相关论文: Strongly Correlated Cerium Systems: Non-Kondo Mech…
The nature of the elemental cerium phases, undergoing an isostructural volume collapse transition, cannot be understood using conventional solid state concepts. Using the combination of density functional theory and dynamical mean-field…
A review is given of the experimental situation and theoretical predictions concerning unconventional magnetic ordering in dense Kondo 4f- and 5f-systems, including recently investigated on cerium, ytterbium, and actinide based ternary…
Cerium-based intermetallics are currently attracting much interest as a possible alternative to existing high-performance magnets containing scarce heavy rare-earth elements. However, the intrinsic magnetic properties of Ce in these systems…
Spectra of x-ray absorption and magnetic circular dichroism were measured at M4,5(3d) and L2,3(2p) edges of Ce in multilayers [Ce(1-x)Six/Fe]xn, with x between 0.1 and 0.65. The study uncovers the highly correlated nature of this layered…
The cerium iso-structural phase transition (gamma to alpha) is dominated by f-electron localization changes that results in a magnetic ordering change and a volume collapse. Generally, these physics are difficult to capture with ab initio…
Heavy fermion systems represent one of the paradigmatic strongly correlated states of matter. They have been used as a platform for investigating exotic behavior ranging from quantum criticality and non-Fermi liquid behavior to…
Microscopic models for heavy-fermion materials often assume a local, i.e., momentum-independent, hybridization between the conduction band and the local-moment f electrons. Motivated by recent experiments, we consider situations where this…
We investigated the electronic structure of the enigmatic CeRh$_3$B$_2$ using resonant inelastic scattering and x-ray absorption spectroscopy in combination with $ab$ $initio$ density functional calculations. We find that the Rh 4$d$ states…
Cerium, in which the 4$f$ valence electrons live at the brink between localized and itinerant characters, exhibits varying crystal structures and therefore anomalous physical properties with respect to temperature and pressure.…
CeSiI has been recently isolated in the ultrathin limit, establishing CeSiI as the first intrinsic two-dimensional van der Waals heavy-fermion material up to 85 K. We show that, due to the strong Ce spin-orbit coupling, the local moments…
Ultrafast optical spectroscopy was used to investigate the ultrafast quasiparticle dynamics of antiferromagnetic Kondo lattice CeAuSb$_2$ as a function of temperature and fluence. Our results reveal (i) the opening of a narrow hybridization…
Heavy fermions represent an archetypal example of strongly correlated electron systems which, due to entanglement among different interactions, often exhibit exotic and fascinating physics involving Kondo screening, magnetism and…
We use x-ray absorption and magnetic circular dichroism to study electronic configuration and local susceptibility of CePt5/Pt(111) surface alloys from well above to well below the impurity Kondo temperature. The anisotropic paramagnetic…
We consider electronic correlation effects and their impact on magnetic properties of tetragonally distorted chemically ordered FeCo alloys (L1$_0$ structure) being a promising candidate for rare-earth-free permanent magnets. We employ a…
The unusual and interesting physical properties of rare earth intemetallic compounds have their origin in the combination of strongly correlated 4f states and their hybridization with the conduction electron sea, which gives rise to their…
The "melting" of self-formed rigid structures made of a small number of interacting classical particles confined in an irregular two-dimensional space is investigated using Monte Carlo simulations. It is shown that the interplay of…
Accurate calculations of strongly correlated materials remain a formidable challenge in condensed matter physics, particularly due to the computational demand of conventional methods. This paper presents an efficient solver for dynamical…
The cerium alpha-gamma phase transition is characterized by means of a many-body Jastrow-correlated wave function, which minimizes the variational energy of the first-principles scalar-relativistic Hamiltonian, and includes correlation…
We report a study of the La$_{1-x}$Ce$_x$FeSiH solid solution ($0 \leq x \leq 1$), a family of intermetallic hydrides of ZrCuSiAs-type structure, with space group $P4/nmm$. For low cerium concentrations $x \leq 0.20$, we observe the…
There are two views of antiferromagnets. The first proceeds from atomic physics, which predicts that atoms with unpaired electrons develop magnetic moments. In a solid, the coupling between moments on nearby ions then yields…