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相关论文: Slater Transition in the Pyrochlore Cd2Os2O7

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Infrared reflectance measurements were made on the single crystal pyrochlore Cd$_{2}$Os$_{2}$O$_{7}$ in order to examine the transformations of the electronic structure and crystal lattice across the boundary of the metal insulator…

强关联电子 · 物理学 2009-11-07 W. J. Padilla , D. N. Basov , D. Mandrus

We present an angle-resolved photoemission study of the electronic structure of the three-dimensional pyrochlore iridate Nd2Ir2O7 through its magnetic metal-insulator transition. Our data reveal that metallic Nd2Ir2O7 has a quadratic band,…

Semimetallic osmium pyrochlore oxide Cd2Os2O7 undergoes a magnetic transition to an all-in-all-out (AIAO)-type order at 227 K, followed by a crossover to an AIAO insulator at around 210 K. Here, we studied the isostructural and…

强关联电子 · 物理学 2022-02-09 Kota Kataoka , Daigorou Hirai , Akihiro Koda , Ryosuke Kadono , Takashi Honda , Zenji Hiroi

Cd2Os2O7 shows a peculiar metal-insulator transition at 227 K with magnetic ordering in a frustrated pyrochlore lattice, but its magnetic structure in the ordered state and the transition origin are yet uncovered. We observed a commensurate…

Layered 5d transition metal oxides (TMOs) have attracted significant interest in recent years because of the rich physical properties induced by the interplay between spin-orbit coupling, bandwidth and on-site Coulomb repulsion. In Sr2IrO4,…

We report the observation of superconductivity in high-quality Cd$_2$Re$_2$O$_7$ single crystals with room-temperature pyrochlore structure. Resistivity and ac susceptibility measurements establish an onset transition temperature…

超导电性 · 物理学 2009-11-07 R. Jin , J. He , S. McCall , C. S. Alexander , F. Drymiotis , D. Mandrus

In CsW2O6, which undergoes a metal-insulator transition (MIT) at 213 K, the emergence of exotic properties associated with rattling motion of Cs is expected owing to its characteristic \beta-pyrochlore-type structure. However, a hurdle for…

强关联电子 · 物理学 2018-12-05 Takuto Soma , Kohei Yoshimatsu , Koji Horiba , Hiroshi Kumigashira , Akira Ohtomo

We investigate the metal-insulator transition (MIT) of the osmium pyrochlore oxide Cd2Os2O7 through transport and magnetization measurements. The MIT and a magnetic transition to the all-in/all-out (AIAO) order occur simultaneously at 227…

强关联电子 · 物理学 2015-02-03 Z. Hiroi , J. Yamaura , T. Hirose , I. Nagashima , Y. Okamoto

Metal-insulator transitions involve a mix of charge, spin, and structural degrees of freedom, and when strongly-correlated, can underlay the emergence of exotic quantum states. Mott insulators induced by the opening of a Coulomb gap are an…

强关联电子 · 物理学 2021-05-14 Yejun Feng , Yishu Wang , D. M. Silevitch , S. E. Cooper , D. Mandrus , Patrick A. Lee , T. F. Rosenbaum

Metal-to-insulator transitions (MITs), particularly near room temperature, have been extensively studied in nonmagnetic and conventional ferromagnetic and antiferromagnetic systems, yet the co-emergence of MIT and altermagnetism (AM)…

Evidence for another phase transition at 120 K in the metallic pyrochlore oxide Cd2Re2O7, following the structural transition at 200 K and followed by the superconducting transition at 1.0 K, is given through resistivity, magnetoresistance,…

强关联电子 · 物理学 2009-11-07 Zenji Hiroi , Jun-Ichi Yamaura , Yuji Muraoka , Masafumi Hanawa

Electronic properties of the metallic pyrochlore oxide Cd2Re2O7 are studied by means of electrical resistivity and Hall measurements. Semimetallic band structures are revealed as expected from band structure calculations. It is found that…

强关联电子 · 物理学 2009-11-07 Z. Hiroi , M. Hanawa , Y. Muraoka , H. Harima

We report a structural phase transition found at Ts = 200 K in a pyrochlore oxide Cd2Re2O7 which shows superconductivity at Tc = 1.0 K. X-ray diffractionexperiments indicate that the phase transition is of the second order, from a…

超导电性 · 物理学 2009-11-07 M. Hanawa , J. Yamaura , Y. Muraoka , F. Sakai , Z. Hiroi

We report on the evolution of the thermal metal-insulator transition in polycrystalline samples of Nd$_2$Ir$_2$O$_7$ upon hole-doping via substitution of Ca$^{2+}$ for Nd$^{3+}$. Ca substitution mediates a filling-controlled Mott-like…

The cubic symmetry of pyrochlore iridium oxides R2Ir2O7 (R = Nd, Eu, and Pr) has been investigated by high resolution X-ray diffraction experiments down to 4 K,in order to clarify the relationship between the metal-insulator transition…

强关联电子 · 物理学 2014-12-12 Hiroshi Takatsu , Kunihiko Watanabe , Kazuki Goto , Hiroaki Kadowaki

We report on the structural, magnetic, and electronic properties of two new double-perovskites synthesized under high pressure; Pb2CaOsO6 and Pb2ZnOsO6. Upon cooling below 80 K, Pb2CaOsO6 simultaneously undergoes a metal--insulator…

We address the concomitant metal-insulator transition (MIT) and antiferromagnetic ordering in the novel pyrochlore iridate Eu2Ir2O7 by combining x-ray absorption spectroscopy, x-ray and neutron diffractions and density functional theory…

The magnetically driven metal-insulator transition (MIT) was predicted by Slater in the fifties. Here a long-range antiferromagnetic (AF) order can open up a gap at the Brillouin electronic band boundary regardless of the Coulomb repulsion…

We present the specific heat, magnetization, optical spectroscopy measurements and the firstprinciple calculations on the Weberite structure Ca2Os2O7 single crystal/polycrystalline sample. The Ca2Os2O7 shows a Curie-Weiss nature at high…

强关联电子 · 物理学 2015-06-11 P. Zheng , Y. G. Shi , Q. S. Wu , G. Xu , T. Dong , Z. G. Chen , R. H. Yuan , B. Cheng , K. Yamaura , J. L. Luo , N. L. Wang

We report on the muon spin rotation/relaxation study of a pyrochlore oxide, Cd2Os2O7, which exhibits a metal-insulator (MI) transition at T_{MI}~225 K without structural phase transition. It reveals strong spin fluctuation (>10^8/s) below…

强关联电子 · 物理学 2009-11-13 A. Koda , R. Kadono , K. Ohishi , S. R. Saha , W. Higemoto , S. Yonezawa , Y. Muraoka , Z. Hiroi
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