相关论文: Control of relaxation properties of a macroscopic …
Motivated by a recent proposal by O. P. Sushkov and co-workers to search for a P,T-violating Schiff moment of the $^{207}$Pb nucleus in a ferroelectric solid, we have carried out a high-field nuclear magnetic resonance study of the…
The unique combination of outstanding optical quality and attractive spin properties opens new avenues for optical spin control in hybrid organic-inorganic perovskite semiconductors. Using the optically detected magnetic resonance…
Perovskite nanocrystals are a convenient model system for optical spin orientation and manipulation. However, its real potential might be underestimated due to the incomplete knowledge on spin relaxation times, which are obscured by the…
The magnetic interactions between the spin of an unpaired electron and the surrounding nuclear spins can be exploited to gain structural information, to reduce nuclear relaxation times as well as to create nuclear hyperpolarization via…
The nuclear spin-lattice relaxation time ($T_1$) of lanthanum and aluminum nuclei in a single crystal of lanthanum aluminate doped with neodymium ions is studied to estimate the feasibility of the dynamically polarized lanthanum target…
Nuclear spins in certain solids couple weakly to their environment, making them attractive candidates for quantum information processing and inertial sensing. When coupled to the spin of an optically-active electron, nuclear spins can be…
Spin-lattice relaxation of the nuclear spin system in p-type GaAs is studied using a three-stage experimental protocol including optical pumping and measuring the difference of the nuclear spin polarization before and after a dark interval…
Long spin coherence times of carriers are essential for implementing quantum technologies using semiconductor devices for which, however, a possible obstacle is spin relaxation. For the spin dynamics, decisive features are the band…
The negatively charged boron vacancy $V_B^-$ defect in hexagonal boron nitride (hBN) has recently emerged as a promising spin qubit for sensing due to its high-temperature spin control and versatile integration into van der Waals…
A theoretical interpretation is given to recent proton spin relaxation-time (T_1) measurements on NiCu(C_7H_6N_2O_6)(H_2O)_3$\cdot$2H_2O, which is an ideal one-dimensional ferrimagnetic Heisenberg model system of alternating spins 1 and…
A room temperature nuclear magnetic resonance force microscope (MRFM), fitted in a $^1$Tesla electromagnet, is used to measure the nuclear spin relaxation of $^1$H in a micron-size (70ng) crystal of ammonium sulfate. NMR sequences,…
Coherent control of quantum systems has far-reaching implications in quantum engineering. In this context, coherent population trapping (CPT) involving dark resonances has played a prominent role, leading to a wealth of major applications…
Optically active defects in solids with accessible spin states are promising candidates for solid state quantum information and sensing applications. To employ these defects as quantum building blocks, coherent manipulation of their spin…
We present a joint experimental and theoretical study of spin coherence properties of 39K, 85Rb, 87Rb, and 133Cs atoms trapped in a solid parahydrogen matrix. We use optical pumping to prepare the spin states of the implanted atoms and…
Experimental investigation of nuclear spin effects on the electron spin polarization in singly negatively charged InP quantum dots is reported. Pump-probe photoluminescence measurements of electron spin relaxation in the microsecond…
The inhomogeneity of an electron spin ensemble as well as fluctuating environment acting upon individual spins drastically shorten the spin coherence time $T_2$ and hinder coherent spin manipulation. We show that this problem can be solved…
We investigate the electron and nuclear spin coherence properties of ytterbium ($\mathrm{Yb}^{3+}$) ions with non-zero nuclear spin, within an yttrium orthosilicate (Y$_2$SiO$_5$) crystal, with a view to their potential application in…
In response to recent proton spin relaxation-time measurements on NiCu(pba)(H$_2$O)$_3$$\cdot$2H$_2$O with ${pba}=1,3{-propylenebis(oxamato)}$, which is an excellent one-dimensional ferrimagnetic Heisenberg model system of spin-$(1,{1/2})$,…
The nitrogen-vacancy (NV) center is an emerging platform for constructing inertial sensors. Its native nitrogen spin can serve as a gyroscope using Ramsey interferometry protocols. The sensitivities of these nuclear-spin-based NV gyroscopes…
We demonstrate a wide-band all-optical method of nanoscale magnetic resonance (MR) spectroscopy under ambient conditions. Our method relies on cross-relaxation between a probe spin, the electronic spin of a nitrogen-vacancy centre in…