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The laws of quantum mechanics are often tested against the behaviour of the lightest element in the periodic table, hydrogen. One of the most striking properties of molecular hydrogen is the coupling between molecular rotational properties…

Except for ortho- and para-H2, very little is known about nuclear spin isomers (or spin modifications) of molecules. The main reason is the lack of practical enrichment techniques. Recently a few enrichment methods were developed, which…

化学物理 · 物理学 2007-05-23 P. L. Chapovsky , L. J. F. Hermans

Among the factors determining the quantum coherence of the spin in molecular magnets is the presence and the nature of nuclear spins in the molecule. We have explored modifying the nuclear spin environment in Cr$_7$Ni-based molecular…

Controlling electron spins strongly coupled to magnetic and nuclear spins in solid state systems is an important challenege in the field of spintronics and quantum computation. We show here that electron droplets with no net spin in…

介观与纳米尺度物理 · 物理学 2015-06-03 Ramin M. Abolfath , Marek Korkusinski , Thomas Brabec , Pawel Hawrylak

We explore the quantum dynamics of nuclear spin relaxation in cold collisions of $^1\Sigma^+$ molecules with structureless atoms in an external magnetic field. To this end, we develop a rigorous coupled-channel methodology, which accounts…

化学物理 · 物理学 2023-06-29 Rebekah Hermsmeier , Xiaodong Xing , Timur V. Tscherbul

A theoretical model of nuclear spin conversion in molecules controlled by an external electromagnetic radiation resonant to rotational transition has been developed. It has been shown that one can produce an enrichment of spin isomers and…

化学物理 · 物理学 2009-11-06 P. L. Chapovsky

Nuclear spins are known to experience spontaneous long-range correlations only below 2.5 mili-Kelvin in superfluid $^3$He. Here we present the first evidence of nuclear spin coupling in molecular hydrogen (H$_2$) at 74-92 Kelvin using…

材料科学 · 物理学 2016-02-05 Raina J. Olsen , Jon W. Taylor , Cristian I. Contescu , James R. Morris

We present the first quantum mechanical study of hyperfine effects in the rotational cluster states of a symmetric triatomic molecule H$_2$S. Rotational clusters arise from spontaneous symmetry breaking induced by high-angular-momentum…

原子与分子团簇 · 物理学 2025-03-27 Andrey Yachmenev , Guang Yang

Hydrogen molecules have two nuclear spin isomers: ortho-H2 and para-H2. The ortho-to-para ratio (OPR) is known to affect chemical evolution as well as gas dynamics in space. Therefore, understanding the mechanism of OPR variation in…

星系天体物理 · 物理学 2021-12-22 Masashi Tsuge , Akira Kouchi , Naoki Watanabe

The shaping of nuclear spin polarization profiles and the induction of nuclear resonances are demonstrated within a parabolic quantum well using an externally applied gate voltage. Voltage control of the electron and hole wave functions…

介观与纳米尺度物理 · 物理学 2007-05-23 M. Poggio , G. M. Steeves , R. C. Myers , Y. Kato , A. C. Gossard , D. D. Awschalom

The effect of isospin-dependent nuclear forces on the inner crust of neutron stars is modeled within the framework of Quantum Molecular Dynamics (QMD). To successfully control the density dependence of the symmetry energy of neutron-star…

核理论 · 物理学 2022-07-14 Parit Mehta , Rana Nandi , R. O. Gomes , V. Dexheimer , J. Steinheimer

Spin polarized states in nuclear matter with an effective nucleon-nucleon interaction are studied for a wide range of isospin asymmetries and densities. Based on a Fermi liquid theory, it is shown that there are a few possible scenarios of…

核理论 · 物理学 2007-09-22 A. A. Isayev

The nuclear spin--rotation interaction in the hyperfine structure of the hydrogen molecular ion is investigated. The interaction constants are determined and are found to differ in sign and magnitude compared to another theory, but they are…

atom-ph · 物理学 2008-02-03 James F. Babb

We demonstrate a method to quantify and manipulate nuclear spin decoherence mechanisms that are active in zero to ultralow magnetic fields. These include: (i) non-adiabatic switching of spin quantization axis, due to residual background…

化学物理 · 物理学 2022-06-28 Sven Bodenstedt , Morgan W. Mitchell , Michael C. D. Tayler

The main obstacle to coherent control of two-level quantum systems is their coupling to an uncontrolled environment. For electron spins in III-V quantum dots, the random environment is mostly given by the nuclear spins in the quantum dot…

介观与纳米尺度物理 · 物理学 2015-05-13 I. T. Vink , K. C. Nowack , F. H. L. Koppens , J. Danon , Yu. V. Nazarov , L. M. K. Vandersypen

The nucleon is naturally viewed as a bipartite system of valence spin -- defined by its non-vanishing chiral charge -- and non-valence or sea spin. The sea spin can be traced over to give a reduced density matrix, and it is shown that the…

高能物理 - 唯象学 · 物理学 2020-04-22 Silas R. Beane , Peter Ehlers

The nuclear polarization of $\mathrm{H}_2$ molecules formed by recombination of nuclear polarized H atoms on the surface of a storage cell initially coated with a silicon-based polymer has been measured by using the longitudinal double-spin…

原子物理 · 物理学 2012-08-27 The HERMES collaboration

As a nuclear spin model of scalable quantum register, the one-dimensional chain of the magnetic atoms with nuclear spins 1/2 substituting the basic atoms in the plate of nuclear spin free easy-axis 3D antiferromagnet is considered. It is…

量子物理 · 物理学 2008-12-02 A. A. Kokin , V. A. Kokin

Forbidden transitions between energy levels typically involve violation of selection rules imposed by symmetry and/or conservation laws. A nanomagnet tunneling between up and down states violates angular momentum conservation because of…

Spin space groups, formed by operations where the rotation of the spins is independent of the accompanying operation acting on the crystal structure, are appropriate groups to describe the symmetry of magnetic structures with null…

材料科学 · 物理学 2025-07-25 Jesus Etxebarria , J. Manuel Perez-Mato , Emre S. Tasci , Luis Elcoro
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