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Exchanged interactions in recently observed helical structure in LiCu2O2 is probed by inelastic neutron scattering. The main conlusions of Refs. [1,2] are confirmed: nn interactions in single chains are ferromagnetic and frustrated by nnn…

强关联电子 · 物理学 2009-11-10 T. Masuda , A. Zheludev , A. Bush , M. Markina , A. Vasiliev

Neutron diffraction and bulk measurements are used to determine the nature of the low-temperature ordered state in LiCu$_2$O$_2$, a $S=1/2$ spin-chain compound with competing interactions. The magnetic structure is found to be helimagnetic,…

强关联电子 · 物理学 2007-05-23 T. Masuda , A. Zheludev , A. Bush , M. Markina , A. Vasiliev

The quasi-one-dimensional helimagnet LiCu2O2 was studied by single crystal inelastic neutron scattering. The dispersion relation of spin wave excitations was measured in the vicinity of the principal magnetic Bragg reflection. A spin wave…

强关联电子 · 物理学 2009-11-10 T. Masuda , A. Zheludev , B. Roessli , A. Bush , M. Markina A. Vasiliev

We show by unbiased numerical calculations that the ferromagnetic nearest-neighbor exchange interaction stabilizes a vector spin chiral order against the quantum fluctuation in a frustrated spin-1/2 chain relevant to multiferroic cuprates,…

强关联电子 · 物理学 2015-05-18 Shunsuke Furukawa , Masahiro Sato , Shigeki Onoda

We show that LiVCuO4 should be described by strongly ferromagnetically coupled Heisenberg antiferromagnetic chains (HAC) in sharp contrast with the effective exchange integrals Ji given in Enderle et al., Phys. Rev. Lett. vol. 104, 237207…

A ferroelectric transition occurring simultaneously with helical spin order has been found in both the polycrystalline and single crystal samples of LiCuVO4. The system has Cu2+ spins (s=1/2) of the CuO2 chains formed of edge-sharing CuO4…

强关联电子 · 物理学 2015-06-25 Yutaka Naito , Kenji Sato , Yukio Yasui , Yusuke Kobayashi , Yoshiaki Kobayashi , Masatoshi Sato

In a frustrated J_1-J_2 chain with the nearest-neighbor ferromagnetic interaction J_1 and the next-nearest-neighbor antiferromagnetic interaction J_2, novel magnetic states such as a spin-nematic state are theoretically expected. However,…

A complete phase diagram of Zn substituted quantum quasi-two-dimensional helimagnet LiCu2O2 has been presented. Helical ordering transition temperature (T_h) of the original LiCu2O2 follows finite size scaling for less than ~ 5.5% Zn…

强关联电子 · 物理学 2013-05-29 H. C. Hsu , J. -Y. Lin , W. L. Lee , M. -W. Chu , T. Imai , Y. J. Kao , C. D. Hu , H. L. Liu , F. C. Chou

A spin model of quasi-one dimensional LiCu$_{2}$O$_{2}$ compound with ground state of ellipsoidal helical structure in which the helical axis is along the diagonal of CuO$_{4}$ squares has been adopted. By taking into account the interchain…

材料科学 · 物理学 2015-06-18 Yan Qi , An Du

We report susceptibility, specific heat, and neutron diffraction measurements on NaCu$_2$O$_2$, a spin-1/2 chain compound isostructural to LiCu$_2$O$_2$, which has been extensively investigated. Below 13 K, we find a long-range ordered,…

强关联电子 · 物理学 2013-05-29 L. Capogna , M. Mayr , P. Horsch , M. Raichle , R. K. Kremer , M. Sofin , A. Maljuk , M. Jansen , B. Keimer

In a comment on arXiv:1006.5070v2, Drechsler et al. claim that the frustrated ferromagnetic spin-1/2 chain LiCuVO4 should be described by a strong rather than weak ferromagnetic nearest-neighbor interaction, in contradiction with their…

强关联电子 · 物理学 2011-03-21 M. Enderle , B. Fak , H. -J. Mikeska , R. K. Kremer

Starting from \textit{ab-initio} calculations, we derive a five-band Hubbard model to describe the CuO$_2$ chains of LiCu$_2$O$_2$. This model is further simplified to a low-energy effective Heisenberg model with nearest-neighbor (NN)…

强关联电子 · 物理学 2023-12-14 N. Aucar Boidi , Christian Helman , Y. Núñez-Fernández , K. Hallberg , A. A. Aligia

In a comment on arXiv:1006.5070v1, Drechsler et al. present new band-structure calculations suggesting that the frustrated ferromagnetic spin-1/2 chain LiCuVO4 should be described by a strong rather than weak ferromagnetic nearest-neighbor…

强关联电子 · 物理学 2010-09-09 M. Enderle , B. Fåk , H. -J. Mikeska , R. K. Kremer

The magnetic structure of the edge sharing cuprate compound Li2CuO2 has been investigated by means of ab initio electronic structure calculations. The first and second neighbor in-chain magnetic interactions are calculated to be -142 K and…

We report the crystal structure, magnetization measurements, and band-structure calculations for the spin-1/2 quantum magnet CaCu2(SeO3)2Cl2. The magnetic behavior of this compound is well reproduced by a uniform spin-1/2 chain model with…

In a recent work devoted to the magnetism of Li$_{2}$CuO$_{2}$, Shu et al. [New J. Phys. 19 (2017) 023026] have proposed a "simplified" unfrustrated microscopic model that differs considerably from the models refined through decades of…

Neutron diffraction and 7Li-NMR have been applied to determine the multiferroic system LiCu2O2, which has four chains (ribbon chains) of edge-sharing CuO4 square planes in a unit cell. We have confirmed that there are successive magnetic…

On the basis of first principles density functional theory electronic structure calculations as well as classical spin analysis, we explored why the magnetic oxide Li2CuO2, consisting of CuO2 ribbon chains made up of edge-sharing CuO4…

强关联电子 · 物理学 2008-01-04 H. J. Xiang , C. Lee , M. -H. Whangbo

Raman scattering studies of the frustrated spin chain system LiCu$_{2}$O$_{2}$ are reported. Two transitions into a magnetically ordered phase (taken place at temperatures $\sim$ 9 K and $\sim$ 24 K) have been confirmed from the analysis of…

强关联电子 · 物理学 2009-11-10 K. -Y. Choi , S. A. Zvyagin , G. Cao , P. Lemmens

LiCu2O2 is the first multiferroic cuprate to be reported and its ferroelectricity is induced by complex magnetic ordering in ground state, which is still in controversy today. Herein, we have grown nearly untwinned LiCu2O2 single crystals…

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