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We demonstrate coherent control of both the rotational and hyperfine state of ultracold, chemically stable $^{87}$Rb$^{133}$Cs molecules with external microwave fields. We create a sample of ~2000 molecules in the lowest hyperfine level of…

量子气体 · 物理学 2016-11-02 Philip D. Gregory , Jesus Aldegunde , Jeremy M. Hutson , Simon L. Cornish

We spectroscopically investigate the hyperfine, rotational and Zeeman structure of the vibrational levels $\text{v}'=0$, $7$, $13$ within the electronically excited $c^3\Sigma_g^+$ state of $^{87}\text{Rb}_2$ for magnetic fields of up to…

We report a detailed molecular spectroscopy study on the lowest excited electronic states of $^{23}\rm{Na}^{87}\rm{Rb}$ for producing ultracold $^{23}\rm{Na}^{87}\rm{Rb}$ molecules in the electronic, rovibrational and hyperfine ground…

量子气体 · 物理学 2017-11-22 Mingyang Guo , Romain Vexiau , Bing Zhu , Bo Lu , Nadia Bouloufa-Maafa , Olivier Dulieu , Dajun Wang

We study the combination of hyperfine and Zeeman structure in the spin-orbit coupled $A^1\Sigma_u^+-b^3\Pi_u$ complex of $^{87}\textrm{Rb}_2$. For this purpose, absorption spectroscopy at a magnetic field around $B=1000\:\textrm{G}$ is…

量子气体 · 物理学 2016-12-07 Markus Deiß , Björn Drews , Johannes Hecker Denschlag , Eberhard Tiemann

We produce ultracold dense trapped samples of 87Rb133Cs molecules in their rovibrational ground state, with full nuclear hyperfine state control, by stimulated Raman adiabatic passage (STIRAP) with efficiencies of 90%. We observe the onset…

We report the formation of ultracold $^{7}$Li$^{85}$Rb molecules in the $a^{3}\Sigma^{+}$ electronic state by photoassociation (PA) and their detection via resonantly enhanced multiphoton ionization (REMPI). With our dual-species Li and Rb…

原子物理 · 物理学 2015-06-22 Adeel Altaf , Sourav Dutta , John Lorenz , Jesús Pérez-Ríos , Yong P. Chen , D. S. Elliott

We report our spectroscopic studies of the $d \ ^3\Pi$ state of ultra-cold $^7$Li$^{85}$Rb using resonantly-enhanced multi-photon ionization and depletion spectroscopy with bound-to-bound transitions originating from the metastable $a \…

原子物理 · 物理学 2016-12-21 I. Stevenson , D. Blasing , A. Altaf , Y. P. Chen , D. S. Elliott

We present spectra of ultracold $^7$Li$^{85}$Rb molecules in their electronic ground state formed by spontaneous decay of weakly bound photoassociated molecules. Beginning with atoms in a dual species magneto-optical trap (MOT), weakly…

原子物理 · 物理学 2014-12-24 John Lorenz , Adeel Altaf , Sourav Dutta , Yong P. Chen , D. S. Elliott

We investigate the microwave spectra of ultracold alkali metal dimers in magnetic, electric and combined fields, taking account of the hyperfine structure due to the nuclear spins. We consider the molecules 41K87Rb and 7Li133Cs, which are…

化学物理 · 物理学 2015-05-14 Hong Ran , J. Aldegunde , Jeremy M. Hutson

The simple structure of the BH molecule makes it an excellent candidate for direct laser cooling. We measure the branching ratios for the decay of the ${\rm A}^{1}\Pi (v'=0)$ state to vibrational levels of the ground state, ${\rm…

原子物理 · 物理学 2014-08-06 R. J. Hendricks , D. A. Holland , S. Truppe , B. E. Sauer , M. R. Tarbutt

We report the full control over the internal states of ultracold $^{23}$Na$^{87}$Rb molecules, including vibrational, rotational and hyperfine degrees of freedom. Starting from a sample of weakly bound Feshbach molecules, we realize the…

量子气体 · 物理学 2018-03-07 Mingyang Guo , Xin Ye , Junyu He , Goulven Quéméner , Dajun Wang

Using resonance-enhanced two-photon ionization, we detect ultracold, ground-state RbCs molecules formed via photoassociation in a laser-cooled mixture of 85Rb and 133Cs atoms. We obtain extensive bound-bound excitation spectra of these…

原子物理 · 物理学 2009-11-10 Andrew J. Kerman , Jeremy M. Sage , Sunil Sainis , Thomas Bergeman , David DeMille

We present the results of an experimental and theoretical study of the electronically excited $\tripletex$ state of $^{87}$Rb$_2$ molecules. The vibrational energies are measured for deeply bound states from the bottom up to $v'=15$ using…

原子物理 · 物理学 2015-05-27 T. Takekoshi , C. Strauss , F. Lang , J. Hecker Denschlag , M. Lysebo , L. Veseth

Starting from an ultracold sample of ground-state $^{23}$Na$^{87}$Rb molecules, we investigate the lowest ro-vibrational level of the $b^3\Pi$ state with high resolution laser spectroscopy. This electronic spin-forbidden $X^1\Sigma^+…

原子物理 · 物理学 2021-11-17 Junyu He , Junyu Lin , Romain Vexiau , Nadia Bouloufa , Olivier Dulieu , Dajun Wang

We report the production of a high phase-space density mixture of $^{87}$Rb and $^{133}$Cs atoms in a levitated crossed optical dipole trap as the first step towards the creation of ultracold RbCs molecules via magneto-association. We…

原子物理 · 物理学 2011-07-29 H. W. Cho , D. J. McCarron , D. L. Jenkin , M. P. Köppinger , S. L. Cornish

We describe the theoretical advances that influenced the experimental creation of vibrationally and translationally cold polar $^{40}$K$^{87}$Rb molecules \cite{nphys08,science08}. Cold molecules were created from very-weakly bound…

量子物理 · 物理学 2015-05-13 Svetlana Kotochigova , Eite Tiesinga , Paul S. Julienne

We have measured and analyzed the hyperfine structure of two lines, one at 583nm and one at 401nm, of the only stable fermionic isotope of atomic erbium as well as determined its isotope shift relative to the four most-abundant bosonic…

Ultracold paramagnetic and polar diatomic molecules are among the promising systems for quantum simulation of lattice-spin models. Unfortunately, their experimental observation is still challenging. Based on our recent \textit{ab-initio}…

The formation of ultracold metastable RbCs molecules is observed in a double species magneto-optical trap through photoassociation below the ^85Rb(5S_1/2)+^133Cs(6P_3/2) dissociation limit followed by spontaneous emission. The molecules are…

原子物理 · 物理学 2015-06-03 N. Bouloufa-Maafa , M. Aymar , O. Dulieu , C. Gabbanini

High-resolution spectroscopy on the $A^2\Pi$ - $X^2\Sigma^+$ electronic system of $^{138}$Ba$^{19}$F is performed using a cold molecular beam produced by a buffer gas source. The hyperfine structure in both $X^2\Sigma^+$ ground and $A^2\Pi$…

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