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Inelastic neutron scattering experiments on the S=1 quasi-one-dimensional bond-alternating antiferromagnet Ni(C9D24N4)(NO2)ClO4 have been performed under magnetic fields below and above a critical field Hc at which the energy gap closes.…

We report the results of elastic and inelastic neutron scattering experiments on the Haldane gap quantum antiferromagnet Ni(C5D14N2)2N3(PF6) performed at mK temperatures in a wide range of magnetic field applied parallel to the S = 1 spin…

Inelastic neutron scattering experiments on the Haldane-gap quantum antiferromagnet NDMAP are performed in magnetic fields below and above the critical field Hc at which the gap closes. Quasi-elastic neutron scattering is found for H>Hc…

强关联电子 · 物理学 2009-11-07 A. Zheludev , Z. Honda , Y. Chen , C. L. Broholm , K. Katsumata

We investigate the magnetic field behaviour of an antiferromagnetic Heisenberg spin-1 chain with the most general single-ion anisotropy. We discuss the regime in which the magnetic field is below the transition value. The splitting of the…

凝聚态物理 · 物理学 2009-10-22 O. Golinelli , Th. Jolicoeur , R. Lacaze

Inelastic neutron scattering on deuterated single-crystal samples is used to study Haldane-gap excitations in the new S=1 one-dimensional quantum antiferromagnet NDMAP, that was recently recognized as an ideal model system for high-field…

强关联电子 · 物理学 2009-10-31 A. Zheludev , Y. Chen , C. L. Broholm , Z. Honda , K. Katsumata

Magnetic excitations in the quasi-one-dimensional antiferromagnet IPA-CuCl3 are studied by cold neutron inelastic scattering. Strongly dispersive gap excitations are observed. Contrary to previously proposed models, the system is best…

强关联电子 · 物理学 2009-11-11 T. Masuda , A. Zheludev , H. Manaka , L. -P. Regnault , J. -H. Chung , Y. Qiu

Polarized and unpolarized inelastic neutron scattering is used to study Haldane-gap excitations in the mixed-spin linear-chain antiferromagnet Nd2BaNiO5. The longitudinal mode, polarized along the direction of ordered moments, is observed…

强关联电子 · 物理学 2009-10-31 S. Raymond , T. Yokoo , A. Zheludev , S. E. Nagler , A. Wildes , J. Akimitsu

We report inelastic time-of-flight and triple-axis neutron scattering measurements of the excitation spectrum of the coupled antiferromagnetic spin-1 Heisenberg chain system CsNiCl3. Measurements over a wide range of wave-vector transfers…

强关联电子 · 物理学 2009-11-07 M. Kenzelmann , R. A. Cowley , W. J. L. Buyers , Z. Tun , R. Coldea , M. Enderle

Two quasi-1-dimensional S=1 quantum antiferromagnetic materials, PbNi2V2O8 and SrNi2V2O8, are studied by inelastic neutron scattering on powder samples. While magnetic interactions in the two systems are found to be very similar, subtle…

强关联电子 · 物理学 2009-10-31 A. Zheludev , T. Masuda , I. Tsukada , Y. Uchiyama , K. Uchinokura , P. Boni , S. -H. Lee

We report an inelastic neutron scattering study of antiferromagnetic spin dynamics in the Haldane chain compound Ni(C2H8N2)2NO2ClO4 (NENP) under external hydrostatic pressure P = 2.5 GPa. At ambient pressure, the magnetic excitations in…

凝聚态物理 · 物理学 2016-08-31 I. A. Zaliznyak , D. C. Dender , C. Broholm , Daniel H. Reich

Inelastic neutron scattering was used to probe edge states in a quantum spin liquid. The experiment was performed on finite length antiferromagnetic spin-1 chains in Y_2BaNi_{1-x}Mg_xO_5. At finite fields, there is a Zeeman resonance below…

强关联电子 · 物理学 2009-11-07 M. Kenzelmann , G. Xu , I. A. Zaliznyak , C. Broholm , J. F. DiTusa , G. Aeppli , T. Ito , K. Oka , H. Takagi

Linear-chain nickelates with the composition (Nd_x Y_{1-x})_2 Ba Ni O_5 (x=1, x=0.75, x=0.5, and x=0.25) are studied in a series of neutron scattering experiments. Powder diffraction is used to determine the temperature dependence of the…

强关联电子 · 物理学 2008-12-18 T. Yokoo , S. Raymond , A. Zheludev , S. Maslov , E. Ressouche , I. Zaliznyak , R. Erwin , M. Nakamura , J. Akimitsu

The challenge of one-dimensional systems is to understand their physics beyond the level of known elementary excitations. By high-resolution neutron spectroscopy in a quantum spin ladder material, we probe the leading multiparticle…

We performed single-crystal magnetic susceptibility and $^1$H NMR measurements on a quasi-1D, spin-1 antiferromagnet NiC$_2$O$_4$$\cdot$2NH$_3$, with temperature down to 100 mK and with field up to 26 T. With field applied along the chain…

High intensity inelastic neutron scattering experiments on the S=1 quasi-one-dimensional bond-alternating antiferromagnet Ni(C9D24N4)(NO2)ClO4 (NTENP) are performed in magnetic fields of up to 14.8~T. Excitation in the high field magnetized…

强关联电子 · 物理学 2009-11-11 L. -P. Regnault , A. Zheludev , M. Hagiwara , A. Stunault

The spin dynamics of the S=1 Ni-chains in mixed-spin antiferromagnets Pr_2 Ba Ni O_5 and Nd_x Y_2-x Ba Ni O_5 is described in terms of a simple Ginzburg-Landau Lagrangian coupled to the sublattice of rare-earth ions. Within this framework…

强关联电子 · 物理学 2009-10-30 S. Maslov , A. Zheludev

Inelastic neutron scattering experiments were performed on single crystals of the heavy-fermion compound CeIn$_{3}$ for temperatures below and above the N\'eel temperature, $T_N$. In the antiferromagnetically ordered phase, well-defined…

强关联电子 · 物理学 2009-11-10 W. Knafo , S. Raymond , B. Fak , G. Lapertot , P. C. Canfield , J. Flouquet

Neutron diffraction experiments performed on the Haldane gap material NDMAP in high magnetic fields applied at an angle to the principal anisotropy axes reveal two consecutive field-induced phase transitions. The low-field phase is the…

强关联电子 · 物理学 2009-11-10 A. Zheludev , B. Grenier , E. Ressouche , L. -P. Regnault , Z. Honda K. Katsumata

Inelastic neutron scattering is used to investigate magnetic excitations in the quasi-one-dimensional quantum spin-liquid system Cu2Cl4 D8C4SO2. Contrary to previously conjectured models that relied on bond-alternating nearest neighbor…

强关联电子 · 物理学 2007-11-14 V. O. Garlea , A. Zheludev , L. -P. Regnault , J. -H. Chung , Y. Qiu , M. Boehm , K. Habicht , M. Meissner

[Ni(HF$_2$)(3-Clpyridine)$_4$]BF$_4$ (NBCT) is a one-dimensional, $S = 1$ spin chain material that shows no magnetic neutron Bragg peaks down temperatures of 0.1 K. Previous work identified NBCT to be in the Haldane phase and near a quantum…

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