相关论文: Thermalization Rate of Light in Weakly Coupled Mol…
A microscopic model for thermal excitation of vibrational ground state of a molecule interacting with a condensed medium is developed. The master equation for evolution of occupancies of the vibrational levels is derived. The rate constant…
The thermoelectric properties of a molecular junction model, appropriate for large molecules such as fullerenes, are studied within a non-equilibrium adiabatic approach in the linear regime at room temperature. A self-consistent calculation…
Bose-Einstein condensation has in the last two decades been observed in cold atomic gases and in solid-state physics quasiparticles, exciton-polaritons and magnons, respectively. The perhaps most widely known example of a bosonic gas,…
In this work, we present a stochastic variational calculation (SVM) of energies and wave functions of few particle systems coupled to quantum fields in cavity QED. The light-matter coupled system is described by the Pauli-Fierz Hamiltonian.…
We study the internal state dynamics of optically trapped polyatomic molecules subject to room temperature blackbody radiation. Using rate equations that account for radiative decay and blackbody excitation between rovibrational levels of…
We investigate the propagation of light with ultra low group velocity in a Bose-Einstein condensate where the phase is not uniform. The light is shown to couple strongly to the phase gradient of the condensate. The interaction between the…
For over a decade, cold atoms in lattice potentials have been an attractive platform to simulate phenomena known from solid state theory, as the Mott-insulator transition. In contrast, the field of photonics usually deals with…
When a charged particle penetrates through an optical interface, photon emissions emerge - a phenomenon known as transition radiation. Being paramount to fundamental physics, transition radiation has enabled many applications from…
A fast optical spectroscopic method for determination rotational ($T_{rot}$) and vibrational ($T_{vib}$) temperatures in two-temperature Boltzmann distribution of the excited state by using machine learning approach is presented. The method…
The interaction between molecules and surface plasmons in defined geometries can lead to new light mater hybrid states where light propagation is strongly influenced by molecular photon absorption. Their application range from lasing LEDs…
We review recent experiments on the Bose-Einstein condensation of photons in a dye-filled optical microresonator. The most well-known example of a photon gas, photons in blackbody radiation, does not show Bose-Einstein condensation. Instead…
We propose an experimental set up allowing to convert an input light of wavelengths about $1-2 \mu m$ into an output light of a lower frequency. The basic principle of operating relies on the nonlinear optical properties exhibited by a…
Understanding how the effectiveness of natural photosynthetic energy harvesting systems arises from the interplay between quantum coherence and environmental noise represents a significant challenge for quantum theory. Recently it has begun…
We theoretically analyze the temperature behavior of paraxial light in thermal equilibrium with a dye-filled optical microcavity. At low temperatures the photon gas undergoes Bose-Einstein condensation (BEC), and the photon number in the…
We derive the transition rates, dephasing rates, and Lamb shifts for a system consisting of many molecules collectively coupled to a resonant cavity mode. Using a variational polaron master equation, we show that strong vibrational…
The optical response of a moving medium suitably driven into a slow-light propagation regime strongly depends on its velocity. This effect can be used to devise a novel scheme for imaging ultraslow velocity fields. The scheme turns out to…
Ensemble averaging of molecular states is fundamental for the experimental determination of thermodynamic quantities. A special case occurs for single-molecule investigations under equilibrium conditions, for which free energy, entropy and…
We construct a theory for Bose-Einstein condensation of light in nano-fabricated semiconductor microcavities. We model the semiconductor by one conduction and one valence band which consist of electrons and holes that interact via a Coulomb…
Strong interaction between light and matter waves, such as electron beams in electron microscopes, has recently emerged as a new tool for understanding entanglement. Here, we systematically investigate electron-light interactions from first…
We experimentally study Bose-Einstein condensation of photons (phBEC) in a dye-filled microcavity. Through multiple absorption and emission cycles the photons inside the microcavity thermalize to the rovibronic temperature of the dye…