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Neutron and x-ray diffraction techniques have been used to study the competing long and short-range polar order in the relaxor ferroelectric Pb(Mg$_{1/3}$Nb$_{2/3}$)O$_{3}$ (PMN) under a [111] applied electric field. Despite reports of a…

材料科学 · 物理学 2009-11-13 C. Stock , Guangyong Xu , P. M. Gehring , H. Luo , X. Zhao , H. Cao , J. F. Li , D. Viehland , G. Shirane

Diffuse neutron scattering is a valuable tool to obtain information about the size and orientation of the polar nanoregions that are a characteristic feature of relaxor ferroelectrics. In this paper, we present new diffuse scattering…

材料科学 · 物理学 2009-11-07 D. La-Orauttapong , J. Toulouse , Z. -G. Ye , R. Erwin , J. L. Robertson , W. Chen

We have performed elastic diffuse neutron scattering studies on the relaxor Pb(Mg$_{1/3}$Nb$_{2/3}$)O$_3$ (PMN). The measured intensity distribution near a (100) Bragg peak in the (hk0) scattering plane assumes the shape of a butterfly with…

材料科学 · 物理学 2009-11-10 Guangyong Xu , G. Shirane , J. R. D. Copley , P. M. Gehring

We have performed a series of neutron diffuse scattering measurements on a single crystal of the solid solution Pb(Zn$_{1/3}$Nb$_{2/3}$)O$_3$ (PZN) doped with 8% PbTiO$_3$ (PT), a relaxor compound with a Curie temperature T$_C \sim 450$ K,…

材料科学 · 物理学 2009-11-11 Guangyong Xu , P. M. Gehring , G. Shirane

We report measurements of the neutron diffuse scattering from a single crystal of the relaxor ferroelectric Pb(Zn_1/3Nb_2/3)O_3 doped with 8% PbTiO_3 (PZN-8%PT) for temperatures 100 K < T < 530 K and electric fields 0 kV/cm < E < 10 kV/cm.…

材料科学 · 物理学 2009-11-10 P. M. Gehring , K. Ohwada , G. Shirane

Diffuse scattering around the (110) reciprocal lattice point has been investigated by elastic neutron scattering in the paraelectric and the relaxor phases of the disordered complex perovskite crystal-Pb(Zn1/3Nb2/3)O3(PZN). The appearance…

材料科学 · 物理学 2009-11-07 D. La-Orauttapong , J. Toulouse , J. L. Robertson , Z. -G. Ye

Using neutron pair distribution function (PDF) analysis over the temperature range from 1000 K to 15 K, we demonstrate the existence of local polarization and the formation of medium-range, polar nanoregions (PNRs) with local rhombohedral…

无序系统与神经网络 · 物理学 2009-11-10 I. -K. Jeong , T. W. Darling , J. K. Lee , Th. Proffen , R. H. Heffner , J. S. Park , K. S. Hong , W. Dmowski , T. Egami

We have characterized the dynamics of the polar nanoregions in Pb(Mg$_{1/3}$Nb$_{2/3}$)O$_{3}$ (PMN) through high-resolution neutron backscattering and spin-echo measurements of the diffuse scattering cross section. We find that the diffuse…

Single crystals of the relaxor PZN-xPT display an enormously strong piezoelectric character. Recent x-ray scattering studies have revealed novel electric-field induced phase transitions in PZN-8%PT. As-grown crystals exhibit a rhombohedral…

X-ray and neutron scattering studies of the lead-based family of perovskite relaxors PZN-$x$PT and PMN-$x$PT have documented a highly unusual situation in which the near-surface region of a single crystal can exhibit a structure that is…

材料科学 · 物理学 2007-05-23 Guangyong Xu , P. M. Gehring , C. Stock , K. Conlon

The relaxor ferroelectric PbMg_1/3Ta_2/3O_3 was studied by single-crystal neutron and synchrotron x-ray diffraction and its detailed atomic structure has been modeled in terms of static Pb-displacements that lead to the formation of polar…

We report measurements of the evolution of the diffuse scattering in a single crystal PbMg1/3Nb2/3O3 as a function of hydrostatic pressure. Upon applying pressure the diffuse scattering intensity decreases and is suppressed at about 3 GPa,…

材料科学 · 物理学 2009-10-13 G -M Rotaru , B Padmanabhan , S N Gvasaliya , B Roessli , Th Strassle , R A Cowley , S G Lushnikov , S Klotz

High energy x-ray diffraction measurements on Pb(Zn$_{1/3}$Nb$_{2/3}$)O$_3$ (PZN) single crystals show that the system does not have a rhombohedral symmetry at room temperature as previously believed. The new phase (X) in the bulk of the…

强关联电子 · 物理学 2009-11-07 Guangyong Xu , Z. Zhong , Y. Bing , Z. -G. Ye , C. Stock , G. Shirane

We report neutron diffuse scattering measurements on a single crystal of 68%Pb(Mg1/3Nb2/3)O3-32%PbTiO3. Strong diffuse scattering is observed at low temperatures. An external field applied along the [001] direction affects the diffuse…

材料科学 · 物理学 2008-08-26 Jinsheng Wen , Guangyong Xu , C. Stock , P. M. Gehring

We present a generalized method to describe the x-ray scattering intensity of the Bragg spots in a diffraction pattern from nanocrystals exposed to intense x-ray pulses. Our method involves the subdivision of a crystal into smaller units.…

原子与分子团簇 · 物理学 2017-08-24 Malik Muhammad Abdullah , Zoltan Jurek , Sang-Kil Son , Robin Santra

We present high energy x-ray (67 keV) and neutron scattering measurements on a single crystal of K$_{1-x}$Li$_x$TaO$_3$ for which the Li content ($x=0.02$) is less than $x_c = 0.022$, the critical value below which no structural phase…

The spectral dependence of the Bragg peak position under conditions of extremely asymmetric diffraction has been analyzed in the kinematical and dynamical approximations of the diffraction theory. Simulations have been performed for the…

材料科学 · 物理学 2025-04-28 M A Andreeva , Yu. Repchenko , A G Smekhova , Karine Dumesnil , F. Wilhelm , A. Rogalev

High-pressure and variable temperature single crystal synchrotron X-ray measurements combined with first-principles based molecular dynamics simulations study diffuse scattering in the relaxor ferroelectric system PSN…

材料科学 · 物理学 2015-05-13 P. Ganesh , E. Cockayne , M. Ahart , R. E. Cohen , B. Burton , R. J. Hemley , Yang Ren , Wenge Yang , Z-G Ye

We discuss the applicability of holographically recorded gratings in photopolymers and holographic polymer-dispersed liquid crystals as neutron optical elements. An experimental investigation of their properties for light and neutrons with…

Neutron scattering investigations were carried out in PbMg$_{1/3}$Ta$_{2/3}$O$_3$ and BaMg$_{1/3}$Ta$_{2/3}$O$_3$ complex perovskites. The crystal structure of both compounds does not show any phase transition in the temperature range 1.5…

材料科学 · 物理学 2007-05-23 S. N. Gvasaliya , B. Roessli , D. Sheptyakov , S. G. Lushnikov , T. A. Shaplygina
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