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Excited-state methods within the nuclear--electronic orbital (NEO) framework have the potential to capture vibrational, electronic, and vibronic transitions in a single calculation. In the NEO approach, specified nuclei, typically protons,…

化学物理 · 物理学 2026-03-16 Jonathan H. Fetherolf , Fabijan Pavošević , Sharon Hammes-Schiffer

The nuclear spins in nanostructured semiconductors play a central role in quantum applications. The nuclear spins represent a useful resource for generating local magnetic fields but nuclear spin noise represents a major source of dephasing…

Quantum Information processing by NMR with small number of qubits is well established. Scaling to higher number of qubits is hindered by two major requirements (i) mutual coupling among qubits and (ii) qubit addressability. It has been…

量子物理 · 物理学 2009-11-10 Ranabir Das , Rangeet Bhattacharyya , Anil Kumar

Magnetic excitations are important quantum phenomena in magnetic systems and have been widely studied in individual magnetic atoms and molecules as well as their assembled structures over the past few decades. Using scanning tunneling…

A promising platform for quantum information processing is that of silicon impurities, where the quantum states are manipulated by magnetic resonance. Such systems, in abstraction, can be considered as a nucleus of arbitrary spin coupled to…

量子物理 · 物理学 2013-05-07 M. H. Mohammady

The use of spin echoes to refocus one spin interactions (chemical shifts) and two spin interactions (spin-spin couplings) plays a central role in both conventional NMR experiments and NMR quantum computation. Here we describe schemes for…

量子物理 · 物理学 2009-10-31 J. A. Jones , E. Knill

Pairing correlation of Cooper pair is a fundamental property of multi-fermion interacting systems. For nucleons, two modes of the Cooper-pair coupling may exist, namely of $S_{12}=0$ with $L_{12}=0$ (spin-singlet s-wave) and $S_{12}=1$ with…

核理论 · 物理学 2021-05-18 Tomohiro Oishi , Goran Kruzic , Nils Paar

A theoretical spin-based scheme for performing a variety of quantum computations is presented. It makes use of an array of multiple identical computer vectors of phosphorus-doped silicon where the nuclei serve as logical qubits and the…

量子物理 · 物理学 2013-02-08 Aharon Blank

In a closed quantum system of N coupled spins with magnetic quantum number I, there are about (2I + 1)^N constants of motion. However, the possibility of observing such quasi-invariant (QI) states in solid-like spin systems in Nuclear…

原子与分子团簇 · 物理学 2015-06-15 C. J. Bonin , C. E. González , H. H. Segnorile , R. C. Zamar

We present a NMR pulse double-irradiation method which allows one to separate magnetic from quadrupolar contributions in the spin-lattice relaxation. The pulse sequence fully saturates one transition while another is observed. In the…

材料科学 · 物理学 2009-10-31 A. Suter , M. Mali , J. Ross , D. Brinkmann

Nuclear magnetic resonance (NMR) provides an experimental setting to explore physical implementations of quantum information processing (QIP). Here we introduce the basic background for understanding applications of NMR to QIP and explain…

This paper is devoted to the multiple-quantum (MQ) NMR spectroscopy in nanopores filled by a gas of spin-carrying molecules (s=1/2) in a strong external magnetic field. It turned out that the high symmetry of the spin system in nanopores…

化学物理 · 物理学 2019-03-27 Sergei I. Doronin , Anna V. Fedorova , Edward B. Fel'dman , Alexander I. Zenchuk

We propose a new approach to the measurement of a single spin state, based on nuclear magnetic resonance (NMR) techniques and inspired by the coherent control over many-body systems envisaged by Quantum Information Processing (QIP). A…

Pursuing fractionalized particles that do not bear properties of conventional measurable objects, exemplified by bare particles in the vacuum such as electrons and elementary excitations such as magnons, is a challenge in physics. Here we…

强关联电子 · 物理学 2021-08-17 Yusuke Nomura , Masatoshi Imada

Coherent oscillations between any two levels from four nuclear spin states of I=3/2 have been demonstrated in a nanometre-scale NMR semiconductor device, where nuclear spins are all-electrically controlled. Using this device, we discuss…

量子物理 · 物理学 2009-08-04 S. K. Ozdemir , A. Miranowicz , T. Ota , G. Yusa , N. Imoto , Y. Hirayama

Multiple quantum (MQ) NMR methods \cite{Baum} are applied to the analysis of various problems of quantum information processing. It is shown that the two-spin/two-quantum Hamiltonian \cite{Baum} describing MQ NMR dynamics is related to the…

量子物理 · 物理学 2017-01-16 G. A. Bochkin , S. I. Doronin , S. G. Vasil'ev , A. V. Fedorova , E. B. Fel'dman

Physical implementation of Quantum Information Processing (QIP) by liquid-state Nuclear Magnetic Resonance (NMR), using weakly coupled spin-1/2 nuclei of a molecule, is well established. Nuclei with spin$>$1/2 oriented in liquid crystalline…

量子物理 · 物理学 2009-11-10 Ranabir Das , Anil Kumar

Zero-field nuclear magnetic resonance (NMR) provides complementary analysis modalities to those of high-field NMR and allows for ultra-high-resolution spectroscopy and measurement of untruncated spin-spin interactions. Unlike for the…

量子物理 · 物理学 2022-03-01 Min Jiang , Teng Wu , John W. Blanchard , Guanru Feng , Xinhua Peng , Dmitry Budker

The hyperpolarisation of nuclear spins within target molecules is a critical and complex challenge in magnetic resonance imaging (MRI) and nuclear magnetic resonance (NMR) spectroscopy. Hyperpolarisation offers enormous gains in signal and…

We study the symmetric nuclear matter using bare nucleon-nucleon ($NN$) interactions with finite particle-number approach within finite cubic boxes. Due to the $NN$ correlations originating from bare $NN$ interaction, two nucleons can be…