相关论文: A delay-programmable two-color femtosecond source …
We present an integrated source of polarization entangled photon pairs in the telecom regime, which is based on type II-phasematched parametric down-conversion (PDC) in a Ti-indiffused waveguide in periodically poled lithium niobate. The…
We discuss techniques that allow for long coherence times in laser spectroscopy experiments with two trapped ions. We show that for this purpose not only entangled ions prepared in decoherence-free subspaces can be used but also a pair of…
Single-photon sources with near-unity efficiency and indistinguishability play a major role in the development of quantum technologies. However, on-demand excitation of the emitter imposes substantial limitations to the source performance.…
We combine different wavelengths from an intense high-order harmonics source with variable delay at the focus of a split-mirror interferometer to conduct pump-probe experiments on gas-phase molecules. We report measurements of the time…
We describe two noncollinear optical parametric amplifier (NOPA) systems pumped by either the second (515 nm) or the third (343 nm) harmonic of an Yb:KGW amplifier, respectively. Pulse durations as short as 6.8 fs are readily obtained by…
Delayed cavity-free forward lasing at the wavelengths of 391 and 428 nm was observed in recent experiments in air or pure nitrogen pumped with an intense femtosecond laser pulse at wavelength of 800~nm. The mechanism responsible for the…
Second-harmonic generation allows for coherently bridging distant regions of the optical spectrum, with applications ranging from laser technology to self-referencing of frequency combs. However, accessing the nonlinear response of a medium…
We introduce an ultrafast, bright, entangled twin-beam source generated by type-0 parametric down-conversion in periodically-poled lithium niobate at MHz repetition rate, with continuously tunable Schmidt number $K$ set by the pump pulse…
Quantum entanglement of two photons created by spontaneous parametric downconversion (SPDC) can be used to probe quantum optical phenomena during a single cycle of light. Harris [Phys. Rev. Lett. 98, 063602 (2007)] suggested using…
This study theoretically investigates the angular distribution of core-level photoemission time delay within a molecular frame. This phenomenon can be measured with the advancement of attosecond pulsed lasers and metrology. Our focus is on…
Sources of quantum light, in particular correlated photon pairs that are indistinguishable in all degrees of freedom, are the fundamental resource that enables continuous-variable quantum computation and paradigms such as Gaussian boson…
A new double time-of-flight (dTOF) neutron spectroscopy technique has been developed for pulsed broad spectrum sources with a duty cycle that results in frame overlap, where fast neutrons from a given pulse overtake slower neutrons from…
Measured photoionization time delays may exhibit large variations as a function of the emission angles, even for spherically symmetric targets, as shown in recent RABBITT (reconstruction of attosecond beating by interference of two-photon…
We extend the powerful frequency-domain analysis of femtosecond two-photon absorption to the intermediate-field regime, which involves both two- and four-photon transitions. Consequently, we find a broad family of shaped pulses that enhance…
Photo-doped states in strongly correlated charge transfer insulators are characterized by $d$-$d$ and $d$-$p$ interactions and the resulting intertwined dynamics of charge excitations and local multiplets. Here we use femtosecond x-ray…
We demonstrate the generation of degenerate photon pairs from spontaneous parametric down-conversion in titanium in-diffused waveguides in lithium niobate at cryogenic temperatures. Since the phase-matching cannot be temperature tuned…
We theoretically prove a multifunctional photonic differentiation (DIFF) scheme based on phase demodulation using two cascaded linear filters. The photonic DIFF has a diversity of output forms, such as 1st order intensity DIFF, 1st order…
The switching and control of optical fields based on nonlinear optical effects are often limited to relatively weak nonlinear susceptibility and strong optical pump fields. Here, an optical medium with programmable susceptibility tensor…
Second-order nonlinear optical interactions, including second harmonic generation (SHG) and sum-frequency generation (SFG), can reveal a wealth of information about chemical, electronic, and vibrational dynamics at the nanoscale. Here, we…
Improving the efficiency of photothermal (PT) therapies and photoacoustic (PA) imaging at the microscopic scale hinges on developing multiphoton-absorbing photothermal molecules or contrast agents that operate in the near-infrared (NIR)…