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Phase separation of multicomponent liquid mixtures plays an integral part in many processes ranging from industry to cellular biology. In many cases the morphology of coexisting phases is crucially linked to the function of the separated…

软凝聚态物质 · 物理学 2020-11-25 Sheng Mao , Milena S. Chakraverti-Wuerthwein , Hunter Gaudio , Andrej Kosmrlj

This paper investigates a Cahn-Hilliard-Swift-Hohenberg system, focusing on a three-species chemical mixture subject to physical constraints on volume fractions. The resulting system leads to complex patterns involving a separation into…

偏微分方程分析 · 数学 2024-10-02 Harald Garcke , Kei Fong Lam , Robert Nürnberg , Andrea Signori

Atomically thin 2-dimensional heterostructures are a promising, novel class of materials with groundbreaking properties. The possiblity of choosing the many constituent components and their proportions allows optimizing these materials to…

介观与纳米尺度物理 · 物理学 2019-10-23 Petri Hirvonen , Vili Heinonen , Haikuan Dong , Zheyong Fan , Ken R. Elder , Tapio Ala-Nissila

We investigate binary mixtures undergoing phase separation after a second (deeper) temperature quench into two- and three-phase coexistence regions. The analysis is based on a lattice theory previously developed for gas-liquid separation in…

软凝聚态物质 · 物理学 2019-11-22 Pablo de Castro , Peter Sollich

We report a study of the phase behavior of multiple-occupancy crystals through simulation. We argue that in order to reproduce the equilibrium behavior of such crystals it is essential to treat the number of lattice sites as a constraining…

软凝聚态物质 · 物理学 2009-11-13 Bianca M. Mladek , Patrick Charbonneau , Daan Frenkel

Fluid polyamorphism, the existence of multiple amorphous fluid states in a single-component system, has been observed or predicted in a variety of substances. A remarkable example of this phenomenon is the fluid-fluid phase transition in…

软凝聚态物质 · 物理学 2022-09-21 Nathaniel R. Fried , Thomas J. Longo , Mikhail A. Anisimov

An existence result is proved for a nonlinear diffusion problem of phase-field type, consisting of a parabolic system of two partial differential equations, complemented by Neumann homogeneous boundary conditions and initial conditions.…

偏微分方程分析 · 数学 2012-02-24 Pierluigi Colli , Gianni Gilardi , Paolo Podio-Guidugli , Jürgen Sprekels

Studies of multiphase fluids utilizing the lattice Boltzmann method (LBM) are typically severely restricted by the number of components or chemical species being modeled. This restriction is particularly pronounced for multiphase systems…

流体动力学 · 物理学 2023-06-21 Muzammil Soomro , Luis F. Ayala

We review various methods to investigate the statics and the dynamics of collective composition fluctuations in dense polymer mixtures within fluctuating-field approaches. The central idea of fluctuating-field theories is to rewrite the…

软凝聚态物质 · 物理学 2007-05-23 Marcus Mueller , Friederike Schmid

Modern materials are often synthesized or operated in complex chemical environments, where there can be numerous elemental species, competing phases, and reaction pathways. When analyzing reactions using the Gibbs free energy, which has a…

材料科学 · 物理学 2024-04-10 Jiadong Chen , Matthew J. Powell-Palm , Wenhao Sun

A ring polymer in a confining space may exhibit at least two phases, namely an expanded (or solvent-rich phase) if its concentration is small, or a collapsed (or polymer-rich phase) when it is concentrated and compressed. These phases are…

软凝聚态物质 · 物理学 2026-03-24 EJ Janse van Rensburg , E Orlandini , MC Tesi

Lattice models parameterized using first-principles calculations constitute an effective framework to simulate the thermodynamic behavior of physical systems. The cluster expansion method is a flexible lattice-based method used extensively…

材料科学 · 物理学 2023-01-09 Luis Barroso-Luque , Gerbrand Ceder

We present a new multiphase-field theory for describing pattern formation in multi-domain and/or multi-component systems. The construction of the free energy functional and the dynamic equations is based on criteria that ensure mathematical…

材料科学 · 物理学 2015-12-09 Gyula I. Toth , Tamas Pusztai , Laszlo Granasy

We introduce hybrid fractals as a class of fractals constructed by gluing several fractal pieces in a specific manner and study energy forms and Laplacians on them. We consider in particular a hybrid based on the $3$-level Sierpinski…

泛函分析 · 数学 2018-04-17 Patricia Alonso Ruiz , Yuming Chen , Haotian Gu , Robert S. Strichartz , Zirui Zhou

Agglomeration, adsorption, and extraction in dispersed multiphase systems are ubiquitously encountered in biological systems, energy industry, and medical science. In this work, a novel lattice model is extended to the three-component…

统计力学 · 物理学 2022-10-12 Yiran Li , Yunfan Huang , Xukang Lu , Moran Wang

The heavy quark expansion of Quantum Chromodynamics and the strong coupling flux tube picture of nonperturbative glue are employed to develop the phenomenology of hybrid meson decays. The decay mechanism explicitly couples gluonic degrees…

高能物理 - 唯象学 · 物理学 2016-09-06 Eric S. Swanson , Adam P. Szczepaniak

We propose the quantitative mean-field theory of mechanical unfolding of a globule formed by long flexible homopolymer chain collapsed in poor solvent and subjected to extensional deformation. We demonstrate that depending on the degree of…

软凝聚态物质 · 物理学 2012-05-15 Alexey A. Polotsky , Mohamed Daoud , Oleg Borisov , Tatiana M. Birshtein

The phase field fracture method has emerged as a promising computational tool for modelling a variety of problems including, since recently, hydrogen embrittlement and stress corrosion cracking. In this work, we demonstrate the potential of…

应用物理 · 物理学 2020-11-17 P. K. Kristensen , C. F. Niordson , E. Martínez-Pañeda

We study analytically a continuum model for phase-separation in binary polymer blends based on the Flory-Huggins-De Gennes free energy, by means of the self-consistent large-$n$ limit approach. The model is solved for values of the…

统计力学 · 物理学 2009-10-30 Claudio Castellano , Federico Corberi

We developed a general framework for simulating multicomponent and multiphase systems using the lattice Boltzmann framework. Despite the fact that there is no restriction on the number of components in principle, in this article we focus an…

软凝聚态物质 · 物理学 2018-10-24 Kent S. Ridl , Alexander J. Wagner