相关论文: Ionic strength-driven cavitation nucleation: from …
Laser-induced cavitation in liquids originates from optical breakdown processes that depend sensitively on both laser-plasma dynamics and the chemical microenvironment of the solvent. Herein, we experimentally decouple the effects of ionic…
We demonstrate that a cavitation bubble initiated by a Nd:YAG laser pulse below breakdown threshold induces crystallization from supersaturated aqueous solutions with supersaturation and laser-energy dependent nucleation kinetics. Combining…
Despite its relevance in biology and engineering, the molecular mechanism driving cavitation in water remains unknown. Using computer simulations, we investigate the structure and dynamics of vapor bubbles emerging from metastable water at…
Bubble nucleation in water induced by boiling, gas supersaturation or cavitation usually originates from pre-existing gas cavities trapped into solid defects. Even though the destabilization of such gas pockets, called nuclei, has been…
We present an in-depth analysis of the energy dependence of optical breakdown in water by tightly focused laser pulses, from plasma formation to shock waves and cavitation. Laser pulses of fs to ns durations and UV to IR wavelengths are…
We investigate the role of nuclear motion and strong-field-induced electronic couplings during the double ionization of deuterated water using momentum-resolved coincidence spectroscopy. By examining the three-body dicationic dissociation…
Water at negative pressures can remain in a metastable state for a surprisingly long time before it reaches equilibrium by cavitation, i.e. by the formation of vapor bubbles. The wide spread of experimentally measured cavitation pressures…
Laser-induced cavitation under nanosecond optical breakdown is central to applications such as laser-induced forward transfer, microsurgery, and microfluidic actuation, yet the physical origin of the earliest cavity and its connection to…
Water can exist in a metastable liquid state under tension for long times before the system relaxes into the vapor via cavitation, i.e., bubble nucleation. Microscopic information on the cavitation process can be extracted from experimental…
In this work, we present experiments and simulations on the nucleation and successive dynamics of laser-induced bubbles inside liquid droplets in free-fall motion, i.e. a case with a free boundary in all directions. The droplets of a…
Cavitation has historically been related to parameters measured at equilibrium, such as vapor pressure and surface tension. However, nucleation might occur when the liquid is metastable, especially for fast phenomena such as cavitation…
We use molecular dynamics simulations of the primitive model of electrolytes to study the ionic structure in aqueous monovalent electrolyte solutions confined by charged planar interfaces over a wide range of electrolyte concentration,…
Ionic liquids are widely used as electrolytes in electrochemical devices. In this context, many experimental and theoretical approaches have been recently developed for characterizing their interface with electrodes. In this perspective…
In this paper, the Rayleigh scattering method is used to study the formation of cavitation in water in a pulsed inhomogeneous electric field when a nanosecond high voltage pulse is applied to a needle-like electrode. The observational…
Cavitation, the formation of vapor bubbles in metastable liquids, is highly sensitive to nanoscale surface defects. Using molecular dynamics simulations and classical nucleation theory, we show that pure water confined within defect-free…
This research demonstrates high-repetition-rate laser-accelerated ion beams via dual, intersecting, counterpropagating laser-driven blast waves to precisely shape underdense gas into long-lived near-critical density targets. The collision…
A model for the excitation of a non-linear ion-wake mode by a train of plasma electron oscillations in the non-linear time-asymmetric regime is developed using analytical theory and particle-in-cell based computational solutions. The…
The composition of the gaseous phase of cavitation bubbles and its role on the collapse remains to date poorly understood. In this work, experiments of single cavitation bubbles in aqueous ammonia serve as a novel approach to investigate…
We report the results obtained by cavitating water solutions of iron salts (iron chloride and iron nitrate) with different concentrations at different ultrasound powers. In all cases we detected a neutron radiation well higher than the…
Ionic liquid ion sources are a promising technology that can be used for many applications from space propulsion to focused ion beam microetching. Ionic liquid ion sources produce ion beams by extracting single ions and metastable solvated…