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High-quality single crystals of NaYbSe$_2$, which resembles a perfect triangular-lattice antiferromagnet without the intrinsic disorder, are investigated by magnetization and specific heat, as well as the local probe techniques nuclear…

We present the low-temperature magnetic properties of two Yb$^{3+}$-based triangular lattice compounds NaSrYb(BO$_3$)$_2$ and K$_3$YbSi$_2$O$_7$ via thermodynamic measurements followed by crystal electric field (CEF) calculations.…

材料科学 · 物理学 2025-01-27 S. Guchhait , R. Kolay , A. Magar , R. Nath

Here, we report the synthesis and magnetic properties of a Yb-based triangular-lattice compound LiYbS$_2$. At low temperatures, it features an effective spin-$\frac{1}{2}$ state due to the combined effect of crystal electric field and spin…

强关联电子 · 物理学 2020-04-22 K. M. Ranjith , Ph. Schlender , Th. Doert , M. Baenitz

Disordered magnetic states known as spin liquids are of paramount importance in both fundamental and applied science. A classical state of this kind was predicted for the Ising antiferromagnetic triangular model more than half a century…

强关联电子 · 物理学 2022-11-15 T. Arh , B. Sana , M. Pregelj , P. Khuntia , Z. Jagličić , M. D. Le , P. Biswas , A. Ozarowski , A. Zorko

Rare-earth delafossites were recently proposed as promising candidates for the realization of an effective $S$=1/2 quantum spin liquid (QSL) on the triangular lattice. In contrast to the most actively studied triangular-lattice…

强关联电子 · 物理学 2020-01-08 R. Sarkar , Ph. Schlender , V. Grinenko , E. Haeussler , Peter J. Baker , Th. Doert , H. -H. Klauss

Quantum spin liquids (QSL) are theoretical states of matter with long-range entanglement and exotic quasiparticles. However, they generally elude quantitative theory, rendering their underlying phases mysterious and hampering efforts to…

We investigated the spin dynamics by electron spin resonance (ESR) of the Yb-based, effective spin-1/2 delafossites NaYbO$_{2}$, AgYbO$_{2}$, LiYbS$_{2}$, NaYbS$_{2}$, and NaYbSe$_{2}$ which all show an absence of magnetic order down to…

The Heisenberg triangular lattice quantum spin liquid and the phase transitions to nearby magnetic orders have received much theoretical attention, but clear experimental manifestations of these states are rare. This work investigates a new…

Employing exact diagonalization, we systematically study the anisotropic Heisenberg model which is related to rare-earth triangular-lattice materials. We probe its full 3D phase diagram afresh and identify a large region of quantum spin…

强关联电子 · 物理学 2021-05-18 Muwei Wu , Dao-Xin Yao , Han-Qing Wu

The quantum spin-1/2 antiferromagnetic Heisenberg model on a two dimensional triangular lattice geometry with spatial anisotropy is relevant to describe materials like ${\rm Cs_2 Cu Cl_4}$ and organic compounds like…

强关联电子 · 物理学 2011-11-09 Seiji Yunoki , Sandro Sorella

Spin-$1/2$ kagome antiferromagnets are leading candidates for realizing quantum spin liquid (QSL) ground states. While QSL ground states are predicted for the pure Heisenberg model, understanding the robustness of the QSL to additional…

Triangular lattice of rare-earth ions with interacting effective spin-$1/2$ local moments is an ideal platform to explore the physics of quantum spin liquids (QSLs) in the presence of strong spin-orbit coupling, crystal electric fields, and…

We report a comprehensive experimental investigation of the structural, thermodynamic, static, and dynamic properties of a triangular lattice antiferromagnet Rb$_3$Yb(VO$_4$)$_2$. Through the analysis of magnetic susceptibility,…

材料科学 · 物理学 2025-06-10 Sebin J. Sebastian , R. Kolay , Abhidev. B , Q. -P. Ding , Y. Furukawa , R. Nath

Motivated by the recent synthesis of two insulating Li$_2$IrO$_3$ polymorphs, where Ir$^{4+}$ $S_{eff}$=1/2 moments form 3D ("harmonic") honeycomb structures with threefold coordination, we study magnetic Hamiltonians on the resulting…

强关联电子 · 物理学 2014-11-26 Itamar Kimchi , James G. Analytis , Ashvin Vishwanath

We study the ground-state properties of the quantum spin liquid (QSL) phases of the spin-$1/2$ antiferromagnetic Heisenberg model on the triangular lattice with nearest- ($J_1$), next-nearest- ($J_2$), and third-neighbor ($J_3$)…

强关联电子 · 物理学 2023-05-10 Yi-Fan Jiang , Hong-Chen Jiang

We study the spin-$1/2$ Heisenberg model on the triangular lattice with the nearest-neighbor $J_1 > 0$, the next-nearest-neighobr $J_2 > 0$ Heisenberg interactions, and the additional scalar chiral interaction $J_{\chi}(\vec{S}_i \times…

强关联电子 · 物理学 2017-08-16 Shou-Shu Gong , W. Zhu , J. -X. Zhu , D. N. Sheng , Kun Yang

An effective quantum pseudospin-1/2 Hamiltonian for Yb_2TM_2O_7 (TM = Ti and Sn) is obtained in terms of the atomic Kramers ground doublet of the LS coupling and the crystalline electric field, which is almost described with J^z=\pm 1/2. It…

强关联电子 · 物理学 2015-05-20 Shigeki Onoda

We derive a quantum spin Hamiltonian of the spin-1/2 zigzag chain realized in a rare earth ytterbium-based magnetic insulator, YbCuS2. This material undergoes a transition at 0.95K to an incommensurate magnetic phase with small moments,…

强关联电子 · 物理学 2024-08-02 Hidehiro Saito , Hiroki Nakai , Chisa Hotta

The delafossite-like compound NaYbO$_2$ hosts a triangular lattice of Yb$^{3+}$ moments and is a promising candidate for the realization of a quantum spin liquid ground state -- an exotic, quantum-disordered magnetic phase featuring…

We study the spin-$1/2$ Heisenberg model on the triangular lattice with the antiferromagnetic first ($J_1$) and second ($J_2$) nearest-neighbor interactions using density matrix renormalization group. By studying the spin correlation…

强关联电子 · 物理学 2015-10-07 Wen-Jun Hu , Shou-Shu Gong , Wei Zhu , D. N. Sheng
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