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We report experimental studies of crystals of Mn12 molecular magnetic clusters in pulsed magnetic fields with sweep rates up to 4x10^3 T/s. The steps in the magnetization curve are observed at fields that are shifted with respect to the…
The magnetization of the prototypical molecular magnet Mn12-acetate exhibits a series of sharp steps at low temperatures due to quantum tunneling at specific resonant values of magnetic field applied along the easy c-axis. An abrupt…
The reversal of the magnetization of crystals of molecular magnets that have a large spin and high anisotropy barrier generally proceeds below the blocking temperature by quantum tunneling. This is manifested as a series of controlled steps…
The spin relaxation in the molecular magnet \Mn12 is investigated by a novel type of high-frequency magnetic spectroscopy. By reversing the external magnetic field the intensities of the $|\pm 10>\to |\pm 9>$ transitions within the ground…
We present a comprehensive derivation of the magnetization relaxation in a Mn12-acetate crystal based on thermally assisted spin tunneling induced by quartic anisotropy and weak transverse magnetic fields. The overall relaxation rate as…
We study the magnetization reversal and electromagnetic radiation due to collective Landau-Zener relaxation in a crystal of molecular magnets. Analytical and numerical solutions for the time dependence of the relaxation process are…
For the first time, the morphology and dynamics of spin avalanches in Mn12-Acetate crystals using magneto-optical imaging has been explored. We observe an inhomogeneous relaxation of the magnetization, the spins reversing first at one edge…
A magnetic particle with atomic spins ordered in an unstable direction is an example of a false vacuum that decays via excitation of internal spin waves. Coupled evolution of the particle's magnetization (or the vacuum state) and spin…
Magnetization reversal in magnetic nanostructures is investigated numerically over time-scales ranging from fast switching processes on a picosecond scale to thermally activated reversal on a microsecond time-scale. A simulation of the…
Using micron-sized thermometers and Hall bars, we report time-resolved studies of the local temperature and local magnetization for two types of magnetic avalanches (abrupt spin reversals) in the molecular magneti Mn12-acetate,…
We present a comprehensive theory of the magnetization relaxation in a Mn12-acetate crystal in the high-temperature regime (T>1 K), which is based on phonon-assisted spin tunneling induced by quartic magnetic anisotropy and weak transverse…
By numerically solving the equations of motion for atomic spins we show that internal spin-wave processes in large enough magnetic particles, initially in unstable states, lead to complete magnetization reversal and thermalization. The…
Magnetization reversal in magnetic particles is one of the fundamental issues in magnetic data storage. Technological improvements require the understanding of dynamical magnetization reversal processes at nanosecond time scales. New…
Crystals of the molecular magnet Mn12-acetate are known to contain a small fraction of low- symmetry (minor) species with a small anisotropy barrier against spin reversal. The lower barrier leads to faster magnetic relaxation and lower…
Quantum nanomagnets can show a field dependence of the relaxation time very different from their classical counterparts, due to resonant tunneling via excited states (near the anisotropy barrier top). The relaxation time then shows minima…
An effective method for ultrafast magnetization reversal of nanoclusters is suggested. The method is based on coupling a nanocluster to a resonant electric circuit. This coupling causes the appearance of a magnetic feedback field acting on…
We show that a slowly decaying current pulse can lead to nearly deterministic precessional switching in the presence of noise. We consider a biaxial macrospin, with an easy axis in the plane and a hard axis out-of-the plane, typical of thin…
We study the precessional switching of the magnetization in microscopic spin valve cells induced by ultra short in-plane hard axis magnetic field pulses. Stable and highly efficient switching is monitored following pulses as short as 140 ps…
We report measurements and theoretical analysis of resonant spin tunneling in randomly oriented nanospheres of a molecular magnet. Amorphous nanospheres of Mn$_{12}$ acetate have been fabricated and characterized by chemical, infrared, TEM,…
Using micron-sized Hall sensor arrays to obtain time-resolved measurements of the local magnetization, we report a systematic study in the molecular magnet Mn$_{12}$-acetate of magnetic avalanches controllably triggered in different fixed…