相关论文: Photon-assisted tunneling in a Fe8 Single-Molecule…
We measure magnetization changes in a single crystal of the single-molecule magnet Fe8 when exposed to intense, short (<20 $\mu$s) pulses of microwave radiation resonant with the m = 10 to 9 transition. We find that radiation induces a…
We report measurements on magnetization reversal in the Fe$_8$ molecular magnet using fast pulsed magnetic fields of 1.5 kT/s and in the temperature range of 0.6-4.1 K. We observe and analyze the temperature dependence of the reversal…
Single molecule magnets straddle the classical and quantum mechanical worlds, displaying many fascinating phenomena. They may have important technological applications in information storage and quantum computation. We review the physical…
We have studied the crossover between thermally assisted and pure quantum tunneling in single crystals of high spin (S=10) uniaxial single molecule magnet Mn12-acetate using micro-Hall effect magnetometry. Magnetic hysteresis experiments…
We review the present state of theory and experiments on the quantum tunneling of magnetization in mesoscopic spin systems. Most attention is paid to the relaxation of magnetization in the molecular complexes Mn12 and Fe8. The role of the…
We investigate the effect of dynamic nuclear spin fluctuation on quantum tunneling of the magnetization (QTM) in the molecular magnet Fe8 by increasing the nuclei temperature using radio frequency (RF) pulses before the hysteresis loop…
Resonant microwave radiation applied to a single crystal of the molecular magnet Fe_8 induces dramatic changes in the sample's magnetization. Transitions between excited states are found even though at the nominal system temperature these…
Magnetization measurements made in small fields as a function of temperature reveal an unusual equilibrium below 900 mK for the molecular nano-magnet Fe_8. Measurements of the relaxation of the magnetization demonstrate that the approach to…
We investigate real-time dynamics of spin-polarized current in a quantum dot coupled to ferromagnetic leads in both parallel and antiparallel alignments. While an external bias voltage is taken constant in time, a gate terminal,…
Spin tunneling in the particular case of the magnetic molecular cluster octanuclear iron(III), Fe8, is treated by an effective Hamiltonian that allows for an angle-based description of the process. The presence of an external magnetic field…
We study spin tunneling in magnetic molecules, with special reference to Fe8. The article aims to give a pedagogical discussion of what is meant by the tunneling of a spin, and how tunneling amplitudes or energy level splittings may be…
We consider transport through a single-molecule magnet strongly coupled to metallic electrodes. We demonstrate that for half-integer spin of the molecule electron- and spin-tunneling \emph{cooperate} to produce both quantum tunneling of the…
A new quantum approach is presented that can account for the description of small ferromagnetic particles magnetization tunneling. An estimate of the saturation value of an external applied magnetic field along the easy axis is obtained. An…
Fractional photon-assisted tunnelling is investigated both numerically and analytically in a double-well lattice. While integer photon-assisted tunnelling is a single-particle effect, fractional photon-assisted tunnelling is an…
A new approach is used that allows to describe the magnetic molecules main properties in a direct and simple way. Results obtained for the Fe8 cluster show good agreement with the experimental data.
The spin-reversal in dilute Li$_2$(Li$_{1-x}$Fe$_{x}$)N with $x < 1$ % is dominated by resonant quantum tunneling of spatially well-separated states. We report on the effect of finite couplings between those states that give rise to…
We model magnetization processes that take place through tunneling in crystals of single-molecule magnets, such as Mn_12 and Fe_8. These processes take place when a field H is applied after quenching to very low temperatures. Magnetic…
Tunneling between the two lowest energy levels of single molecule magnets with Ising type anisotropy, accompanied by the emission or absorption of phonons, is considered. Quantitatively accurate calculations of the rates for such tunneling…
The magnetic properties of dilute Li$_2$(Li$_{1-x}$Fe$_x$)N with $x \sim 0.001$ are dominated by the spin of single, isolated Fe atoms. Below $T = 10$ K the spin-relaxation times become temperature-independent indicating a crossover from…
Forbidden transitions between energy levels typically involve violation of selection rules imposed by symmetry and/or conservation laws. A nanomagnet tunneling between up and down states violates angular momentum conservation because of…