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The density profile and surface tension for the interface of phase-separated colloid-polymer mixtures have been studied in the framework of the square gradient approximation for both ideal and interacting polymers in good solvent. The…

软凝聚态物质 · 物理学 2009-11-10 A. Moncho-Jorda , B. Rotenberg , A. A. Louis

The surface tension, the adsorption, and the depletion thickness of polymers close to a single nonadsorbing colloidal sphere are computed by means of Monte Carlo simulations. We consider polymers under good-solvent conditions and in the…

软凝聚态物质 · 物理学 2014-05-06 Giuseppe D'Adamo , Andrea Pelissetto , Carlo Pierleoni

Interfacial properties of colloid--polymer mixtures are examined within an effective one--component representation, where the polymer degrees of freedom are traced out, leaving a fluid of colloidal particles interacting via polymer--induced…

软凝聚态物质 · 物理学 2007-05-23 A. Moncho-Jorda' , J. Dzubiella , J. P. Hansen , A. A. Louis

An extension of the Asakura-Oosawa-Vrij model of hard sphere colloids and non-adsorbing polymers, that takes polymer non-ideality into account through a repulsive stepfunction pair potential between polymers, is studied with grand canonical…

软凝聚态物质 · 物理学 2007-05-23 R. L. C. Vink , M. Schmidt

Colloidal systems are often modelled as fluids of hard particles (possibly with an additional soft attraction, e.g. caused by polymers also contained in the suspension). in simulations of such systems, the virial theorem cannot be…

软凝聚态物质 · 物理学 2015-05-30 Debabrata Deb , Dorothea Wilms , Alexander Winkler , Peter Virnau , Kurt Binder

The depletion interactions between two colloidal plates or between two colloidal spheres, induced by interacting polymers in a good solvent, are calculated theoretically and by computer simulations. A simple analytical theory is shown to be…

软凝聚态物质 · 物理学 2009-11-07 A. A. Louis , P. G. Bolhuis , E. J. Meijer , J. P. Hansen

The equilibrium phase behavior of a binary mixture of charged colloids and neutral, non-adsorbing polymers is studied within free-volume theory. A model mixture of charged hard-sphere macroions and ideal, coarse-grained, effective-sphere…

软凝聚态物质 · 物理学 2009-11-11 Alan R. Denton , Matthias Schmidt

We have developed a simulation model to describe particle adsorption to and desorption from liquid interfaces. Using this model we formulate a closed interfacial equation of state for repulsive elastic spheres. The effect of a long-range…

软凝聚态物质 · 物理学 2011-02-24 Robert D. Groot , Simeon D. Stoyanov

The influence of poor solvent quality on fluid demixing of a model mixture of colloids and nonadsorbing polymers is investigated using density functional theory. The colloidal particles are modelled as hard spheres and the polymer coils as…

软凝聚态物质 · 物理学 2009-11-07 Matthias Schmidt , Alan R. Denton

Solutions of semiflexible polymers confined by repulsive planar walls are studied by density functional theory and Molecular Dynamics simulations, to clarify the competition between the chain alignment favored by the wall and the depletion…

软凝聚态物质 · 物理学 2016-05-25 Sergei A. Egorov , Andrey Milchev , Peter Virnau , Kurt Binder

The possibility to induce demixing in a colloidal mixture by adding small polymers, or other equivalent depletant agents, is theoretically investigated. By use of Mean Field Theory, suitably generalized to deal with short range effective…

软凝聚态物质 · 物理学 2015-10-28 Alberto Parola , Luciano Reatto

We explore the pressure of active particles on curved surfaces and its relation to other interfacial properties. We use both direct simulations of the active systems as well as simulations of an equilibrium system with effective (pair)…

软凝聚态物质 · 物理学 2019-05-14 René Wittmann , Frank Smallenburg , Joseph M. Brader

We study the structure and interfacial properties of model athermal mixtures of colloids and excluded volume polymers. The colloid particles are modeled as hard spheres whereas the polymer coils are modeled as chains formed from…

软凝聚态物质 · 物理学 2007-05-23 Pawel Bryk

We map dilute or semi-dilute solutions of non-intersecting polymer chains onto a fluid of ``soft'' particles interacting via a concentration dependent effective pair potential, by inverting the pair distribution function of the centers of…

软凝聚态物质 · 物理学 2009-10-31 A. A. Louis , P. G. Bolhuis , J. P. Hansen , E. J. Meijer

An extended theoretical study of interface potentials in adsorbed colloid-polymer mixtures is performed. To describe the colloid-polymer mixture near a hard wall, a simple Cahn-Nakanishi-Fisher free-energy functional is used. The bulk phase…

软凝聚态物质 · 物理学 2015-06-19 Jesper Koning , Yves Vandecan , Joseph Indekeu

We consider the Asakura-Oosawa model of hard sphere colloids and ideal polymers in contact with a porous matrix modeled by immobilized configurations of hard spheres. For this ternary mixture a fundamental measure density functional theory…

软凝聚态物质 · 物理学 2009-11-10 Paul P. F. Wessels , Matthias Schmidt , Hartmut Löwen

We consider a model mixture of hard colloidal spheres and non-adsorbing polymer chains in a theta solvent. The polymer component is modelled as a polydisperse mixture of effective spheres, mutually noninteracting but excluded from the…

软凝聚态物质 · 物理学 2009-11-10 A. R. Denton , M. Schmidt

We perform a study of the interfacial properties of a model suspension of hard sphere colloids with diameter $\sigma_c$ and non-adsorbing ideal polymer coils with diameter $\sigma_p$. For the mixture in contact with a planar hard wall, we…

软凝聚态物质 · 物理学 2009-11-11 Andrea Fortini , Marjolein Dijkstra , Matthias Schmidt , Paul P. F. Wessels

We report a numerical study of equilibrium phase-diagrams and interfacial properties of bulk and confined colloid-polymer mixtures using grand canonical Monte Carlo simulations. Colloidal particles are treated as hard spheres, while the…

软凝聚态物质 · 物理学 2009-11-13 Andrea Fortini , Peter G. Bolhuis , Marjolein Dijkstra

The effective interaction between two planar walls immersed in a fluid is investigated by use of Density Functional Theory in the super-critical region of the phase diagram. A hard core Yukawa model of fluid is studied with special…

统计力学 · 物理学 2017-04-05 Pietro Anzini , Alberto Parola
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