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Attosecond pulses from free-electron lasers have opened the doors to atomic site-specific pumping and probing of quantum systems. Key to their success has been electron beam shaping techniques enabling the generation of sub-femtosecond…

The birth of attosecond light sources is expected to inspire a breakthrough in ultrafast optics, which may extend human real-time measurement and control techniques into atomic-scale electronic dynamics. For applications, it is essential to…

等离子体物理 · 物理学 2016-10-12 X. R. Xu , B. Qiao , Y. X. Zhang , H. Y. Lu , H. Zhang , B. Dromey , S. P. Zhu , C. T. Zhou , M. Zepf , X. T. He

High harmonic generation driven by femtosecond lasers makes it possible to capture the fastest dynamics in molecules and materials. However, to date the shortest attosecond (as) pulses have been produced only in the extreme ultraviolet…

A feasible method is proposed to generate isolated attosecond terawatt x-ray radiation pulses in high-gain free-electron lasers. In the proposed scheme, a frequency chirped laser pulse is employed to generate a gradually-varied spacing…

加速器物理 · 物理学 2017-04-26 Zhen Wang , Chao Feng , Zhentang Zhao

Attosecond light pulses in the extreme ultraviolet have drawn a great deal of attention due to their ability to interrogate electronic dynamics in real time. Nevertheless, to follow charge dynamics and excitations in materials, element…

原子物理 · 物理学 2016-06-08 S. M. Teichmann , F. Silva , S. L. Cousin , M. Hemmer , J. Biegert

The duration of isolated attosecond pulses created via high-order harmonic generation is determined by the number of optical cycles in the driving laser. Achieving shorter attosecond soft X-ray pulses requires minimizing the number of…

光学 · 物理学 2025-11-03 Kaito Nishimiya , Rambabu Rajpoot , Eiji J Takahashi

Attosecond pulses, produced through high-order harmonic generation in gases, have been successfully used for observing ultrafast, sub-femtosecond electron dynamics in atoms, molecules and solid state systems. Today's typical attosecond…

High-repetition-rate attosecond pulse sources are indispensable tools of time-resolved studies of electron dynamics, such as coincidence spectroscopy and experiments with high demands on statistics or signal-to-noise ratio, especially in…

Attosecond pulses from X-ray free-electron laser (XFEL) have opened new opportunities for probing ultrafast electronic dynamics on the Angstrom--attosecond spatiotemporal scale. Most attosecond XFEL concepts rely on generating an ultrashort…

加速器物理 · 物理学 2026-04-22 Chenzhi Xu , Jiawei Yan , Ye Chen , Winfried Decking , Marc Guetg , Tianyun Long , Bingyang Yan , Haixiao Deng

We propose a technique for the production of attosecond X-ray pulses which is based on the use of X-ray SASE FEL combined with a femtosecond laser system. A few-cycle optical pulse from a Ti:sapphire laser interacts with the electron beam…

加速器物理 · 物理学 2009-11-10 E. L. Saldin , E. A. Schneidmiller , M. V. Yurkov

Attosecond X-ray pulses are a critical tool for tracking ultrafast electron dynamics in condensed matter, molecular systems, and strongly correlated materials. Recent breakthroughs have pushed X-ray free electron lasers (XFELs) into the…

加速器物理 · 物理学 2026-01-21 Bingyang Yan , Chenzhi Xu , Si Chen , Duan Gu , Ye Chen , Jiawei Yan , Haixiao Deng

We propose a scheme for generation of single 100 GW 300-as pulse in the X-ray free electron laser with the use of a few cycles optical pulse from Ti:sapphire laser system. Femtosecond optical pulse interacts with the electron beam in the…

加速器物理 · 物理学 2009-11-10 E. L. Saldin , E. A. Schneidmiller , M. V. Yurkov

Attosecond pulses in the soft-X-ray (SXR) to water-window energy region offer the tools for creating and studying target specific localized inner-shell electrons or holes in materials, enable monitoring or controlling charge and energy…

原子与分子团簇 · 物理学 2020-03-25 Zhao Xi , Wang Su-Ju , Yu Wei-Wei , Wei Hui , Lin C. D

Parametric amplification of attosecond coherent pulses around 100 eV at the single-atom level is demonstrated for the first time by using the 3D time-dependent Schr{\"o}dinger equation in high-harmonic generation processes from excited…

光学 · 物理学 2020-08-26 C. Serrat , J. Seres , E. Seres , T-H. Dinh , N. Hasegawa , M. Nishikino , S. Namba

In this paper, we present the analytical theory of attosecond pulse formation via optical modulation of an active medium of the hydrogen-like C5+ plasma-based X-ray laser at 3.4 nm wavelength in the "water window" range, taking into account…

光学 · 物理学 2021-01-04 V. A. Antonov , I. R. Khairulin , Olga Kocharovskaya

Generating ever-shorter and brighter light pulses has long been a central pursuit in ultrafast science, as it benchmarks our ability to create and manipulate the coherence on the intrinsic timescale of sub-atomic electron motion. The…

High-order harmonic generation from atomic systems is considered in the crossed fields of a relativistically strong infrared laser and a weak attosecond-pulse train of soft x-rays. Due to one-photon ionization by the x-ray pulse, the…

原子物理 · 物理学 2009-11-13 Michael Klaiber , Karen Z. Hatsagortsyan , Carsten Müller , Christoph H. Keitel
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