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Piezoelectricity of organic polymers has attracted increasing interest because of several advantages they exhibit over traditional inorganic ceramics. While most organic piezoelectrics rely on the presence of intrinsic local dipoles, a…

材料科学 · 物理学 2025-06-06 Stefano Paolo Villani , Marco Campetella , Paolo Barone , Francesco Mauri

Dabconium hybrid perovskites include a number of recently-discovered ferroelectric phases with large spontaneous polarisations. The origin of ferroelectric response has been rationalised in general terms in the context of hydrogen bonding,…

The oxide heterostructure [(YFeO$_3$)$_5$(LaFeO$_3$)$_5$]$_{40}$, which is magnetically ordered and piezoelectric at room temperature, has been constructed from two weak ferromagnetic AFeO$_3$ perovskites with different A cations using…

Piezoelectrics play a critical role in various applications. The permanent dipole associated with the molecular cations in organometal-halide perovskites (OMHPs) may lead to spontaneous polarization and thus piezoelectricity. Here, we…

材料科学 · 物理学 2015-12-17 Shi Liu , Fan Zheng , Ilya Grinberg , Andrew M. Rappe

We present a detailed first-principles investigation of the structural and polar properties of 3D hybrid perovskite, methylhydrazinium lead chloride, MHyPbCl3, as it transitions from a highly polar Phase-I (high temperature, HT) to less…

材料科学 · 物理学 2025-01-17 Pradhi Srivastava , Sayan Maity , Varadharajan Srinivasan

A comprehensive understand of the intrinsic piezoelectric anisotropy stemming from diverse chemical and physical factors is a key step for the rational design of highly anisotropic materials. We performed high-throughput calculations on…

材料科学 · 物理学 2023-10-26 Fanhao Jia , Shaowen Xu , Shunbo Hu , Jianguo Chen , Yongchen Wang , Yuan Li , Wei Ren , Jinrong Cheng

Spin splitting, or removal of spin degeneracy in the electronic energy band/level is often a measure of spin-orbit coupling strength and a way to manipulate spin degrees of freedom. We use first-principles simulations to predict giant spin…

材料科学 · 物理学 2024-03-18 Nikhilesh Maity , Ravi Kashikar , S. Lisenkov , I. Ponomareva

We present a thorough dielectric investigation of the hexagonal perovskites La1.2Sr2.7IrO7.33 and La1.2Sr2.7RuO7.33 in a broad frequency and temperature range, supplemented by additional infrared measurements. The occurrence of giant…

强关联电子 · 物理学 2016-08-16 P. Lunkenheimer , T. Götzfried , R. Fichtl , S. Weber , T. Rudolf , A. Loidl , A. Reller , S. G. Ebbinghaus

Freestanding ferroelectric oxide membranes emerge as a promising platform for exploring the interplay between topological polar ordering and dipolar interactions that are continuously tunable by strain. Our investigations combining density…

材料科学 · 物理学 2024-07-31 Yihao Hu , Jiyuan Yang , Shi Liu

Halide perovskite semiconductors respond to electric fields in a way that varies across time and length scales. We discuss the microscopic processes that give rise to the macroscopic polarization of these materials, ranging from the optical…

材料科学 · 物理学 2018-12-04 Jacob N. Wilson , Jarvist M. Frost , Suzanne K. Wallace , Aron Walsh

Hybrid organic-inorganic perovskites (HOIPs) have emerged to the forefront of optoelectronic materials advancement in the past few years. Due to the nature of organic compounds within the perovskite structure, its optoelectronic properties…

Titanium based-perovskites have got surprising attraction due to their environmentfriendly photocatalysts behavior. The Rietveld refinement of X-ray diffraction (XRD) pattern authenticates the orthorhombic Pnma structure of Pr2MgTiO6 (PMT).…

材料科学 · 物理学 2023-07-04 Moumin Rudra , T. K. Bhowmik , H. S. Tripathi , R. A. Kumar , R. Sutradhar , T. P. Sinha

Interaction between dipoles often emerges intriguing physical phenomena, such as exchange bias in the magnetic heterostructures and magnetoelectric effect in multiferroics, which lead to advances in multifunctional heterostructures.…

Two-dimensional (2D) hybrid organic--inorganic perovskites (HOIPs) are promising candidates for next-generation optoelectronic and spintronic applications. This work systematically investigates the relationship between structural…

材料科学 · 物理学 2026-04-10 Yue Zhao , Fu Li , Vikrant Chaudhary , Hongbin Zhang , Gaoyang Gou , Niuzhuang Yang , Yue Hao , Wenyi Liu

From lithium-ion batteries to high-temperature superconductors, oxide materials have been widely used in electronic devices. However, demands of future technologies require materials beyond oxides, as anion chemistries distinct from oxygen…

THz-range dielectric spectroscopy and first-principle-based effective-Hamiltonian molecular dynamics simulations were employed to elucidate the dielectric response in the paraelectric phase of (Ba,Sr)TiO3 solid solutions. Analysis of the…

材料科学 · 物理学 2012-11-30 J. Weerasinghe , L. Bellaiche , T. Ostapchuk , P. Kuzel , C. Kadlec , S. Lisenkov , I. Ponomareva , J. Hlinka

The origin of the very large piezoelectric response observed in the vicinity of the morphotropic phase boundary (MPB) in perovskite lead zirconate titanate and related systems has been under intensive studies. Polarization rotation ideas…

材料科学 · 物理学 2009-11-13 Johannes Frantti , Yukari Fujioka , Risto M. Nieminen

Ferroelectrics remain in the focus of scientific attention for decades owing to their fundamental and practical appeal. Recently, ferroelectricity has been demonstrated in semiconducting halide perovskites, offering both a rare combination…

材料科学 · 物理学 2025-06-17 Ravi Kashikar , S. Lisenkov , I. Ponomareva

Recent realizations of ultrathin freestanding perovskite oxides offer a unique platform to probe novel properties in two-dimensional oxides. Here, we observed a giant flexoelectric response in freestanding BiFeO3 and SrTiO3 in their bent…

By means of a model Hamiltonian approach we study the role of volume expansion, Hund's coupling and electron correlation in the standard hybridization mechanism for ferroelectricity in cubic CaMnO$_3$, a prototypical non-$d^0$ perovskite.…

强关联电子 · 物理学 2015-05-30 Paolo Barone , Sudipta Kanungo , Silvia Picozzi , Tanusri Saha-Dasgupta
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