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Synchronisation is a collective phenomenon widely investigated in classical oscillators and, more recently, in quantum systems. However, it remains unclear what features distinguish synchronous behaviour in these two scenarios. Recent works…

量子物理 · 物理学 2019-07-19 Stefan Siwiak-Jaszek , Alexandra Olaya-Castro

During the long course of evolution, nature has learnt how to exploit quantum effects. In fact, recent experiments reveal the existence of quantum processes whose coherence extends over unexpectedly long time and space ranges. In…

量子物理 · 物理学 2015-07-14 G. L. Giorgi , M. Roncaglia , F. A. Raffa , M. Genovese

Recently the quantum nature in the energy transport in solar cell and light-harvesting complexes have attracted much attention, as being triggered by the experimental observations. We model the light-harvesting complex (i.e., PEB50 dimer)…

化学物理 · 物理学 2015-03-05 Zhedong Zhang , Jin Wang

The theoretical and experimental study of energy transfer in photosynthesis has revealed an interesting transport regime, which lies at the borderline between classical transport dynamics and quantum-mechanical interference effects.…

生物物理 · 物理学 2014-02-13 Tobias Kramer , Christoph Kreisbeck

Spontaneous synchronisation is a collective phenomenon that can occur in both dynamical classical and quantum systems. Here, we analyse the spontaneous synchronisation dynamics of vibrations assisting energy transfer in a bio-inspired…

量子物理 · 物理学 2020-09-30 Stefan Siwiak-Jaszek , Thao P. Le , Alexandra Olaya-Castro

The interplay between coherence and system-environment interactions is at the basis of a wide range of phenomena, from quantum information processing to charge and energy transfer in molecular systems, biomolecules, and photochemical…

量子物理 · 物理学 2025-11-30 Diego Fallas Padilla , Visal So , Abhishek Menon , Roman Zhuravel , Han Pu , Guido Pagano

The rate of energy transfer in donor-acceptor systems can be manipulated via the common interaction with the confined electromagnetic modes of a micro-cavity. We analyze the competition between the near-field short range dipole-dipole…

量子物理 · 物理学 2018-07-27 Michael Reitz , Francesca Mineo , Claudiu Genes

Synchronization is a widespread phenomenon encountered in many natural and engineered systems with nonlinear classical dynamics. How synchronization concepts and mechanisms transfer to the quantum realm and whether features are universal or…

介观与纳米尺度物理 · 物理学 2024-11-12 Florian Höhe , Lukas Danner , Ciprian Padurariu , Brecht I. C Donvil , Joachim Ankerhold , Björn Kubala

Understanding how the effectiveness of natural photosynthetic energy harvesting systems arises from the interplay between quantum coherence and environmental noise represents a significant challenge for quantum theory. Recently it has begun…

生物物理 · 物理学 2015-06-16 E. K. Irish , R. Gómez-Bombarelli , B. W. Lovett

In a network of interacting quantum systems achieving fast coherent energy transfer is a challenging task. While quantum systems are susceptible to a wide range of environmental factors, in many physical settings their interactions with…

量子物理 · 物理学 2014-05-09 James Lim , Mark Tame , Ki Hyuk Yee , Joong-Sung Lee , Jinhyoung Lee

Light-harvesting via the transport and trapping of optically-induced electronic excitations is of fundamental interest to the design of new energy efficient quantum technologies. Using a paradigmatic quantum optical model, we study the…

量子物理 · 物理学 2024-08-08 Jonah S. Peter , Raphael Holzinger , Stefan Ostermann , Susanne F. Yelin

The non-hermitian quantum dynamics of excitonic energy transfer in photosynthetic systems is investigated using a dissipative two-level dimer model. The approach is based on the Green's function formalism which permits consideration of…

量子物理 · 物理学 2012-04-03 A. Thilagam

We present a theory that efficiently describes the quantum dynamics of an electronic excitation that is coupled to a continuous, highly structured phonon environment. Based on a stochastic approach to non-Markovian open quantum systems, we…

量子物理 · 物理学 2009-11-05 Jan Roden , Alexander Eisfeld , Wolfgang Wolff , Walter T. Strunz

The influence of fast vibrations on energy transfer and conversion in natural molecular aggregates is an issue of central interest. This article shows the important role of high-energy quantized vibrations and their non-equilibrium dynamics…

生物物理 · 物理学 2013-01-30 Avinash Kolli , Edward J. O'Reilly , Gregory D. Scholes , Alexandra Olaya-Castro

Recent evidence suggests that quantum effects may have functional importance in biological light-harvesting systems. Along with delocalized electronic excitations, it is now suspected that quantum coherent interactions with certain…

化学物理 · 物理学 2015-10-22 Nathan Killoran , Susana F. Huelga , Martin B. Plenio

Quantum simulation offers a route to study open-system molecular dynamics in non-perturbative regimes by programming the interactions among electronic, vibrational, and environmental degrees of freedom on similar energy scales. Trapped-ion…

The time-development of photoexcitations in molecular aggregates exhibits specific dynamics of electronic states and vibrational wavefunction. We discuss the dynamical formation of entanglement between electronic and vibrational degrees of…

量子物理 · 物理学 2007-05-23 Dmitri S. Kilin , Jeffrey A. Cina , Oleg V. Prezhdo

In this paper, we study the synchronization of qubits induced by the dynamical Casimir effect in an atom-cavity quantum electrodynamics system. Our investigation revolves around a pragmatic configuration of a quantum system, where two…

量子物理 · 物理学 2024-11-25 Haruki Mitarai , Yoshihiko Hasegawa

Recent ultrafast optical experiments show that excitons in large biological light-harvesting complexes are coupled to molecular vibration modes. These high-frequency vibrations will not only affect the optical response, but also drive the…

量子物理 · 物理学 2015-02-12 Arend G. Dijkstra , Chen Wang , Jianshu Cao , Graham R. Fleming

Macroscopic ensembles of radiating dipoles are ubiquitous in the physical and natural sciences. In the classical limit the dipoles can be described as damped-driven oscillators, which are able to spontaneously synchronize and collectively…

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