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High-harmonic generation (HHG) in solids has typically been explored in transparent dielectrics and semiconductors. Metals have long been dismissed due to their strong reflectivity at infrared wavelengths. Here, we demonstrate HHG from…

Since the discovery of high-order harmonic generation (HHG) in solids, much effort has been devoted to understanding its generation mechanism and both interband and intraband transitions are known to be essential. However, intraband…

High harmonic generation (HHG) in solids has recently emerged as a powerful all-optical approach for probing material properties and ultrafast electron dynamics in quantum systems. It has been widely applied for studying two-dimensional and…

光学 · 物理学 2026-04-28 Eyal Uzner , Ofer Neufeld

High harmonic generation (HHG) is a powerful probe of electron dynamics on attosecond to femtosecond timescales and has been successfully used to detect electronic and structural changes in solid-state quantum materials, including…

材料科学 · 物理学 2026-01-21 Daniel A. Rehn , Towfiq Ahmed , Jinkyoung Yoo , Rohit Prasankumar , Jian-Xin Zhu

High-harmonic generation (HHG) is a coherent optical process in which the incident photon energy is up-converted to the multiples of its initial energy. In solids, under the influence of a strong laser field, electron-hole (e-h) pairs are…

High harmonic generation (HHG) from semiconductors and insulators has become a very active area of research due to its great potential for developing compact HHG devices. Here we show that by growing monolayers (ML) of insulators on…

原子物理 · 物理学 2016-12-28 Néstor F. Aguirre , Fernando Martín

We investigate ultrafast harmonic generation (HG) in Si:B, driven by intense pump pulses with fields reaching ~100 kV/cm and a carrier frequency of 300 GHz, at 4 K and 300 K, both experimentally and theoretically. We report several novel…

High-harmonic generation (HHG) in solids has been touted as a way to probe ultrafast dynamics and crystal symmetries in condensed matter systems. Here, we investigate the polarization properties of high-order harmonics generated in…

The long standing issue of separating resonant from non-resonant processes in extreme nonlinear optics is resolved. The theoretical formalism is applied to high harmonic generation (HHG) in solids and reveals a deeper view into the dominant…

光学 · 物理学 2022-06-03 A. Thorpe , N. Boroumand , A. M. Parks , E. Goulielmakis , T. Brabec

High-harmonic generation (HHG) in solids has emerged in recent years as a rapidly expanding and interdisciplinary field, attracting attention from both the condensed-matter and the atomic, molecular, and optics communities. It has exciting…

原子物理 · 物理学 2022-02-09 Lun Yue , Mette B. Gaarde

We theoretically investigate photo-excitation of electron-hole pairs and high harmonic generation in the bulk of zinc oxide (ZnO) subjected to intense femto-second laser pulses with mid-infrared wavelength. The main microscopic mechanism of…

光学 · 物理学 2025-07-15 Boyan Obreshkov , Tzveta Apostolova

High harmonic generation (HHG) is a manifestation of the strongly nonlinear response of matter to intense laser fields and has, as the basis for coherent XUV sources a variety of applications. Recently, HHG from atoms in a phase and…

光学 · 物理学 2020-05-20 Jonas Wätzel , Jamal Berakdar

With a combination of numerical methods, including quantum Monte Carlo, exact diagonalization, and a simplified dynamical mean-field model, we consider the attosecond charge dynamics of electrons induced by strong-field laser pulses in…

强关联电子 · 物理学 2021-10-08 Christopher Orthodoxou , Amelle Zaïr , George H. Booth

We analytically and numerically investigate the emission of high-harmonic radiation from model solids by intense few-cycle mid-infrared laser pulses. In single-active-electron approximation, we expand the active electron's wavefunction in a…

其他凝聚态物理 · 物理学 2019-07-26 Francisco Navarrete , Marcelo F. Ciappina , Uwe Thumm

This Letter brings together two topics that, until now, have been the focus of intense but non-overlapping research efforts. The first concerns high harmonic generation in solids, which occurs when intense light field excites highly…

强关联电子 · 物理学 2022-04-06 R. E. F. Silva , Igor V. Blinov , Alexey N. Rubtsov , O. Smirnova , M. Ivanov

High harmonic generation (HHG) is a highly nonlinear emission process in which systems driven by intense laser pulses emit integer multiples (harmonics) of the driving field. This feature is considered universal to all occurrences of HHG.…

High-order harmonic generation (HHG) in solids has emerged as a versatile platform for exploring ultrafast and quantum-coherent phenomena in condensed matter. Recent advances reveal Berry-phase and topological effects in harmonic emission,…

光学 · 物理学 2025-10-20 Marcelo F. Ciappina

High-harmonic generation (HHG) in crystalline solids have been examined so far on the basis of one-body energy-band structures arising from electron itineracy in a periodic potential. Here, we show emergence of HHG signals which are…

强关联电子 · 物理学 2020-04-22 Shohei Imai , Atsushi Ono , Sumio Ishihara

An analytic description of high harmonic generation (HHG) in solids induced by intense low-frequency pulses is presented within an adiabatic approach, which treats laser-matter interactions nonperturbatively. We derive the analytical…

光学 · 物理学 2026-01-01 A. V. Flegel , Liang-Wen Pi , M. V. Frolov

High-harmonic generation (HHG) normally requires a careful adjustment of the driving laser intensity (typically $10^{14} - 10^{15}$ W/cm$^2$) and gas medium parameters to enable good phase matching conditions. In contrast with conventional…

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