. Sugimoto , Y. Masubuchi , S. Kikkawa , R. Kanno , M. Karppinen , H. Yamauchi

We have performed specific heat and electric resistivity measurements of Na$_{x}$CoO$_{2}$ ($x=0.70$-0.78). Two anomalies have been observed in the specific heat data for $x=0.78$, corresponding to magnetic transitions at $T_{c}=22$ K and…

材料科学 · 物理学 2009-11-10 H. Sakurai , N. Tsujii , E. Takayama-Muromachi

Using muon spin rotation, well-defined bulk ~ 100% magnetic phases in NaxCoO2 are revealed. A novel magnetic phase is detected for x = 0.85 with the highest transition temperature ever observed for x >= 0.75. This stresses the diversity of…

Specific heat of the layered NaxCoO2 (x=0.65, 0.70 and 0.75) oxides has been measured in the temperature range of 3-360 K and magnetic field of 0 and 9 T. The analysis of data, assuming the combined effect of inter-layer superexchange and…

强关联电子 · 物理学 2009-11-11 A. Zorkovska , M. Orendac , J. Sebek , E. Santava , P. Svoboda , I. Bradaric , I. Savic , A. Feher

We prove the direct link between low temperature magnetism and high temperature sodium ordering in NaxCoO2 using the example of a heretofore unreported magnetic transition at 8 K which involves a weak ferromagnetic moment. The 8 K feature…

强关联电子 · 物理学 2009-11-13 T. F. Schulze , P. S. Häfliger , C. Niedermayer , K. Mattenberger , S. Bubenhofer , B. Batlogg

Magnetic properties of the novel layered superconductor, Na$_{0.35}$CoO$_{2}$$\cdot$1.3H$_{2}$O have been investigated. From the temperature dependence and field dependence of the magnetization, the superconducting transition temperature,…

Studies of the NMR Knight shift K of Na0.3CoO2.yH2O have been carried out in detail. The suppression of K by the occurrence of the superconductivity reported previously by the present authors in both magnetic field directions perpendicular…

超导电性 · 物理学 2009-11-11 Yoshiaki Kobayashi , Taketo Moyoshi , Hidekazu Watanabe , Mai Yokoi , Masatoshi Sato

Electronic properties of the sodium cobaltate NaxCoO2 are systematically studied through a precise control of band filling. Resistivity, magnetic susceptibility and specific heat measurements are carried out on a series of high-quality…

We have synthesized and characterized four different stable phases of Na ordered Na$_{x}$CoO$_{2}$, for $0.65<x<0.8$. Above 100 K they display similar Curie-Weiss susceptibilities as well as ferromagnetic $q=0$ spin fluctuations in the…

强关联电子 · 物理学 2008-03-12 H. Alloul , I. R. Mukhamedshin , G. Collin , N. Blanchard

We measured the resistivity and magnetic susceptibility to map out the phase diagram of single crystalline NaFe$_{1-x}$Co$_x$As. Replacement of Fe by Co suppresses both the structural and magnetic transition, while enhances the…

超导电性 · 物理学 2012-06-21 A. F. Wang , X. G. Luo , Y. J. Yan , J. J. Ying , Z. J. Xiang , G. J. Ye , P. Cheng , Z. Y. Li , W. J. Hu , X. H. Chen

The magnetic properties of alkali-metal peroxychromate K$_2$NaCrO$_8$ are governed by the $S = 1/2$ pentavalent chromium cation, Cr$^{5+}$. Specific heat, magnetocalorimetry, ac magnetic susceptibility, torque magnetometry, and inelastic…

We have performed a temperature-dependent photoemission study of a NaxCoO2 (x~0.8) epitaxial thin film prepared by the reactive solid-phase epitaxy method. The chemical potential shift as a function of temperature was derived from the Co 3d…

强关联电子 · 物理学 2007-10-11 Y. Ishida , H. Ohta , A. Fujimori , H. Hosono

Dimerized magnets forming alternating Heisenberg chains exhibit quantum coherence and entanglement and thus can find potential applications in quantum information and computation. However, magnetic systems typically undergo thermal…

We synthesized the five batches of the samples of the novel P3 type superconductor, Na$_{x}$(H$_{3}$O)$_{y'}$CoO$_{2}\cdot y''$H$_{2}$O, by the soft chemical process starting from $\alpha$-NaCoO$_{2}$. The chemical and structural properties…

超导电性 · 物理学 2009-11-10 H. Sakurai , K. Takada , T. Sasaki , F. Izumi , R. A. Dilanian , E. Takayama-Muromachi

Magnetic, transport, and specific heat measurements have been performed on layered metallic oxide Na$_{1.5}$Co$_2$O$_4$ as a function of temperature $T$. Below a characteristic temperature $T^*$=30$-$40 K, electrical resistivity shows a…

强关联电子 · 物理学 2009-11-10 K. Miyoshi , E. Morikuni , K. Fujiwara , J. Takeuchi , T. Hamasaki
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