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The classic density-functional theory (DFT) formalism introduced by Hohenberg, Kohn, and Sham in the mid-1960s, is based upon the idea that the complicated N-electron wavefunction can be replaced with the mathematically simpler 1-electron…

化学物理 · 物理学 2015-05-30 M. E. Casida , M. Huix-Rotllant

The expression for the intensity of the electromagnetic field radiation is derived in the approximation next to the dipole one. The presented approach is based on fundamental equations from the introductory course on classical…

经典物理 · 物理学 2018-09-21 Andrij Rovenchak , Yuri Krynytskyi

Important information about strong-field atomic or molecular ionization can be missed when using linearly polarized laser fields. The field strength at which an electron was ionized, or the time during a pulse of the ionization event are…

原子物理 · 物理学 2013-01-31 Xu Wang , J. H. Eberly

State-of-the-art methods for calculating neutral excitation energies are typically demanding and limited to single electron-hole pairs and their composite plasmons. Here we introduce excitonic density-functional theory (XDFT) a…

化学物理 · 物理学 2023-01-09 Subhayan Roychoudhury , Stefano Sanvito , David D. O'Regan

We theoretically investigate the optically-induced demagnetization of ferromagnetic FePt using the time-dependent density functional theory (TDDFT). We compare the demagnetization mechanism in the perturbative and nonperturbative limits of…

材料科学 · 物理学 2024-04-26 M. S. Mrudul , Peter M. Oppeneer

We study ab initio computations of the interaction of Lithium with a strong laser field. Numerical solutions of the time-dependent fully-correlated three-particle Schroedinger equation restricted to the one-dimensional soft-core…

原子物理 · 物理学 2009-11-10 Camilo Ruiz , Luis Plaja , Luis Roso

Emission lines of Be-like ions are frequently observed in astrophysical plasmas, and many are useful for density and temperature diagnostics. However, accurate atomic data for energy levels, radiative rates (A-values) and effective electron…

太阳与恒星天体物理 · 物理学 2015-06-23 K. M. Aggarwal , F. P. Keenan

Modern intense ultrafast pulsed lasers generate an electric field of sufficient strength to permit tunnel ionization of the valence electrons in atoms. This process is usually treated as a rapid succession of isolated events, in which the…

In ion irradiation processes, electronic stopping power describes the energy transfer rate from the irradiating ion to the target material's electrons. Due to the scarcity and significant uncertainties in experimental electronic stopping…

材料科学 · 物理学 2018-05-04 Dillon C. Yost , Yi Yao , Yosuke Kanai

Phase-of-the-phase spectroscopy using two-color colinearly polarized laser pulses has been introduced and experimentally applied to strong-field tunneling ionization in S. Skruszewicz et al., Phys. Rev. Lett. 115, 043001 (2015) and recently…

原子物理 · 物理学 2018-12-05 V. Tulsky , M. A. Almajid , D. Bauer

The time-dependent surface flux (t-SURFF) method is introduced for computing of strong-field infrared photo-ionization spectra of atoms by numerically solving the time-dependent Schr\"odinger equation on minimal simulation volumes. The…

计算物理 · 物理学 2015-05-30 Liang Tao , Armin Scrinzi

The adiabatic approximation in time-dependent density functional theory (TDDFT) yields reliable excitation spectra with great efficiency in many cases, but fundamentally fails for states of double excitation character. We discuss how…

化学物理 · 物理学 2015-05-27 Peter Elliott , Sharma Goldson , Chris Canahui , Neepa T. Maitra

An ultrarelativistic electron beam passing through an intense laser pulse emits radiation around its direction of propagation into a characteristic angular profile. Here we show that measurement of the variances of this profile in the…

等离子体物理 · 物理学 2020-07-01 T. G. Blackburn , E. Gerstmayr , S. P. D. Mangles , M. Marklund

The modern Free-Electron-Lasers generate a highly intense polarized radiation which initiate a sequence of ionization and decay events. Their probability depends on the polarization of each state as function of time. Its complete accounting…

Strong-field enhanced ionization (EI) is a phenomenon in which stretching of interatomic bonds into a distorted molecular geometry leads to an increase in the tunneling ionization rate driven by a strong field. Isolating the momentum…

The dynamics of transient electric fields generated by the interaction of high intensity laser pulses with underdense plasmas has been studied experimentally with the proton projection imaging technique. The formation of a charged channel,…

We study the excitation of electron currents in a transparent cell of sub-millimeter size filled by an atomic gas and illuminated by an intense two-color femtosecond laser pulse. The pulse consists of a strong fundamental component and its…

原子物理 · 物理学 2020-08-26 T. V. Liseykina , S. V. Popruzhenko

We study nondipole effects in multiphoton ionization of a two-dimensional hydrogen-like atom by a flat-top laser pulse of varied intensity. For this purpose, we solve numerically a two-dimensional Schr\"odinger equation treating a…

原子物理 · 物理学 2024-12-25 J. Z. Kamiński , K. Krajewska

Time-dependent density-functional theory (TDDFT) is deemed to be a formally rigorous way of dealing with the time-evolution of a many-electron system at the level of electron densities rather than the underlying wavefunctions, which in turn…

化学物理 · 物理学 2024-11-26 Jochen Schirmer

A theoretical study of laser and plasma based electron acceleration is presented. An effective model has been used, in which the presence of an underdense plasma has been taken account via its index of refraction $n_{m}$. In the confines of…

等离子体物理 · 物理学 2015-10-14 Mihály András Pocsai , Imre Ferenc Barna , Sándor Varró
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