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相关论文: Infrared optical properties of the spin-1/2 quantu…

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We report infrared and Raman spectroscopy results of the spin-1/2 quantum magnet TiOCl. Giant anomalies are found in the temperature dependence of the phonon spectrum, which hint to unusual coupling of the electronic degrees of freedom to…

强关联电子 · 物理学 2022-06-08 P. Lemmens , K. Y. Choi , G. Caimi , L. Degiorgi , N. N. Kovaleva , A. Seidel , F. C. Chou

We have studied the S=1/2 quasi-one-dimensional antiferromagnet TiOCl using single crystal x-ray diffraction and inelastic x-ray scattering techniques. The Ti ions form staggered spin chains which dimerize below Tc1 = 66 K and have an…

强关联电子 · 物理学 2009-11-13 E. T. Abel , K. Matan , F. C. Chou , E. D. Isaacs , D. E. Moncton , H. Sinn , A. Alatas , Y. S. Lee

We have investigated the spin fluctuations and their interplay with lattice instabilities in a layered S=1/2 quantum spin system TiOCl. Our Ti and Cl NMR data demonstrate a pseudo spin-gap behavior below T*=135 K, followed by successive…

强关联电子 · 物理学 2007-05-23 T. Imai , F. C. Chou

We have used a combination of neutron resonant spin-echo and triple-axis spectroscopies to determine the energy, fine structure, and linewidth of the magnon resonance in the model spin-1/2 ladder antiferromagnet IPA-CuCl_3 at temperatures T…

强关联电子 · 物理学 2015-03-18 B. Náfrádi , T. Keller , H. Manaka , A. Zheludev , B. Keimer

We have measured near normal incidence far infrared (FIR) reflectivity spectra of a single crystal of TbMnO3 from 10K to 300K in the spectral range of 50 cm$^{-1}$ to 700 cm$^{-1}$. Fifteen transverse optic (TO) and longitudinal optic (LO)…

材料科学 · 物理学 2015-05-13 Pradeep Kumar , Surajit Saha , C. R. Serrao , A. K. Sood , C. N. R. Rao

In the layered quantum spin systems TiOCl and TiOBr the magnetic susceptibility shows a very weak temperature dependence at high temperatures and transition-induced phenomena at low temperatures. There is a clear connection of the observed…

强关联电子 · 物理学 2010-03-09 P. Lemmens , K. Y. Choi , R. Valenti , T. Saha-Dasgupta , E. Abel , Y. S. Lee , F. C. Chou

Spin and lattice dynamics of CaMn7O12 ceramics were investigated using infrared, THz and inelastic neutron scattering (INS) spectroscopies in the temperature range 2 to 590 K, and, at low temperatures, in applied magnetic fields of up to 12…

Measurements of the heat capacity C(T,H) of the one-dimensional quantum magnet TiOCl are presented for temperatures 2K < T < 300K and magnetic fields up to 5T. Distinct anomalies at 91K and 67K signal two subsequent phase transitions. The…

强关联电子 · 物理学 2007-05-23 J. Hemberger , M. Hoinkis , M. Klemm , M. Sing , R. Claessen , S. Horn , A. Loidl

Temperature-dependent x-ray diffraction of the low-dimensional spin 1/2 quantum magnet TiOCl shows that the phase transition at T_{c2} = 90 K corresponds to a lowering of the lattice symmetry. Below T_{c1} = 66 K a twofold superstructure…

材料科学 · 物理学 2009-11-11 M. Shaz , S. van Smaalen , L. Palatinus , M. Hoinkis , M. Klemm , S. Horn , R. Claessen

We present the electrodynamic response of TiOBr, which undergoes a transition to a spin-singlet ground state for temperatures below T$_{C1}=28$ K. The temperature evolution of the phonon anomalies indicates, like in \cl, an extended…

材料科学 · 物理学 2009-11-10 G. Caimi , L. Degiorgi , P. Lemmens , F. C. Chou

We report temperature-dependent Raman scattering and X-ray diffraction studies of pyrochlore iridates, (Eu$_{1-x}$Bi$_x$)$_2$Ir$_2$O$_7$, for x=0, 0.02, 0.035, 0.05 and 0.1. The temperature variation in Raman experiments spans from 4 K to…

Raman scattering experiments on stoichiometric, Mott-insulating LaTiO$_3$ over a wide range of excitation energies reveal a broad electronic continuum which is featureless in the paramagnetic state, but develops a gap of $\sim 800$…

强关联电子 · 物理学 2015-10-28 C. Ulrich , G. Khaliullin , M. Guennou , H. Roth , T. Lorenz , B. Keimer

Band calculations on HgBa$_2$CuO$_4$ and La$_{(2-x)}$Sr$_x$CuO$_4$ with phonon and spin-waves within the CuO planes show that partial gaps are created at various energies depending on wavelengths. Spin and phonon gaps appear at different…

超导电性 · 物理学 2009-11-11 T. Jarlborg

We present a comprehensive study of polar and magnetic excitations in BiFeO3 ceramics and a thin film epitaxially grown on an orthorhombic (110) TbScO3 substrate. Infrared reflectivity spectroscopy was performed at temperatures from 5 to…

材料科学 · 物理学 2015-05-22 S. Skiadopoulou , V. Goian , C. Kadlec , F. Kadlec , X. F. Bai , I. C. Infante , B. Dkhil , C. Adamo , D. G. Schlom , S. Kamba

We present a $^{125}$Te nuclear magnetic resonance (NMR) study in the three-dimensional spin web lattice Cu$_3$TeO$_6$, which harbors topological magnons. The $^{125}$Te NMR spectra and the Knight shift $\mathcal{K}$ as a function of…

强关联电子 · 物理学 2021-08-04 Seung-Ho Baek , Hyeon Woo Yeo , Jena Park , Kwang-Yong Choi , Bernd Büchner

We have studied the electronic structure of the spin-1/2 quantum magnet TiOCl by polarization-dependent momentum-resolved photoelectron spectroscopy. From that, we confirm the quasi-one-dimensional nature of the electronic structure along…

Inelastic light scattering studies on single crystal of electron-doped Ca(Fe0.95Co0.05)2As2 superconductor, covering the tetragonal to orthorhombic structural transition as well as magnetic transition at TSM ~ 140 K and superconducting…

We report experimental results on the heat conductivity \kappa of the S=1/2 spin chain compounds TiOBr and TiOCl for temperatures 5K<T<300K and magnetic fields up to 14. Surprisingly, we find no evidence of a significant magnetic…

强关联电子 · 物理学 2010-04-30 N. Hlubek , M. Sing , S. Glawion , R. Claessen , S. van Smaalen , P. H. M. van Loosdrecht , B. Büchner , C. Hess

The temperature evolution of the electron spin resonance is studied at cooling the crystal samples of Cs2CuCl4 through the Neel point 0.62 K. A coexistence of the high-frequency spinon type resonance developed in the spin-liquid phase and…

强关联电子 · 物理学 2013-05-30 A. I. Smirnov , K. Yu. Povarov , S. V. Petrov , A. Ya. Shapiro

We present detailed ESR investigations on single crystals of the low-dimensional quantum magnet TiOCl. The anisotropy of the g-factor indicates a stable orbital configuration below room temperature, and allows to estimate the energy of the…

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