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Direct atomically resolved observation of dynamics deep in the glassy regime has proved elusive for atomic and molecular glasses. Studies below the glass transition temperature Tg are especially rare due to long waiting times required to…

介观与纳米尺度物理 · 物理学 2010-06-10 Sumit Ashtekar , Gregory Scott , Joseph Lyding , Martin Gruebele

In conventional glassformers at sufficiently short times and low enough temperatures, molecules are mutually caged by the intermolecular potential. The fluctuation and dissipation from motion of caged molecules when observed by elastic…

软凝聚态物质 · 物理学 2011-06-30 K. L. Ngai , S. Capaccioli , A. Paciaroni

Amorphous solids exhibit quasi-universal low-temperature anomalies whose origin has been ascribed to localized tunneling defects. Using an advanced Monte Carlo procedure, we create {\it in silico} glasses spanning from hyperquenched to…

无序系统与神经网络 · 物理学 2020-06-17 Dmytro Khomenko , Camille Scalliet , Ludovic Berthier , David R. Reichman , Francesco Zamponi

The element of metastability is incorporated in the fluctuating nonlinear hydrodynamic description of the mode coupling theory (MCT) of the liquid-glass transition. This is achieved through the introduction of the defect density variable…

凝聚态物理 · 物理学 2009-10-22 Joonhyun Yeo , Gene F. Mazenko

We perform experiments with a granular system that consists of a collection of identical hollow spheres (ping-pong balls). Particles rest on a horizontal metallic grid and are confined within a circular region. Fluidization is achieved by…

Supercooled liquids and dense colloids exhibit anomalous behaviour known as "spatially heterogeneous dynamics" (SHD), which becomes increasingly pronounced with approach to the glass transition. Recently, SHD has been observed in confined…

软凝聚态物质 · 物理学 2010-12-23 Aaron S. Keys , Adam R. Abate , Sharon C. Glotzer , Douglas J. Durian

The time evolution of the pore size distributions and mechanical properties of amorphous solids at constant pressure is studied using molecular dynamics simulations. The porous glasses were initially prepared at constant volume conditions…

软凝聚态物质 · 物理学 2018-10-22 Nikolai V. Priezjev , Maxim A. Makeev

Using molecular dynamics simulation, we investigate the slow dynamics of a supercooled binary mixture of soft particles interacting with a generalized Hertzian potential. At low density, it displays typical slow dynamics near its glass…

软凝聚态物质 · 物理学 2016-10-18 Ryoji Miyazaki , Takeshi Kawasaki , Kunimasa Miyazaki

In equilibrium, disorder conspires with topological defects to redefine the ordered states of matter in systems as diverse as crystals, superconductors and liquid crystals. Far from equilibrium, however, the consequences of quenched…

软凝聚态物质 · 物理学 2021-03-09 Amélie Chardac , Suraj Shankar , M. Cristina Marchetti , Denis Bartolo

Previous studies have suggested a conundrum in the relaxation dynamics of polydisperse supercooled liquids. It has been shown that in two dimensions, the relative relaxation times of particles of different sizes become more similar as the…

软凝聚态物质 · 物理学 2025-03-06 Ilian Pihlajamaa , Lotte van Gessel , Corentin Laudicina , Luc van Burik , Liesbeth Janssen

We determine the speed of a crystallisation (or more generally, a solidification) front as it advances into the uniform liquid phase after the system has been quenched into the crystalline region of the phase diagram. We calculate the front…

软凝聚态物质 · 物理学 2013-03-25 A. J. Archer , M. J. Robbins , U. Thiele , E. Knobloch

Using holographic duality, we investigate the impact of finite temperature on the instability and splitting patterns of quadruply quantized vortices, providing the first-ever analysis in this context. Through linear stability analysis, we…

量子气体 · 物理学 2023-12-01 Shanquan Lan , Xin Li , Yu Tian , Peng Yang , Hongbao Zhang

We study in this work the dynamics of a collection of identical hollow spheres (ping-pong balls) that rest on a horizontal metallic grid. Fluidization is achieved by means of a turbulent air current coming from below. The upflow is adjusted…

We report a metadynamics simulation study of crystallization in a deep undercooled metallic glass-forming liquid by developing appropriate collective variables. Through a combined analysis of free energy surface (FES) and atomic-level…

无序系统与神经网络 · 物理学 2020-02-25 Wen-Xiong Song , Yong Yang , Weihua Wang , Pengfei Guan

Dense active systems are widespread in nature, examples range from bacterial colonies to biological tissues. Dense clusters of active particles can be obtained by increasing the packing fraction of the system or taking advantage of a…

软凝聚态物质 · 物理学 2022-04-13 Matteo Paoluzzi , Demian Levis , Ignacio Pagonabarraga

Using molecular dynamics simulations, we have studied the atomic correlations characterizing the second peak in the radial distribution function (RDF) of metallic glasses and liquids. The analysis was conducted from the perspective of…

材料科学 · 物理学 2015-11-13 Jun Ding , Evan Ma , Mark Asta , Robert O. Ritchie

We study the shear induced fluidization of amorphous solids subjected to external loading by investigating the relaxation dynamics of the deformed states using computer simulation. A simple shear deformation is employed at constant rate to…

软凝聚态物质 · 物理学 2021-12-07 Santhosh Kumar R , Bhaskar Sen Gupta

We present simulation results addressing the dynamics of a colloidal system with attractive interactions close to gelation. Our interaction also has a soft, long range repulsive barrier which suppresses liquid-gas type phase separation at…

软凝聚态物质 · 物理学 2007-05-23 Antonio M. Puertas , Matthias Fuchs , Michael E. Cates

We use a swap Monte Carlo algorithm to numerically prepare bulk glasses with kinetic stability comparable to that of glass films produced experimentally by physical vapor deposition. By melting these systems into the liquid state, we show…

软凝聚态物质 · 物理学 2017-10-18 Christopher J. Fullerton , Ludovic Berthier

Diatomic nitrogen is an archetypal molecular system known for its exceptional stability and complex behavior at high pressures and temperatures, including rich solid polymorphism, formation of energetic states, and an insulator-to-metal…