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Nb$_3$Cl$_8$, a cluster Mott insulator with a distinctive magnetic molecular orbital structure organized into a breathing kagome lattice, showcases critical phase transitions under specialized conditions. By transitioning from paramagnetic…

材料科学 · 物理学 2024-09-10 Yuya Haraguchi , Kazuyoshi Yoshimura

Flat electronic bands strongly enhance Coulomb interactions and can stabilize unconventional insulating states. Motivated by the recent discovery of flat bands in breathing Kagome lattices, we use first-principles GW--Bethe--Salpeter theory…

The kagome lattice provides a playground to explore novel correlated quantum states due to the presence of flat bands in its electronic structure. Recently discovered layered kagome compound Nb3Cl8 has been proposed as a Mott insulator…

State-of-the-art photon sources based on spontaneous parametric down-conversion (SPDC) currently rely on artificial structuring of the material nonlinearity to satisfy phase-matching conditions. This technique, known as periodic poling, is…

光学 · 物理学 2026-04-21 Tim F. Weiss , Hamed Arianfard , Yang Yang , Alberto Peruzzo

We report direct spectroscopic evidence of correlation-driven Mott states in layered Nb$_3$Cl$_8$ through combining scanning tunneling microscopy (STM) and dynamical mean-field theory. The Hubbard bands persist down to monolayer, providing…

The destructive interference of wavefunctions in a kagome lattice can give rise to topological flat bands (TFBs) with a highly degenerate state of electrons. Recently, TFBs have been observed in several kagome metals, including…

Niobium chloride (Nb3Cl8) is a layered 2D semiconducting material with many exotic properties including a breathing kagome lattice, a topological flat band in its band structure, and a crystal structure that undergoes a structural and…

The Hubbard model provides an idealized description of electronic correlations in solids. Despite its simplicity, the model features a competition between several different phases that have made it one of the most studied systems in…

强关联电子 · 物理学 2023-05-09 Sergii Grytsiuk , Mikhail I. Katsnelson , Erik G. C. P. van Loon , Malte Rösner

By combining ab initio downfolding with cluster dynamical mean-field theory, we study the degree of correlations in monolayer, bilayer and bulk breathing-mode kagome van der Waals materials Nb$_3$(F,Cl,Br,I)$_8$. Our new material-specific…

Colloidal semiconductor nanoplatelets, in which carriers are strongly confined only along one dimension, present fundamentally different excitonic properties than quantum dots, which support strong confinement in all three dimensions. In…

介观与纳米尺度物理 · 物理学 2020-01-08 Daniel Amgar , Gaoling Yang , Ron Tenne , Dan Oron

Integrated quantum optics becomes a consequent tendency towards practical quantum information processing. Here, we report the on-chip generation and manipulation of photonic entanglement based on reconfigurable lithium niobate waveguide…

量子物理 · 物理学 2014-04-02 H. Jin , F. M. Liu , P. Xu , J. L. Xia , M. L. Zhong , Y. Yuan , Y. X. Gong , W. Wang , S. N. Zhu

It has been a longstanding goal in quantum optics to realize controllable sources generating joint multiphoton states, particularly, photon triplet with arbitrary spectral characteristics. We demonstrate that such sources can be realized…

量子物理 · 物理学 2015-05-20 Diana A. Antonosyan , Tigran V. Gevorgyan , Gagik Yu. Kryuchkyan

Electron-hole pair excitations in semiconductors have been predicted to be able to give rise to a highly correlated many-body ground state, the excitonic insulator (EI). Under appropriate conditions below a critical temperature (Tc),…

强关联电子 · 物理学 2023-01-18 Aidan Delgado , Carolin Dusold , Jingwei Jiang , Adam Cronin , Steven G. Louie , Felix R. Fischer

We consider the design of photonic circuits that make use of Ti:LiNbO$_{3}$ diffused channel waveguides for generating photons with various combinations of modal, spectral, and polarization entanglement. Down-converted photon pairs are…

量子物理 · 物理学 2010-09-23 Mohammed F. Saleh , Giovanni Di Giuseppe , Bahaa E. A. Saleh , Malvin Carl Teich

We investigate the electronic reconstruction in (LaNiO$_{3}$)$_n$/(LaAlO$_{3}$)$_3$ (n=3, 5 and 10) superlattices due to the quantum confinement (QC) by d.c. transport and resonant soft x-ray absorption spectroscopy. In proximity to the QC…

强关联电子 · 物理学 2015-05-27 Jian Liu , S. Okamoto , M. van Veenendaal , M. Kareev , B. Gray , P. Ryan , J. W. Freeland , J. Chakhalian

Excitonic band structure is critical for investigating exciton dynamics. Theoretically, quantum effects from exchange scattering between electron-hole pairs significantly modulate exciton dispersion. Here, we report the direct observation…

Third order parametric down-conversion describes a class of nonlinear processes in which a pump photon can be down-converted into triplets of photons. It has been identified as a source of non-classical light, with capabilities beyond those…

量子物理 · 物理学 2022-07-27 Milica Banic , Marco Liscidini , J. E. Sipe

Superconducting circuits are a competitive platform for quantum computation because they offer controllability, long coherence times and strong interactions - properties that are essential for the study of quantum materials comprising…

量子气体 · 物理学 2019-08-06 Ruichao Ma , Brendan Saxberg , Clai Owens , Nelson Leung , Yao Lu , Jonathan Simon , David I. Schuster

Mott transitions in real materials are first order and almost always associated with lattice distortions, both features promoting the emergence of nanotextured phases. This nanoscale self-organization creates spatially inhomogeneous…

Scalable programmable photonic integrated circuits (PICs) can potentially transform the current state of classical and quantum optical information processing. However, traditional means of programming, including thermo-optic, free carrier…

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