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Progress in layered van der Waals materials has resulted in the discovery of ferromagnetic and ferroelectric materials down to the monolayer limit. Recently, evidence of the first purely two-dimensional multiferroic material was reported in…

Layered van der Waals two-dimensional (2D) magnets are a cornerstone of ultrathin spintronic and magnonic devices. The recent discovery of a 2D multiferroic with strong magnetoelectric coupling in NiI$_2$ offers a promising platform for the…

材料科学 · 物理学 2024-08-01 Andrey Rybakov , Adolfo O. Fumega , Dorye L. Esteras , Jose L. Lado , José J. Baldoví

Multiferroic materials have garnered wide interest for their exceptional static and dynamical magnetoelectric properties. In particular, type-II multiferroics exhibit an inversion-symmetry-breaking magnetic order which directly induces a…

The discovery of multiferroic behavior in monolayer NiI$_2$ provides a new symmetry-broken state in van der Waals monolayers, featuring the simultaneous emergence of helimagnetic order and ferroelectric order at a critical temperature of…

材料科学 · 物理学 2022-04-06 Adolfo O. Fumega , J. L. Lado

Multiferroic order with the engineered levels of strain in monolayer NiI$_{2}$ is explored based on density functional theory calculations and Monte Carlo simulations. Through the investigation of strain-free monolayer NiI$_{2}$, we find…

材料科学 · 物理学 2022-09-28 Xiao-sheng Ni , Dao-Xin Yao , Kun Cao

The discovery of atomically thin van der Waals ferroelectric and magnetic materials encourages the exploration of 2D multiferroics, which holds the promise to understand fascinating magnetoelectric interactions and fabricate advanced…

In type II multiferroics, noncollinear spin textures are expected to induce electric polarization directly, leading to strong magnetoelectric coupling. Realizing such spin driven multiferroicity in two-dimensional systems, and elucidating…

The search for two-dimensional (2D) van der Waals (vdW) multiferroics is an exciting yet challenging endeavor. Room-temperature 2D vdW few-layer multiferroic is a much bigger insurmountable obstacle. Here we report the discovery of an…

The recent discovery of type-II multiferroicity in monolayer NiI${_2}$ indicated a new pathway for intrinsic magnetoelectric coupling in the two-dimensional limit. However, determining whether this phenomenon is a unique anomaly or a…

Identifying intrinsic noncollinear magnetic order in monolayer van der Waals (vdW) crystals is highly desirable for understanding the delicate magnetic interactions at reduced spatial constraints and miniaturized spintronic applications,…

介观与纳米尺度物理 · 物理学 2023-09-29 Mao-Peng Miao , Nanshu Liu , Wen-Hao Zhang , Dao-Bo Wang , Wei Ji , Ying-Shuang Fu

Altermagnetism, an emergent magnetic phase featuring compensated collinear magnetic moments and momentum-dependent spin splittings, has recently garnered widespread interest. A critical issue concerns whether the unconventional spin…

材料科学 · 物理学 2026-05-28 Wen-Ti Guo , Junqi Xu , Yurong Yang , Haijun Zhang , Huaiqiang Wang

The van der Waals (vdW) type-II multiferroic NiI$_2$ has emerged as a candidate for exploring non-collinear magnetism and magnetoelectric effects in the 2D limit. Frustrated intralayer exchange interactions on a triangular lattice result in…

Understanding magnetoelectric coupling in emerging van der Waals multiferroics is crucial for developing atomically thin spintronic devices. Here, we present a comprehensive first-principles investigation of magnetoelectric coupling in…

材料科学 · 物理学 2026-03-06 Hui-Shi Yu , Xiao-Sheng Ni , Kun Cao

The quasi-two-dimensional antiferromagnet Ni$_2$P$_2$S$_6$ belongs to the family of magnetic van der Waals compounds that provides a rich material base for the realization of fundamental models of quantum magnetism in low dimensions. Here,…

强关联电子 · 物理学 2022-06-24 K. Mehlawat , A. Alfonsov , S. Selter , Y. Shemerliuk , S. Aswartham , B. Büchner , V. Kataev

Two-dimensional antiferromagnetism has long attracted significant interest in many areas of condensed matter physics, but only recently has experimental exploration become feasible due to the isolation of van der Waals antiferromagnetic…

介观与纳米尺度物理 · 物理学 2025-11-21 Cheol-Yeon Cheon , Volodymyr Multian , Kenji Watanabe , Takashi Taniguchi , Alberto F. Morpurgo , Dmitry Lebedev

The family of monolayer two-dimensional (2D) materials hosts a wide range of interesting phenomena, including superconductivity, charge density waves, topological states and ferromagnetism, but direct evidence for antiferromagnetism in the…

材料科学 · 物理学 2021-10-12 Zhuoliang Ni , A. V. Haglund , H. Wang , B. Xu , C. Bernhard , D. G. Mandrus , X. Qian , E. J. Mele , C. L. Kane , Liang Wu

Realizing a state of matter in two dimensions has repeatedly proven a novel route of discovering new physical phenomena. Van der Waals (vdW) materials have been at the center of these now extensive research activities. They offer a natural…

Twisted magnetic van der Waals materials provide a flexible platform to engineer new forms of unconventional magnetism. Here we demonstrate the emergence of electrically tunable topological moir\'e magnetism in twisted bilayers of the…

强关联电子 · 物理学 2025-11-18 Tiago V. C. Antão , Jose L. Lado , Adolfo O. Fumega

Matters Arising in Nature on "Evidence for a single layer van der Waals multiferroic". The search for two dimensional multiferroic materials is an exciting yet challenging endeavor. Recently, Song reported the exciting discovery of type II…

材料科学 · 物理学 2023-07-24 Yucheng Jiang , Yangliu Wu , Jinlei Zhang , Jingxuan Wei , Bo Peng , Cheng-Wei Qiu

The realization of two-dimensional multiferroics offers significant potential for nanoscale device functionality. However, type-I two-dimensional multiferroics with strong magnetoelectric coupling, enabling electric field control of spin,…

材料科学 · 物理学 2025-01-24 Wei Li , Dongyang Zhu , Shuai Dong , Jun-Jie Zhang
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