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Based on density functional theory band structure calculations, quantum Monte-Carlo simulations, and high-field magnetization measurements, we address the microscopic magnetic model of BaAg2Cu[VO4]2 that was recently proposed as a spin-1/2…

材料科学 · 物理学 2012-06-19 Alexander A. Tsirlin , Angela Moeller , B. Lorenz , Yu. Skourski , H. Rosner

We present single-crystal growth and magnetic property studies of tellurium-bridged copper spin-1/2 system Ba$_2$CuTeO$_6$. The spin-exchange interaction among copper spins via Cu-O-Te-O-Cu super-superexchange route leads to a novel two-leg…

Inelastic neutron scattering measurements have been performed to investigate the spin waves of the quasi-one-dimensional antiferromagnetic ladder compound BaFe$_2$S$_3$, where a superconducting transition was observed under pressure [H.…

Low-dimensional quantum magnets are a versatile materials platform for studying the emergent many-body physics and collective excitations that can arise even in systems with only short-range interactions. Understanding their low-temperature…

We report inelastic neutron scattering measurements of the magnetic excitations in Ba2CuTeO6, proposed by ab initio calculations to magnetically realize weakly coupled antiferromagnetic two-leg spin-1/2 ladders. Isolated ladders are…

A comprehensive theoretical and experimental study is presented of the magnetic susceptibility versus temperature \chi(T) of spin S = 1/2 two- and three-leg Heisenberg ladders and ladder oxide compounds. Extensive quantum Monte Carlo…

Using ab initio wave-function-based calculations, we provide valuable insights with regard to the magnetic exchange in 5$d$ and 4$d$ oxides with face-sharing ligand octahedra, BaIrO$_3$ and BaRhO$_3$. Surprisingly strong antiferromagnetic…

强关联电子 · 物理学 2019-03-18 Lei Xu , Ravi Yadav , Viktor Yushankhai , Liudmila Siurakshina , Jeroen van den Brink , Liviu Hozoi

We derive and investigate the microscopic model of the quantum magnet BiCu2PO6 using band structure calculations, magnetic susceptibility and high-field magnetization measurements, as well as ED and DMRG techniques. The resulting…

We report single crystal growth and magnetic susceptibility and neutron diffraction studies of the S=1/2 quasi-1D antiferromagnet CaCu2O3. The structure of this material is similar to that of the prototype two-leg spin-ladder compound…

凝聚态物理 · 物理学 2009-10-31 V. Kiryukhin , Y. J. Kim , K. J. Thomas , F. C. Chow , R. W. Erwin , Q. Huang , M. A. Kastner , R. J. Birgeneau

We study the magnetic, structural, and electronic properties of the recently discovered iron- based superconductor BaFe2S3 based on density functional theory with the generalized gradient approximation. The calculations show that the…

强关联电子 · 物理学 2015-08-19 Michi-To Suzuki , Ryotaro Arita , Hiroaki Ikeda

We study a frustrated two-leg spin ladder with alternate isotropic Heisenberg and Ising rung exchange interactions, whereas, interactions along legs and diagonals are Ising-type. All the interactions in the ladder are anti-ferromagnetic in…

强关联电子 · 物理学 2020-11-25 Sk Saniur Rahaman , Shaon Sahoo , Manoranjan Kumar

The $S=1/2$ Heisenberg antiferromagnet in the ladder geometry is studied as a model for the spin degrees of freedom of SrCu$_2$O$_3$. The susceptibility and the spin echo decay rate are calculated using a quantum Monte Carlo technique, and…

凝聚态物理 · 物理学 2009-10-28 A. W. Sandvik , E. Dagotto , D. J. Scalapino

The magnetic properties of polycrystalline samples of Ba3Cu3In4O12 (In-334) and Ba3Cu3Sc4O12 (Sc-334) are reported. Both 334 phases have a structure derived from perovskite, with CuO4 squares interconnected to form half-twist ladders along…

强关联电子 · 物理学 2012-03-28 S. E. Dutton , M. Kumar , Z. G. Soos , C. L. Broholm , R. J. Cava

In this paper we demonstrate the application of high magnetic fields to study the magnetic properties of low dimensional spin systems. We present a case study on the series of 2-leg spin-ladder compounds…

The magnetic anisotropy af a rectangular Cu-O-Cu bond is investigated in second order of the spin-orbit interaction. Such a bond is characteristic for cuprates having edge sharing CuO_2 chains, and exists also in the Cu_3O_4 plane or in…

强关联电子 · 物理学 2009-10-31 V. Yu. Yushankhai , R. Hayn

We report long-range ordered antiferromagnetism concomitant with local iron displacements in the spin-ladder compound BaFe$_2$Se$_3$. Short-range magnetic correlations, present at room temperature, develop into long-range antiferromagnetic…

超导电性 · 物理学 2012-05-17 J. M. Caron , J. R. Neilson , D. C. Miller , A. Llobet , T. M. McQueen

In conventional quasi-one-dimensional antiferromagnets with quantum spins, magnetic excitations are carried by either magnons or spinons in different energy regimes: they do not coexist independently, nor could they interact with each…

We report on the microscopic model of the recently synthesized one-dimensional quantum magnet (NO)Cu(NO3)3. Applying density functional theory band structure calculations, we obtain a leading antiferromagnetic exchange coupling J ~ 200 K,…

强关联电子 · 物理学 2010-11-15 O. Janson , A. A. Tsirlin , H. Rosner

We study the effect of inter-ladder ferromagnetic (FM) coupling in spin-1/2 two-leg ladders with antiferromagnetic (AFM) legs and rungs interactions using the stochastic series expansion quantum Monte Carlo. We have compared the results…

强关联电子 · 物理学 2015-06-23 J. Jahangiri , H. Hadipour , S. Mahdavifar , S. Farjami

The magnetic phase diagram and the thermodynamic properties of a square lattice containing antiferromagnetically coupled spin-1/2 triangles are studied. A Heisenberg Hamiltonian with three strong intra-triangle exchange coupling constants…

强关联电子 · 物理学 2009-10-31 Stefan Wessel , Stephan Haas
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