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The electrodynamic response of DNA in the millimeter wave range is investigated. By performing measurements under a wide range of humidity conditions and comparing the response of single strand DNA and double strand DNA, we show that the…

无序系统与神经网络 · 物理学 2015-06-24 M. Briman , N. P. Armitage , E. Helgren , G. Gruner

Measurements of electron transfer rates as well as of charge transport characteristics in DNA produced a number of seemingly contradictory results, ranging from insulating behaviour to the suggestion that DNA is an efficient medium for…

软凝聚态物质 · 物理学 2007-05-23 R. Bulla , R. Gutierrez , G. Cuniberti

Charge transfer in a DNA duplex chain is studied by constructing a system with virtual electrodes connected at the ends of each DNA strand. The systeym is described by the tight-binding model and its transport is analyzed by the transfer…

介观与纳米尺度物理 · 物理学 2009-11-11 X. F. Wang , Tapash Chakraborty

Numerous experiments on charge transfer in DNA yield a contradictory picture of the transfer: on the one hand they suggest that it is a very slow process and the charge is almost completely localized on one Watson-Crick pair, but on the…

生物物理 · 物理学 2013-04-22 V. D. Lakhno , V. B. Sultanov

Charge migration along DNA molecules has attracted scientific interest for over half a century. Reports on possible high rates of charge transfer between donor and acceptor through the DNA, obtained in the last decade from solution…

材料科学 · 物理学 2009-11-10 Danny Porath , Gianaurelio Cuniberti , Rosa Di Felice

An 1d model with time-dependent random hopping is proposed to describe charge transport in DNA. It admits to investigate both diffusion of electrons and their tunneling between different sites in DNA. The tunneling appears to be strongly…

软凝聚态物质 · 物理学 2009-11-07 E. I. Kats , V. V. Lebedev

The bias-dependent transport properties of short poly(G)-poly(C) A-DNA strands attached to Au electrodes are investigated with first principles electronic transport methods. By using the non- equilibrium Green's function approach combined…

介观与纳米尺度物理 · 物理学 2015-05-19 C. D. Pemmaraju , I. Rungger , X. Chen , A. R. Rocha , S. Sanvito

The dielectrophoresis method for trapping and attaching nanoscale double-stranded DNA between nanoelectrodes was developed. The method gives a high yield of trapping single or a few molecules only which enables transport measurements at the…

软凝聚态物质 · 物理学 2007-05-23 S. Tuukkanen , A. Kuzyk , J. J. Toppari , V. P. Hytonen , T. Ihalainen , P. Torma

We propose a model Hamiltonian for charge transfer along the DNA double helix with temperature driven fluctuations in the base pair positions acting as the rate limiting factor for charge transfer between neighboring base pairs. We compare…

软凝聚态物质 · 物理学 2009-10-31 R. Bruinsma , G. Gruner , M. R. D'Orsogna , J. Rudnick

Charge transfer can take place along double helical DNA over distances as long as 30 nanometers. However, given the active role of the thermal environment surrounding charge carriers in DNA, physical mechanisms driving the transfer process…

介观与纳米尺度物理 · 物理学 2020-12-04 Roman Korol , Dvira Segal

We investigate the charge transfer characteristics of one and two excess charges in a DNA base-pair dimer using a model Hamiltonian approach. The electron part comprises diagonal and off-diagonal Coulomb matrix elements such a correlated…

强关联电子 · 物理学 2015-05-14 Sabine Tornow , Ralf Bulla , Frithjof B. Anders , Gertrud Zwicknagl

The question of whether DNA conducts electric charges is intriguing to physicists and biologists alike. The suggestion that electron transfer/transport in DNA might be biologically important has triggered a series of experimental and…

无序系统与神经网络 · 物理学 2020-05-04 H. Wang , R. Marsh , J. P. Lewis , R. A. Roemer

We study the electronic properties of DNA by way of a tight-binding model applied to four particular DNA sequences. The charge transfer properties are presented in terms of localisation lengths, crudely speaking the length over which…

基因组学 · 定量生物学 2007-05-23 Daphne Klotsa , Rudolf A. Roemer , Matthew S. Turner

Recent works on localized charge transport along DNA, based on a three--dimensional, tight--binding model (Eur. Phys. J. B 30:211, 2002; Phys. D 180:256, 2003), suggest that charge transport is mediated by the coupling of the radial and…

斑图形成与孤子 · 物理学 2007-05-23 F. Palmero , J. F. R. Archilla , D. Hennig , F. R. Romero

The complex mechanisms governing charge migration in DNA oligomers reflect the rich structural and electronic properties of the molecule of life. Controlling the mechanical stability of DNA nanowires in charge transport experiments is a…

介观与纳米尺度物理 · 物理学 2015-05-13 Bo Song , Marcus Elstner , Gianaurelio Cuniberti

Microscopic mechanisms of positive charge transfer in DNA remain unclear. A quantum state of electron hole in DNA is determined by the competition of a pi-stacking interaction $b$ smearing a charge between different base pairs and…

软凝聚态物质 · 物理学 2008-03-15 D. B. Uskov , A. L. Burin

A theoretical study is presented to quantitatively analyze the transport experiment through individual DNA molecules reported recently by Porath {\it et al.} [Nature {\bf 403}, 635 (2000)]. A variety of valuable quantities are identified by…

介观与纳米尺度物理 · 物理学 2009-11-07 Xin-Qi Li , YiJing Yan

Experiments have revealed correlation-driven behavior of DNA in charged solutions, including charge inversion and condensation. This paper presents calculations of a lattice-gas model of charge inversion for the adsorption of charged dimers…

软凝聚态物质 · 物理学 2019-02-15 Matthew D. Sievert , Marilyn F. Bishop , Tom McMullen

Quantum transport for DNA conduction has widely studied with interest in application as a candidate in making nanowires as well as interest in the scientific mechanism. In this paper, we review recent works with concerning the electronic…

无序系统与神经网络 · 物理学 2015-03-13 Hiroaki Yamada , Kazumoto Iguchi

The dependence of DNA assemblies conductance on relative humidity is investigated theoretically. Following earlier suggestions, we consider the ionic conductivity through the layers of water adsorbed by DNA molecules. The increase in…

化学物理 · 物理学 2015-05-14 J. M. Leveritt , S. Tesar , C. Dibaya , R. Shrestha , A. L. Burin
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